100211 nuclear power

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    Instrumentation seminar, KTH 20100211

    The future of nuclear power in Sweden & Europe

    Janne Wallenius

    Professor

    Reactor Physics, KTH

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    Whats going on?

    New policy on nuclear power in Sweden

    Deployment of Generation III reactors

    Research on Generation IV reactors

    The Swedish GENIUS project

    European Sustainable Nuclear Industrial Initiative

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    Out of the dungeon

    February 2009: Swedish Government announces changeof nuclear policy: New nuclear plants may be built if

    1. they replace old power plants

    2. they are located at the site of existing plants

    Text of law circulated for comments in December 2009

    Increased liability for accidents: 700 M -> 1200 m

    Minimum liability for nuclear facility: 80 M

    Decision to be taken by Riksdagen in June 2010.

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    When do we need new nuclear power?

    Technical lifetime of a power plant highly individual

    Most parts can be replaced except for primary vessel

    Vessel life time depends on radiation induced embrittlement of welds.

    Ductile to brittle transition temperature increased from -100C to >100C for some reactors in operation

    Ringhals 3 &4 have serious issues with nickel precipitation in welds.

    O1 and Ringhals reactors to be replaced in 2020s

    F3 and O3 may stay in good condition beyond 2045, possibly to 2065

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    What we might build now

    Generation III +: Water cooled reactors withpassive safety systems dramatically decreasing the probability for core melt

    Examples

    Westinghouse AP1000 (1100 MWe)

    Under construction in China

    GE-Hitachis ESBWR (1500 MWe)

    Pump free design ->

    Core melt frequency < 1 in 10 million years

    AP1000

    ESBWR

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    What is being built

    Finland and France are building EPRs

    China: Two AP1000 reactors under construction

    USA: Non-nuclear work to prepare site for AP1000build has started (License yet to be granted)

    > 50 power reactors presently under construction.

    ~ 420 projects announced, including UK, Italy,

    Switzerland, Bulgaria, Lithuania, Estonia, Poland,Belarus, The Czech republic, Slovakia, Slovenia,Romania & The Netherlands

    EoN investigating the potential for replacement of O1

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    Generation IV objectives

    Generation IV reactors ought to:

    Increase fuel resources (breed ssile nuclides from 238 U or 232 Th)

    Reduce long term radio-toxic inventory in waste streams (Recycle of

    americium and curium).

    Operate at higher temperature,

    to improve electricity conversion factors

    and/or allow commercial utility of heat production

    The economical feasibility of Gen-IV reactors is directly related to the life-time of structural materials.

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    Implications of sustainability criteria

    Breeding requirement implies: > 2.0

    Fast spectrum system operating on U-

    Pu cycle

    (239 Pu) ~ 2.4 2.6

    True thermal spectrum systemoperating on Th-U cycle:

    (233 U) ~ 2.300

    1

    2

    3

    4

    10 1 10 3 10 5 10 710 -3 10 -1

    neutron yield/absorption

    En[eV]

    239 Pu

    233 U

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    Thermal spectrum system: High temperaturereactor with coated particle fuel (HTR).

    HTR operation on Th based fuel technically feasible

    Reprocessing of coated particle fuel cumbersomeand expensive, involving burning of activated

    graphite.

    Thermal spectrum: excessive production of Cf-252.

    VHTR concept (T 900C to permit H 2 production)lacks suitable materials for primary heat exchangers.

    Composite SiC-SiC materials potential solution.

    Arevas proposed ANTARES reactor for industrialapplication: Process heat @ 600 700C, with oncethrough fuel cycle. Arevas ANTARES

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    Fast versus thermal spectrum

    In order to reduced radio-toxic inventory of spentnuclear fuel, both Pu, Am & Cm must be recycled!

    In a thermal spectrum, ssion probability of evenneutron number nuclides ~ 0

    Build-up of the strong neutron emitter Cf-252 in athermal spectrum is 23 orders of magnitude higher!

    0.2 0.4 0.6 0.8 1

    247 Cm

    246 Cm

    245 Cm

    244 Cm

    243 Am

    241 Am

    242 Pu

    241 Pu

    240 Pu

    239 Pu

    238 Pu

    Fissionprobability

    10 2 10 3 10 4 10 5 10 6

    0.01

    0.1

    1

    10

    100

    10 1

    Radiotoxic inventory [Sv/g]

    243 Am

    242 Pu

    239 Pu238 Pu

    240 Pu

    237 Np

    241 Am

    TRU

    t [y]

    Unat

    0.001

    0.01

    0.1

    1

    10

    100Radiotoxic inventory [Sv/g]

    10 2 10 3 10 4 10 5 10 610 1

    TRU

    FP

    Uranium in nature

    t[y]

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    Fast spectrum systems: common issues

    All fast spectrum systems permit breeding ratio 1 and fullrecycling of Am & Cm from own spent fuel.

    Cf-252 production 23 orders of magnitude lower than in a

    thermal spectrum.

    Ability to accept legacy Am from LWRs depend on design.

    Fast neutron recoils lead to radiation damage

    Swelling of austenitic (fcc) steels

    Embrittlement of ferritic (bcc) steels

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    Sodium cooled fast reactor

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    Fast spectrum systems:Sodium cooled fast reactor

    + Based on coolant technology proven on industrial scale

    + Large demonstration facility may be ready by 2020

    + Good breeding performance

    Costs for prevention of sodium-water interaction

    Safety issues related to coolant boiling

    Phnix MarcouleFrance

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    Lead cooled fast reactor

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    Lead cooled fast reactor

    + No chemical interaction with water (no intermediateheat exchanger)

    + High boiling temperature low probability for coolant voiding

    + High fraction of natural circulation passive heatremoval

    Coolant technology proven only in military sub-marines

    Costs for corrosion control & surface protection

    Erosion of pump blade surfaces

    K745Sovietsubmarine

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    Swelling

    SS316 cladding tubes irradiated to

    80 dpa at 510C.

    33% increase in volume

    Swelling due to formation of voidsunder irradiation

    Leads to void induced embrittlement

    Beforeirradiation

    Afterirradiation

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    Dose limits for austenitic steels

    Best available austeniticsteel applicable for doses upto about 120 dpa

    Corresponds to three yearlifetime of fuel cladding atdose rate of 40 dpa/year

    Dose rate dependencesignicant lower dose rate

    reduces swelling threshold!

    Ferritic-Martensitic steelsswells considerably less

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    Choice of steels for fast neutron reactors

    Austenitic steels (1515Ti) qualiedfor application in Gen-IV reactorsup to doses of ~120 dpa at T < 900 K.

    Ferritic-Martensitic steels are more

    radiation resistant, but have poorcreep strength at high temperature.

    Oxide dispersion strengthened(ODS) steels may perform better,but welding is difcult:

    Example of ODS steel

    Fe-14Cr-1Ti-0.3Mo-0.25Y 2O3before irradiation

    oxides

    480C - 80 dpa (Phnix)

    Oxides

    ! particleHalo!

    halo of fine oxides around thebiggest oxides

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    GENIUS project

    Generation IV research in Swedish Universities (KTH, Chalmers & UU)

    36 MSEK funding from VR for three years. 10 PhD students, 18 seniorscientists involved

    Major activities

    Fuel development: fabrication and characterisation of (U,Pu)N & (Pu,Zr)Nfuels

    Materials research: Radiation damage modelling & characterisation,experimental investigation of corrosion kinetics in lead-alloys

    Safety: Fuel-coolant interaction, nuclear data, thermal-hydraulics of lead,transient analysis, fast neutron detector development, safe-guards.

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    Nitride fuel fabrication laboratory at KTH

    Glove boxes, furnace and milloperative in January 2009

    Nitride powders produced by hydriding/nitriding of metallicsource materials

    Pressing of green UN and ZrNpellets to 70% density

    Spark plasma sintering of ZrNperformed

    Coolant compatibility tests to beconducted within GENIUS.

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    TALL loop

    TALL lead-bismuth loop constructed atKTH in 2004.

    Used for test of heat removal by naturalcirculation

    Unique facility in Europe

    Data now used for code validation

    Extensive use within EU projects

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    European Sustainable NuclearIndustrial Initiative (ESNII)

    Research, Development and Demonstration of sustainable nuclearpower generation. Priority given to

    Sodium cooled fast reactor with power of 250600 MWe, to start

    operation in 2022.

    Experimental lead or gas cooled fast reactor with power of 50100MWe, to gain experience with an alternative coolant, startingoperation in 2025.

    Meeting in Brussels tomorrow to establish Concept Plan of ESNII.

    Indicative cost (including fuel fabrication plants and researchinfrastructure): ~10 G .

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    ASTRID

    ASTRID: Advance Sodium Test Reactor for Industrial Demonstration

    EU-project ESFR: Funded with 6 M

    MOX driver fuel

    Test assemblies with Am containing MOX fuel, Am originating from decay of 241 Pu.

    Major design item: Application of ODS steels or not. These could permithigher burn-up, thus compensating for high costs of sodium management.

    Location: Next to Phnix

    2010: Choice of power

    2012: Decision to build

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    Lead Cooled Advanced Experimental Reactor:LEADER

    EU-project approved in August 2009.

    EC-contribution: 3 M

    Objective: Design of 100 MW e Experimental Technology Demonstration Plant

    Major material issues:

    Validation of GESA technique for surface alloying (FeCrAlY)

    Material for pumps: MAXTAL?

    KTH participates in safety work package

    KTH leads work package on education

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    Concluding remarks

    Nuclear renaissance now in full progress.

    Future reactors based on fast neutron spectrum will increase fuelresources by a factor of 100 & reduce time for storage by a factor of 100!

    Sodium Fast Reactor (SFR) demo likely to by built (ASTRID)

    Decision on alternative technology (lead or gas) to be taken in 2012.

    Development of ODS steels presently major effort

    Feasibility of LFR depends on validation of corrosion and erosion resistantmaterials

    Swedish Gen-IV research conducted within GENIUS project