1969 AUDIT OF SRP RADIOACTIVE WASTE

bY

C . Ashley

Apr i l 1970

Radiological Sciences Division Savannah River Laboratory

E. 1. du Pont de Nemours & Co. Aiken, South Carolina 29801

DISCLAIMER

Portions of this document may be illegible in electronic image products. Images are produced from the best avaiiable original document.

. . .

CONTENTS

Page

In t roduc t ion . . . . . . . . . . . . . . . . . . . . . . . . 5

Summary . . . . . . . . . . . . . . . . . . . . . . . . . . 5

Releases t o t h e Atmosphere . . . . . . . . . . . . . . . . . 6

Separa t ions Areas . . . . . . . . . . . . . . . . . . . . 6

TNX and Building 773-A . . . . . . . . . . . . . . . . . 8 Reactor Areas . . . . . . . . . . . . . . . . . . . . . . 7

Releases t o Ef f luen t Streams . . . . . . . . . . . . . . . . 8

Separa t ions Areas . . . . . . . . . . . . . . . . . . . . 8

DArea . . . . . . . . . . . . . . . . . . . . . . . . . 8

Reac to rAreas . . . . . . . . . . . . . . . . . . . . . . 9

R a w Materials Area . . . . . . . . . . . . . . . . . . . 9

Releases t o Seepage Basins . . . . . . . . . . . . . . . . . 10

Waste t o Bur ia l Ground . . . . . . . . . . . . . . . . . . . 1 2

Separa t ions Areas Waste Storage Tanks . . . . . . . . . . . 13

Appendix

Table I . Summary o f Radioact ive Waste Releases by Indiv idua l Areas . . . . . . . . . . . . . . . 1 4

I1 . 1969 Releases t o Atmosphere from Separa t ions Areas S tacks . . . . . . . . . . . . . . . . . 15

I11 . 1969 Releases t o Ef f luen t Streams from Disassembly Basins . . . . . . . . . . . . . . 16

IV . 1969 Releases t o Separa t ions Areas Seepage Basins . . . . . . . . . . . . . . . . . . . . 18

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INTRODUCTION

This report summarizes releases of radioactive waste to the

Total quantities of radioactive waste released from plant environs of the Savannah River Plant during the calendar year 1969. startup through 1969 are also reported. Accuracy is not always implied to the degree indicated by the number of significant figures reported. Values were not rounded off, since data will be used in future cumulative summaries. No explanations are given for unusual releases; this information may be found in the Radiological Sciences Division Monthly Reports and in the Semi- annual and Annual Environmental Monitoring Reports for 1969.

SUMMARY

Total quantities of radioactive waste released from the Savannah River Plant t o the atmosphere, to effluent streams, and to earthen seepage basins during 1969 and during the 16-year period from plant startup through 1969 are presented in the following table. total quantities are listed in Table I in the Appendix.

Contributions by individual plant areas to these

To E f f l u e n t To Seepage To Atmosphere S trearns Basins

Tota l Tota l Tota l S ince S ince S ince

P l a n t P1 a n t P l a n t 1969 S t a r t u p 1969 S t a r t u p 1969 S t a r t u p

Alpha, m i l l i c u r i e s 709.1 4347 1334 21572 3529 19749

Nonvo la t i l e b e t a , c u r i e s 15.0 131.4 232 12984 589.3 7585

Radio iodine , c u r i e s 35.9 2448 5.0 230a 15.9 2618

Tritium, k i l o c u r i e s 458 13460 64.1 778.1' 47.2 408'?

Noble g a s e s , megacuries 0 .62 d - - - - ("Kr and 1 3 1 y 1 3 3 X e )

a. Analyses began Ju ly 1960. b. Reactor a r e a s d i scha rge ana lyses began January 1958;

s e p a r a t i o n s a r e a s d ischarge ana lyses began J u l y 1958. e. Since January 1957. d. Not r epor t ed because o f s e c u r i t y c l a s s i f i c a t i o n .

- 5 -

. .

Total quantities of radioactive waste committed to the burial ground during 1969 and during the through 1969 are presented in the

P utonium, c u r 239Pu 2 3 8 P u

Uranium, grams E& ched Natura l

16-year period from plant startup following table.

To B u r i a l Ground Total S i n c e

1969 P l a n t S t a r t u p es

107 .2 1014.7 421.6 8753.1

Other a1 pha e m i t t e r s , curies

Gamma, k i l o c u r i e s F i s s i o n Induced

T r i t i u m , k l o c u r i e s

- 145 - 53.59 x 105

13679.1 14306.0

13 .75 386.82 113.89 1584.81

375.8 5165.90

Estimated quantities of fission products in underground storage tanks, as of December 20, 1969 totaled 464 megacuries in F Area and 335 megacuries in H Area (data provided by Separations Technology Section).

RELEASES TO THE ATMOSPHERE

Separations Areas

The quantities of radioactivity released from separations areas stacks during 1969 are presented in the following table. F- and H-Area chemical separations plant releases include specific radionuclide distribution, as determined by gamma spectrometry and radiochemical analyses; radioisotopes of the noble gases were estimated. separations areas stacks (except noble gases) is presented in Table I 1 in the Appendix.

The monthly distribution of radionuclides released from

Stack-released radioactivity from Building 235-F, a special facility which began operation in February 1961, was very low (0.1 mCi of nonvolatile beta and 12.4 pCi of alpha).

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. -. , i

SEPARATIONS AREAS STACK RELEASES DURING 1969

H Area F Area \ Jan- Jul- Jan- Jul- 1969 ToJdl

* _ _ _ _ _ Jun Dec J u n Dec _I_ F Area ICK~Y::~ __ Nonvolatile beta , mCi

3 R u 57.8 49.8 9199.2 308.6 107.6 950/.:: 6Ru 51.3 61.5 1086.5 2913.6 112.8 4000.1

e 9 '90s)" 3.9 3.1 94.7 73.7 7.0 10;:.4 5Zr-95Nb 32.1 28.1 178.1 47.2 60.2 225.3 ' 37cs 3.6 5.1 34.8 41 - 8 8.7 7 6 . 6

781.7 I 4 l > l 4 ' + c e 15.4 14.0 633.1 148.6 29.4 Total 164.1 161.6 11226.4 3473.5 325.7 14699.9

- - - - - - _

Alpha, m C i Radioiodine, mCi Tritium, k C i "Kr, M C i

13'xe, C i l 3 3Xe, k C i

14.39 23.71 600.06 49.31 38.10a 649.37tJ 1456 1161 13636 19696 2617- 33331

151.3 122.0 2 7 2 . 3

~~ ~

a. 5% 2 3 9 P u . b. 9% 2 3 9 P u and 86% a 3 e P u .

Reactor Areas

Nonvolatile beta radioactivity that came from the stack exhaust systems of the reactor buildings during 1969 Consisted primarily of atmospheric fission product fallout (from nuclear weapons tests), which had been drawn into the ventilation systems, Quantities of other radioisotopes, identified by gamma spectrometry, were too low to permit accurate specific analyses. Alpha releases from reactor area stacks were negligible. lived argon-41 produced by neutron activation of atmospheric argon were not calculated routinely.

Releases of the short-

REACTOR AREAS STACK RELEASES DURING 1969

P L K C Total ~ _ _ _ _ _ _ _ _ _ _ _ Nonvo 1 a t i 1 e b e t a , m C i

Jan-Jun Jul-Oec Total

Tri t i u r n , k C i

Jan-Jun Jul -Dec Total

0.233 - 0.155 0.145 0.533 0.142 - 0.300 0.190 G.632 p__--____

0.375 - 0.455 0.335 1.165

15.7 - 37.8 28.4 81.9 1 7 . 4 - 49.0 35.6 102.0 ___ __ ___ ~ ____.

33.1 - 86.8 64.0 183.9

TNX and Building 773-A

TNX AND BUILDING 773-A STACK RELEASES DURING 1969

Bldg 773-A TNX l 3 I 1 , mci 3.75 -

‘ O C O , mci 10.99 Other fission products, m C i 10.27 -

Cm-Am 21.13 - Other alpha emitters, m C i 0.46 - T r i t i u m , C i 120 21 40

RELEASES TO EFFLUENT STREAMS

Separations Areas

The quantities of radioactivity released to Four Mile Creek from F and H Areas during 1969 are shown in the following table.

RELEASES TO FOUR MILE CREEK DURING 1969

Nonvol a ti 1 e Migration from Seepaqe Basins Alpha, mCi Beta, m C i a Tritium, C i 9QSr , m C i

F Area H Area F Area H Area F Area H Area F Area H Area -------- Jan-Jun 2.7 4.1 132 68 1625 1888 248 l o

1 7 Jul-Dec 1.8 2.0

Total 4.5 6.1 229 176 2589 3522 440 27 - - - - 108 964 1634 192 - - - - 97

a. An add i t iona l 1 .9 Ci o f I3’Cs was r e l eased from H Area to Four Mile Creek. s p i l l i n May 1967.

This a c t i v i t y i s desorbing from the stream bed s i n c e the

D Area

Releases of radioactive materials from Buildings 772-D and 421-2D (Waste Storage Tank) are shown in the following table.

RELEASES TO 400-0 EFFLUENT DURING 1969

Nonvolat i le Beta , C i T r i t i u m , C i 0.24 10,502

1 4 1 , 1 4 4 ~ ~ The nonvolatile beta consisted yimarily of (0.05 Ci), 95Zr-95Nb (0.11 Ci), 06Ru (0 .02 Ci), 58y60C0 (0.01 Ci), 3 5 S ( 0 . 0 3 Ci), 65Zn (0.01 Ci), and 89’90~r (0.01 Ci).

Reactor Areas

Disas,sembly bas in water was t h e major sou rce of r a d i o a c t i v e l i q u i d yas6.e r e l eased t o t h e r e a c t o r areas e f f l u e n t streams. q u a n t i t i e s of r a d i o a c t i v e material r e l e a s e d from t h e b a s i n s t o t h e streams during 1969 are p resen ted i n t h e fo l lowing t a b l e . Monthly releases f o r each r e a c t o r area are p resen ted i n Table I11 of t h e Appendix.

The

REACTOR AREAS RELEASES TO STREAMS DURING 1969

Annual Operating

Release Guide L - M i scel 1 aneousa Total Radionucl ides

Shor t - l i ved , C i (t+ < 30 days)

239Np "Cr

2P

1 ' + 0 ~ a - ' " O ~ a 1 3 1 1

P K C

1,500 2,500

0.84 38.45 1.05 4.12 0.21

24.86 0.21 25.91

0.25 0.0001 1.30 0.50 0.023 5.04 0.22 - 0.73

45.65 0.24 101 -52

19.82 0.008 68.54 -

10.26

0.40 0.30

- 100 100 15

44.67 10.96 Total

Long-lived, C i ( t 4 > 30 days )

9 1 Y 1 4 1 3 1 4 4 ~ ~

1 0 3 3 1 0 6~~

"Zr- "Nb 'Zn

6 o c o 1 3 4 , l 37cs

89Sr OSr ss

I4'Prn

0.93 1.38 0.27 0.02

9.69 5.48 0.50 3.59 1.55 0.27 20.05 8.82 3.33 64.42 14.56

50 75 25 40 50 25 80

100 10 250 50

1.47 1.66 0.10 0.41 0.53

3.54 0.77 0.80 36.20 4.11

49.59

-

5.91 3.50 0.40 3.17 1.01 0.20 13.07 6.51 1.52 23.43 8.15

66.87

- 0.028 0.0004 0.010 0.009 0.066

<o. 0001 0.004

3.44 - 0.23 1.31 0.59 0.42 - 4.72 0.14 2.16

5.60 10.01 -_I_

- 0.073 - i

0.19 132.26 Total

T r i t i u m , C i 10,803 891 1971 9904 11,232 34,801 100,000

a . From sources o the r t h a n disassembly basins.

Raw Materials Area

Uranium i s t h e predominant r a d i o a c t i v e c o n s t i t u e n t i n l i q u i d The q u a n t i t y o f uranium r e l e a s e d t o t h e waste from t h e 300 Area.

e f f l u e n t stream (Tims Branch -Upper Three Runs Creek) during 1969 is shown i n t h e fol lowing t a b l e .

RELEASES TO 300-AREA EFFLUENT DURING 1969

Uranium, m C i

Jan-Jun 944 Ju l -Dec 31 8

Tota l 1 26Za

a. Annual Operating Release Guide, 2 Cilyr .

RELEASES TO SEEPAGE BASINS

The quantities of radioactivity released to the separations areas, Ford Building, 700 Area, CMX-TNX, and reactor areas seepage basins during 1969 are presented in the following tables. The monthly distribution of specific radionuclides released to the separations areas seepage basins is presented in Table IV in the Appendix .

REL

Nonvol a t i 3 R ~

Io6Ru * 9 , 9 0 s r

ASES TO SEPARATIONS AREAS SEEPAGE BASINS DURING 1969

F Area H Area Jan- J u l - Jan- J u l - 1969 Tota l Jun DPC Jun Dec F Area H Area

e beta, C i

9.07 10.91 6.37 2.70 7.16 3.75 6.84 7.18 18.04 21.09 14.02 39.13 0.60

9 5 Z r - 5Nb 3.97 137cs 7.68

1.30 147pm 1.36 Oco 0.01

Tota l 28.13

141 , 1 4 4 ~ ~

Alpha, m C i 311.1 Radioiodine, C i 0.51

0.58 8.18

14.83 0.89 1.39 0.01

35.76

1596.5 1.02

0.93 1.65 2.05 1.20 4.36 1.76 0.69 1.96 2.27 1.54 0.01 0.65

35.51 33.60

191.2 485.5 - 0.01

1.18 2.58 12.15 3.25 22.51 6.12

2.19 2.65 2.75 3.81 0.02 0.66

63.89 69.11

1907. 6a 676. 7b 1.53 0.01

T r i t i urn 7647 4032 6987 4028 11,679 11,015

a. 24% 239Pu and 25% 238Pu. b. 2% 239Pu and 94% 238Pu.

RELEASES TO FORD BUILDING SEEPAGE BASIN DURING 1969

Nonvolat i le Beta, mCi Tr i t ium, C i 0 0

- 10 -

RELEASES TO 700 AREA SEEPAGE BASINS

1969 Total Operating Release Guide A1 pha , .mCi Nonvolati le be t a , mCi 1396 3 Ci/yr, exclusive o f gost- 8 9 , 9 0 ~ r , mci 6 . 8 0.1 Ci/yr o f 'OSr T r i t i u m , C i 22 -

944 1 Ci/yr, exclusive o f 1 ci o f 2 3 B ~ \

RELEASES TO CMX-TNX SEEPAGE BASIN

1969 Total

Uranium (natural and dep le t ed ) , l b 709 Thorium ( n a t u r a l ) , l b 0

RELEASES TO REACTOR AREAS SEEPAGE BASINS

Radionuclides Shor t - l i ved , C i ( t+ < 30 days)

2 3 9 N p ' ' ~ r " OBa- 140La 1 3 1 1

Total

Long-1 i ved , Ci ( t + > 30 days)

Ce

' 'Zr-' 'Nb

1 4 1 , 1 4 4

1 0 3 Y f 0 6~~

5Zn 6 o c o

8 9 , 9 0 s r

OSr 5s

1 3 4 , 1 3 7 ~ ~

Total

T r i t i um, C i

Oil and

P L Ka C ( L Area) Basin ( K Area)b Total

Chemical 50-mi 11 ion-gal Waste P i t Containment

- ~ - -

- - - - - 1.02 1.02 - - - 0.42 0.001 295.43 295.85 - - - - 0.001 17.79 17.79 - - - - 14.41 14.41

- - - 0.42 0.002 328.65 329.07

- - _ _ _ - -

0.004

0.003

0.001

<O.OOl

<o. 001

0.008

-

-

-

-

- - - - -

0.065 0.030

0.880

0.98

-

0.007 0.001 0.005

0.049

0.001

0.002

0.065

-

-

-

7.80 1.29 1.33 0.56 0.67 2.67

49.22 3.61

75.65

7.81 1.29 1.34 0.56 0.72 2.74

49.25 3.61

76.53

139.19 140.24

- 108 - 399 572 23,415 24,494

,

I

j:

!

a. The re l eases reported in the 1968 Audit t o t he K-Area seepage basin were i n e r r o r and should be added t o the r e l eases t o the 50-mill ion-gallon containment basin i n K Area.

b. Approximately 43.8 x l o 6 ga l lons o f water.

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. Y - -

WASTE TO BURIAL GROUND t .

’ d u r i n g 1969 are p r e s e n t e d i n t h e fo l lowing t a b l e .

Estimates of s o l i d waste d e p o s i t e d i n Bur i a l Ground 643-G

RADIOACTIVE WASTE BURIALS

PlutoniurnYa C i Other Gamma, C i Tri ti urn , Source -- 2 3 9 ~ u 238Pu A1 phas ,a C i -- Fiss ion Induced C i

200 Areas 90.9 421.6 0.3b 3,741 17,753 375,706 700 Area 16.3 13 ,678.8c 9,085 25 Off-P1 a n t 106

100 Areas - - - 923 96,113 -

To ta l 107.2. 421.6 13,679.1 13,749 113,891 375,812

a. Bur ied in concrete.

b. Inc ludes 0.1 C i o f uranium and 0.2 C i o f 240Pu. e. Inc ludes 12,275.5 C i o f cur ium and 1403.3 C i of 210Po.

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1-

P

SEPARATIONS AREAS WASTE STORAGE TANKS

1 The s t a t u s of l i q u i d waste s t o r a g e i n underground t a n k s , as of December 20, 1969, is summarized i n t h e fo l lowing t a b l e . The d a t a , as well as c a l c u l a t i o n s of t h e q u a n t i t i e s of f i s s i o n p roduc t s i n t h e t a n k s , were r e p o r t e d by t h e Sepa ra t ions Technology S e c t i o n i n t h e December 1969 Works Technica l Department Monthly P rogres s Report (DPSP-69-1-12, p 87).

\ .

Tanks F Area

1 2 3 4 5 6 7 8

1 7 18 19 20

Total

H Area 9

10 11 12 13 14 15 16 21 22 23 24

Tota l Grand Total

238U, l b (mul t ip ly 2 3 5 ~ , 2 3 9 ~ u , by l o 3 ) kg kg

7.76 26.17 0.50 1 .68 1.26 4.14 7.13 23.49

16.40 56.86 7.50 24.79

54.09 189.50 23.07 78.99 6.60 22.93

19.98 71.40 0.0 0.0 0.0 0.0

144.3 499.9 --

2.36 0.14 0.32 6.35

10.41 3.05

40.22 14.93

7.45 22.53 0.0 0.0

107.8

0.21 0.70 <0.01 0.07 0.22 0.01 0.0 3.58 2.80 6.44 38.68 12.29

11.21 57.90 19.69 1 .30 4.76 0.89 0.0 13.87 15.19 0.0 0.37 10.56 0.26 8.00 0.09 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

19.50 128.1 61.53 _ _ _ - -

163.8 628.0 169.3

F i s s i o n a Products ,

M C i

19.92 6.70

10.56 48.30

162.20 38.27 35.22

120.50 0.48

19.82 0.36 1.51

463.9

6.40 8.88

11.41 54.49 50.13

5.09 132.60

19.32 13.62 20.43 0.0

12.26

334.6

798.5

a. Error in t h e 1968 Audit - unit f o r fission products is MCi not mCi.

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APPEND I X

TABLE I

SUMMARY OF RADIOACTIVE WASTE RELEASES BY INDIVIDUAL AREAS

N o n v o l a t i l e Beta, C i Rad io iod ine , C i T r i t i u m , kCi T o t a l Since Area o r T o t a l Since T o t a l S ince

To B l d g - 1969 P l a n t S t a r t u p 1969 P l a n t S t a r t u p 1969 P l a n t S t a r t u p 1969 P l a n t S t a r t u p

Atmosphere F 38.1 2908 H 649.4 1417 R P - L - K C -

TNX - 773-A 21.6

0.3 49.5 2.6 1103 14.7 80.5 33.3 1339

11 x 0.38 x 78 x i o - @

33 x 10-3'

0.46 x 10-3 30 x 10-3'

0.34 x 10-3 19 x 10-3' -

0.02 1.32

1900 272 8069

275 33 620

74 1 87 9 56 64 85 1

2 32 0.12 16.4

-

22.1 6.0 0.004

T o t a l 709.1 4347 15.0 131.4 35.9 2448 4 58 13,460

F H R P L K

C

Misc (Reac- t o r Area)

4000 300A 773A

T o t a l

2.6 3.5

10.8 0.9

14.7 9.9

8.1 3 3 . 3 ' 65.8" 92.4c 91 .35

148.0" 128.5"

E f f l u e n t streams

5 6 -

146 124

0.7 2.2

15.1 27.2

3209 2541 2477 2086 2564

55.3 92.9 34.4 30.8 16.2

4.12

0.40 0.50

107.42 5.60

20.57 94.74

1262 61

1334

1908 677

136.3 74.4

0.41

0.2

0.06

231.9

63.89 69.11

0.01

1.4 1.40

56.7

8.2

0.06

12984

1941 959

2700.5 229.9

65.5 26.1

237.6 5.9 0.016

272.9 1147.1

7585

0.02 0.4 11.2 10.5

21241 61

21 572

14176 3923

-

1650

23@

897.7 1701.3

778.1

156.2 125.7

5 . 3 9 .0

7 . 0

4 .7

18.1

0.06 0.5

32.2 46.9

5.0

1.53 0.01

64. I

1 1 . 7 11.0

Seepage bas ins

0.1

0 . 2 C

700A 944 Ford B ldg

Le

K--

0.4

0.02

14.41

15.95

1 . o 18.1

26 1 i!

0 . 6 23.4

-17.2

0.01 453.43

589.31 T o t a l 3529 19749 403

a. Since October 1960. b. Since J u l y 1958. c. Since January 1958.

d. Since J u l y 1960. e . Oil and chemical waste p i t . f. 5 0 - m i l l i o n - g a l l o n containment bas in .

T r i t i u m from K Area t o streams d u r i n g 1969 inc ludes a 12.7 k C i m i g r a t i o n est i ! ! idte f r o r t h e K-Area containment b a s i n .

(C9R.WCP;O - The t o t a l s s i n c e p l a n t s t a r t u p r e f l e c t these cori .ectiol?s.!

F Area Jatiudty I -ebrudry Md r c h A p r i I May June 6-1110 T o t a l J u l y Auyus t Se p t enibe r October I4oveitite r December 6-010 T o t a l

1969 T o t a l

tl Area January Februdry March A p r i 1

June E-nio T o t a l J u l y August Sep teniber October Flovembe r December

_ _

--

May

6- 110 T o t d l

1569 T o t d l

TABLE 11

1969 RELEASES TO ATMOSPHERE FROM SEPARATIONS AREAS STACKS

1.71 4.5 4 . 9 3.17 7.2 8.3 2.44 17.4 7.5 4.92 20.8 10.0 0.88 5.2 13.2 1.27 2.7 7.4

14.39 57.8 51.3 1.42 7.8 10.6

10.08 19.7 21.0 3.82 12.7 14.3 7.58 7.9 9.4 0.29 0.9 1 .7 0.52 0 .8 4.5

23.71 49.8 61.5

38.10 107.6 112.8

1.80 4.14

11.07 563.43

6.42 13.20

600.06 33.71

2.62 2.98 2.64

5.48 49.31

1 .a8

5.4 1 .8 2.9

9134.7 31.7 22.7

9199.2 34.3 21.7 22.3

148.1 66.0 16.2

308.6

13.8 10.7 6.2

1010.7 29.1 16.0

1086.5 43.6

114.6 607.9

1428.9 659.2

59.4 2913.6

649.37 9507.8 4000.1

0.7 0 .6 0.3 1.1 0.7 0.5 3.9 0.5 0.5 0.7 0.5 0.4 0.5 3 . 1

7.0

3.6 0.9 1.7

85.1 1.4 2.0

94.7 3.6 0 .4 0.6 0.7 1.7 6.7

13.7

108.4

7.3 5.2 2.5

11.4 . 3.9 1.8

32.1 10.1 5.4 8.2 2.3 1.1 1 .o

28.1

60.2

15.8 12.8 5.4

127.5 9.1 7.5

178.1 22.7

1.4 4.3 3.5 4.1

11.2 47.2

225.3

0.8 0.3 0.5 1.2 0.5 0.3 3.6 G.2 0 .8 0.7 0 .7 0 .5 2 .2 5.1

8.7

2.2 1 .o 0.9

26.9 2.1 1.7

34.8 1.1 0.5 0.9 2.3 2.5

34.5 41 . 8

76.6

2.3 2.1 1.1 3.5 4.6 1.8

15.4 1.4 2.5 3.2 2.0 2.0 2.9

14.0

29.4

42.7 13.1 68.7

476.1 10.4 22.1

633.1 33.6

2.6 18.3

32.6 43.1

148.6

781.7

18.4

Tota l

20.5 23.7 29.3 48.0 28.1 14.5

164.1 30.6 49.9

22.8 6.6

11.9 161.6

325.7

39.8

83.5

85.8 40.3

10861 .O 83.8 72.0

11226.4 138.9 141.2 654,3

1601.9 766.1 171.1

3473.5

14,699.9

. .

Radioiodine, T r i t i u m , kCi 232-H 234-H 238-H --- mC i

202 122

1036 85

5 6

1456 596

99 329

7 41

1161

261 7

89

87 1829

3386 1021 685

13636 3685 4705 81 27

2631 259

19696

33,332

6628

289

14.9 19.9 - 13.8 13.0 - 13.0 14.2 - 9.5 13.8 -

11.0 5.4 0.10 71.1 79.1 0.10 32.4 6.0 0.10 11.8 8.5 0.15 10.5 8.8 0.20 5.3 16.7 0.35

8.9 12.8 -

4 .4 5.2 0.20 5 .1 6.2 0.15

.69 .5 51.4 1.15

140.6 130.5 1.25

P Area January February March A p r i 1 May June 6-in0 T o t a l J u l y August September October November December 6-mo T o t a l 1969 T o t a l L Area January February March A p r i 1 M aY June 6-mo T o t a l J u l y August September October November December 6-mo T o t a l 1969 T o t a l

TABLE I 1 1

1969 RELEASES TO EFFLUENT STREAMS FROM DISASSEMBLY B A S I N S

0.62 0.25 0.71 0.11 0.40 0.17 2.26 0.38

0.25 0.22 0.20 0.19 1.24 3.50

0.09 0.07 0.08 0.03

0.27 0.27

0.63 0.87 0.95 0.25 0.18 0.68 3.56 1.46 0.54 0.72 1.21 0.64

4.59 8.15

U

0.14

0.14

a

0.14

0.03

0.07 0.04 0.14 0.07

0.07 0.12

0.26 0.40

-- 0.57 0.26 0.68 0.20 0.66 0.53 2.90 0.82 0.18 0.27 0.57 0.64 0.53 3.01 5.91

0.02

0.05 0.06 0.07 0.02 0.22 0.08 0.12 0.18 0.19 0.09 0.05 0.71 0.93

-

0.31 0.11 0.43 0.05 0.17 0.21 1.28 0.21 0.07 0.23 0.59 0.48 0.31 1.89 3.17

0.06 0.03 1.09 0.04 - 0.92 0.14 - 3.73

- 2.41 0.07 - 2.22 0.05 - 1.07 0.36 0.03 11.44 0.18 0.04 1.93 0.20 0.04 0.84 0.23 0.07 3.61 0.04 0.02 4.05 - ' 0.45 - 1.11 0.65 0.17 11.99 1.01 0.20 23.43

0.83 0.50 0.59 0.57 1.71 1.91 6.11 2.06 0.78 0.81 1.33 0.76 1.22 6.96 13.07

0.33 0.49 0.36 0.79 0.67 0.80 3.44 3.44

. .. -- 0.65 4.79 0.25 3.20 0.38 7.64

0.56 6.04 0.83 5.49 3.11 31.19 0.85 8.00 0.44 3.11 0.74 7.00 0.88 9.03 0.63 3.80 1.38 4.74 4.92 35.68 8.03b 66.87

0.44 4.03

0.12 0.28 0.03 0.03 0.02 0.07 0.04 0.10 0.04 0.11 0.03 0.05 0.28 0.64 0.08 0.58 0.25 0.93 0.05 0.67 0.11 1.12 0.01 0.77

0.54 4.96 0.82c 5.60

0.04 0.89

0.07 0.08 0.02

2.45 0.24 1.10 0.20 4.98 0.85

- 3.13 0.77 0.05 4.45 0.18 - 1.52 0.04

0.22 17.63 2.28 0.01 0.95 0.01 - 1.15 -

0.61 10.74 1.41 - 4.61 0.21 - 1.95 0.08 - 1.42 0.13

0.62 20.82 1.84 0.84 38.45 4.12

0.02

0.05 0.18 d.03 0.16 0.44

0.53 0,08

0.61 1.05

-

"P T o t a l

0.01 2.79 0.01 1.39 0.03 5.93 0.03 4.11 0.01 4.72 0.02 1.74 0.11 20.68 - 0.97

1.15 0.01 13.30 0.04 4.94 0.02 2.05 0.03 1.58 0.10 23.99 0.21 44.67

-- Tri t iun t ,

C i

701 472

1034 1297 1352

782 5638

855 404

1041 1906

206 7 5 3

5165 10803

16 1 5 i 1 38 74

129 283 159 111 46 81 62

149

608 89 1

1

TABLE 111 (Cont inued)

1969 RELEASES TO EFFLUENT STREAMS FROM DISASSEMBLY B A S I N S

K Area January February March

Apr i 1 May June 6-mo T o t a l

J u l y August September October November December

6-mo Tota l

1969 Tota l

C Area January February March A p r i 1 1 ay June 6 4 0 T o t a l J u l y August September October November December 6-mo T o t a l

1969 T o t a l

0.02

0.02

0.02

0.44 0.05 0.18 0.21 0.04 0.04 0.96 0.32 0.16 0.04

0.18 0.70

1.66

'Pm - 0.18 0.85 0.08 0.04 0.05 0.18 1.38

0.31 0.07 0.26 0.11 0.03 a

0.78

2.16

0.44 0.32 3.26 0.27 0.10 0.11 1.50 1.23 0.17 0.52 0.58 0.11 a

2.61

4.11

0.01

0.01 0.09

0.09

0.10

0.03 0.18 0.11 0.03 0.14 0.04 0.53

0.24 0.08 0.15 0.12 0.17 0.09

0.85

1 .38

0.14 0.10 0.06 0.19 0.12 0.04 0.65 0.27 0.16 0.10 0.09 0.08 0.12 0.82

1.47

0.01 0.01

0 . 0 7

0.09 0.09 0.05 0.12 0.04 0.02

0.32

0.41

0.01 - 0.06 - 0.17 - 0.09 - 0.33 - 0.08 -

0.12 - 0.20 - 0.53 -

u . No a n a l y s i s b . Inc ludes 1.52 C i o f 9 0 S r w i t h a maximum monthly r e l e a s e o f 0.22 C i . c'. Inc ludes 0.59 C i o f ' " S r w i t h a maximum monthly r e l e a s e o f 0.10 C i . 1. Inc ludes 0.42 C i o f " S r w i t h a maximum monthly r e l e a s e o f 0.15 C i . .<. Inc ludes 0.80 C i o f "Sr w i t h a maximum'monthly r e l e a s e o f 0.11 C i .

1.12 2.48 0.07 0.03 0.04 0.10 3.84

0.17 0.09 0.13 0.12 0.08 0.29

0.88

4.72

2.83 0.46 2.28 3.67 0.37 0.14 9.75 5.09 0.23 3.26 5.03 4.60 8.24

26.45

36.20

0.16 0.09 0.05 0.06

0.20 0.56 0.48 0.57 0.53 0.46 0.37 0.57 2.98

3.54

0.11 1.44 - 2.95 - 0.48 4.01 - 7.09 0.40 0.14 0.40 - 0.06 0.16 - 0.10 0.33 - 0.04 0.36 - 0.93 6.70 - 10.04 0.40

0.08 0.80 - 0.22 - 0.02 . 0.26 - 0.06 0.60 - 0.15 0.50 - 0.13 0.41 - 0.36 0.74 - 0.80 3.31 - 0.22 - 1.73d 10.01 . - 10.26 0.40

0.13 4.16 7.18 6.10 0.06 0.19 1.23 0.82 0.56 0.17 0.08 2.97 3.46 1.61 0.11 0.16 4.80 - 1.72 0.04 0.07 0.70 - 0.07 0.69 - 0.70 14.55 11.46 9.99 0.38 0.23 7.88 2.29 2.94 0.06

0.11 4.68 0.36 0.66 0.04 0.11 1.45 - 0.56 - 0.07 6.27 - 0.42 - 0.07 5.25 10.03 1.78 - 0.28 9.51 0.72 3.47 0.02 0.87 35.04 13.40 9.83 0.12

1.57e 49.59 24.86 19.82 0.50

0.09

0.09 0.14

0.02 0.16

0.25

0.02 2.97 413 0.02 7.51 ' 1308

0.06 0.06 0.04 0.04 0.04 0.04 0.18 10.62

0.03 0.25

0.01 0.01

0.05 0.05 0.03 0.03

0.12 0.34

0.30 10.96

0.03 1 3 . 3 7 0.01 1.65

0.04 1.80

0.01 0.01 0.09 22.01 0.02 5.45 0.02 0.58 - 1 - 0 6 - 0.42

- 5.18

0.01 11.82 0.08 4.3'1 0.13 23.64

0.22 45.65

9

1 1 21 18

1780

27 27 3 2 55 24 26

101

1 9 7 1

1622 100 7 4 2 893

44 52

3453 2007

53 662 634 44 3

2652 6451

9904

\

t

TABLE I V

1969 RELEASES TO SEPARATIONS AREAS SEEPAGE BASINS

LAIS%! :.lOn t h 1 y Operating Release Guide January February March Apri 1 May June 6-1110 Total J u l y August September October November December 6 4 0 Total

1989 Total

ti Area Monthly Operat ing Release Guide January February March Apri 1 May June 6-mo Total J u l y August September October November @e c em be r 6-010 Total

1969 Total

1. 36,000 C i l y r . o. No a n a l y s i s .

500 1 .0

45.5 - 43.5 - 72.2 - 50.6 - 75.1 - 24.2 0.01

311.1 0.01

71.5 - 67.6 0.01

1265.3 - 47.5 - 92.7 -

1596.5 0.01

1907.6 0.02

51.9 -

500 1.0

13 .0 0.01 18.4 - 38.9 - 62.0 - 17.9 - 41.0 -

191.2 0.01 52.3 - 63 .0 0.12

143.1 0.05 79.1 0 .48 65.9 - 82.1 -

485.5 0.65

676.7 0.66

0.9 2.5 2 .0

0.07 0.06 1.23 0.37 0.11 0.10 1.39 0.29 0.24 0.23 2.14 0.36 0.09 0.07 1.05 0.17 0.05 0.03 0.46 0.09 0.04 0.03 1.41 0.08 0.60 0.52 7.68 1.36 0.08 0.07 2.70 0.24 0.06 0.06 3.87 0.46 0.08 0.08 2.60 0.17 0.21 0.16 3.25 0.36 0.05 0.03 1.36 0 . J6 0.10 0.07 1.05 h

0.58 0.47 14.83 1.39

1.18 0.99 22.51 2.75

0.7 1 . 5 2.0

0.16 0.12 0 .72 C.19 0.22 0.14 1.44 0.71 0.09 0.09 0.55 0.64 C.25 0.23 0.67 0.64 0.13 0.10 0.58 0 .02 0.08 0.05 0.40 0.07 0.93 0.73 4.36 2.27 0.10 0.08 0.25 0.38 0.06 0.06 0.45 0.53 0.06 0.06 0.37 0.22 0.11 0.11 0.39 0.23 1.04 0.99 0.20 0.18 0.28 0.26 0.10 h 1.65 1.56 1.76 1.54

2.5s 2.29 6.12 3.81

0.23 0.16 0.67 0.15 0.04 0.05 1.30 0.19

0.14 0.33 0.11 0.12 0.89

2.19

0.17 0.05 0.44 0.03

0.69

0.18 0.31 0.60 0.71 0.16 1.96

2.65

2.71 2.13 0.95 0.71 0.45 0.55 0.86 0.85 0.97 1.90 0.43 0.70 6.37 6.84 0.10 0.76 1.14 2.57 0.30 0.42 0.95 0.63 0.21 F.53

2.70 7.18

9.07 14.02

- 1.27

0.96 2.91 0.69 3.94 0.41 1.90 0.99 2.57 2.13 3.91 1.98 2.81 7.16 18.04 2.07 7.65 3.82 5.91 0.49 2.66 0.30 3.04 0.07 0.94 - 0.89

3.75 21.09

10.91 39.13

3SZr-gSNb Total Ci ~~-

1.26 0.45 0.43 0.71 0.77 0.35 3.97 0.40 1.99 0.80 1.12 1.43 2.44 8.18

12.15

0.18 0.52 0.27 0.55 0.40 0.13 2.05 0.16 0.18 0.29 0.26 0.17 0.14 1.20

3 .25

8.00 0.06 4.06 0.10 4.84 0.33 3.88 0.02 4.28 - 3.07 -

28.13 0.51 4.47 0.58

10.09 0.07 4.52 0.37 6.85 - 4.85 - 4.98 -

35.76 1.02

63.89 1.53

5.13 - 7.69 - 3.91 - 6.11 - 7.20 - 5.47 -

35.51 - 10.61 - 8.25 - 4.45 - 5.41 - 3.31 3.01 1.57 -

33.60 1.01

60.1i 3.01

Tr i t i um, C i

600W

2051 1053 1238 1321 1477 507

7647 456

1349 84 6 665 294 422

4032

11679

6O0Oa

2721 537 28 1

2479 560 409

6987 930 569 638 589 510 792

402c

I1015

!