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Lattice modulation experiments with fermions in optical lattices and more Nonequilibrium dynamics of Hubbard model Ehud Altman Weizmann Institute David Pekker Harvard University Rajdeep Sensarma Harvard University Eugene Demler Harvard University

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Page 1: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Lattice modulation experiments

with fermions in optical lattices

and more

Nonequilibrium dynamics of Hubbard model

Ehud Altman Weizmann InstituteDavid Pekker Harvard University

Rajdeep Sensarma Harvard University

Eugene Demler Harvard University

Page 2: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Antiferromagnetic and superconducting Tc of the order of 100 K

Atoms in optical lattice

Antiferromagnetism and pairing at sub-micro Kelvin temperatures

Fermionic Hubbard modelFrom high temperature superconductors to ultracold atoms

Page 3: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Fermions in optical lattice

t

U

t

Hubbard model plus parabolic potential

Probing many-body states

Electrons in solids Fermions in optical lattice

• Thermodynamic probesi.e. specific heat

• System size, number of doublons

as a function of entropy, U/t, ω0

• X-Ray and neutron scattering

• Bragg spectroscopy,TOF noise correlations

• ARPES ???

• Optical conductivity• STM

• Lattice modulation experiments

Page 4: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Outline

• Introduction. Recent experiments with fermions

in optical lattice. Signatures of Mott state

• Lattice modulation experiments in the Mott state.

Linear response theory

• Comparison to experiments

• Lifetime of repulsively bound pairs

• Lattice modulation experiments with d-wave

superfluids

Page 5: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Mott state of fermions

in optical lattice

Page 6: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Signatures of incompressible Mott state

Suppression in the number of double occupanciesEsslinger et al. arXiv:0804.4009

Page 7: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Signatures of incompressible Mott state

Response to external potentialI. Bloch, A. Rosch, et al., arXiv:0809.1464

Radius of the cloud as a functionof the confining potential

Next step: observation of antiferromagnetic order

Comparison with DMFT+LDA models suggests that temperature is above the Neel transition

However superexchange interactions have already been observed

Page 8: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Radius of the cloud: high temperature expansion

Starting point: zero tunneling.Expand in t/T.

Interaction can be arbitrary

Minimal cloud size for attractive interactionsObserved experimentally

by the Mainz group

Theory: first two terms in t/T expansion

Competition of interaction energy and entropy

Page 9: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Lattice modulation experiments

with fermions in optical lattice.

Mott state

Related theory work: Kollath et al., PRA 74:416049R) (2006)Huber, Ruegg, arXiv:0808:2350

Page 10: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Lattice modulation experimentsProbing dynamics of the Hubbard model

Measure number of doubly occupied sites

Main effect of shaking: modulation of tunneling

Modulate lattice potential

Doubly occupied sites created when frequency ω matches Hubbard U

Page 11: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Lattice modulation experimentsProbing dynamics of the Hubbard model

R. Joerdens et al., arXiv:0804.4009

Page 12: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Mott state

Regime of strong interactions U>>t.

Mott gap for the charge forms at

Antiferromagnetic ordering at

“High” temperature regime

“Low” temperature regime

All spin configurations are equally likely.Can neglect spin dynamics.

Spins are antiferromagnetically ordered or have strong correlations

Page 13: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Schwinger bosons and Slave Fermions

Bosons Fermions

Constraint :

Singlet Creation

Boson Hopping

Page 14: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Schwinger bosons and slave fermions

Fermion hopping

Doublon production due to lattice modulation perturbation

Second order perturbation theory. Number of doublons

Propagation of holes and doublons is coupled to spin excitations.Neglect spontaneous doublon production and relaxation.

Page 15: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

“Low” Temperature

d

h Assume independent propagation of hole and doublon (neglect vertex corrections)

= +

Self-consistent Born approximation Schmitt-Rink et al (1988), Kane et al. (1989)

Spectral function for hole or doublon

Sharp coherent part:dispersion set by J, weight by J/t

Incoherent part:dispersion

Propagation of holes and doublons strongly affected by interaction with spin waves

Page 16: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Propogation of doublons and holes

Spectral function:Oscillations reflect shake-off processes of spin waves

Hopping creates string of altered spins: bound states

Comparison of Born approximation and exact diagonalization: Dagotto et al.

Page 17: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

“Low” Temperature

Rate of doublon production

• Low energy peak due to sharp quasiparticles

• Broad continuum due to incoherent part

Page 18: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

“High” Temperature

Atomic limit. Neglect spin dynamics.All spin configurations are equally likely.

Aij (t’) replaced by probability of having a singlet

Assume independent propagation of doublons and holes.Rate of doublon production

Ad(h) is the spectral function of a single doublon (holon)

Page 19: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Propogation of doublons and holesHopping creates string of altered spins

Retraceable Path Approximation Brinkmann & Rice, 1970

Consider the paths with no closed loops

Spectral Fn. of single hole Doublon Production Rate Experiments

Page 20: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Ad(h) is the spectral function of a single doublon (holon)

Sum Rule :

Experiments:Possible origin of sum rule violation

The total weight does not scale

quadratically with t

• Nonlinearity

• Doublon decay

Lattice modulation experiments. Sum rule

Page 21: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Lattice modulation experimentsProbing dynamics of the Hubbard model

R. Joerdens et al., arXiv:0804.4009

Page 22: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Doublon decay rateinspired by experiments in ETH

Page 23: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Energy Released ~ U

�Energy carried by

spin excitations

~ J =4t2/U

� Relaxation requires

creation of ~U2/t2

spin excitations

Relaxation of doublon hole pairs in the Mott state

Relaxation rate

Large U/t : Very slow Relaxation

Page 24: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Alternative mechanism of relaxation

LHB

UHB

µ

• Thermal escape to edges

• Relaxation in compressible edges

Thermal escape time

Relaxation in compressible edges

Page 25: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Doublon decay in a compressible state

How to get rid of the excess energy U?

Compressible state: Fermi liquid description

Doublon can decay into apair of quasiparticles with

many particle-hole pairs

U

p-p

p-h

p-h

p-h

Page 26: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Doublon decay in a compressible state

Decay amplitude

Page 27: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Doublon decay in a compressible state

Fermi liquid description

Single particle states

Doublons

Interaction

Decay

Scattering

Page 28: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Doublon decay in a compressible state

Decay rate contained

in self-energy

Self-consistent equations for doublon

Page 29: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Doublon decay in a compressible state

Page 30: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Lattice modulation experiments

with fermions in optical lattice.

Detecting d-wave superfluid state

Page 31: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

• consider a mean-field description of the superfluid

• s-wave:

• d-wave:

• anisotropic s-wave:

Setting: BCS superfluid

Can we learn about paired states from lattice modulation

experiments? Can we distinguish pairing symmetries?

Page 32: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Modulating hopping via modulation

of the optical lattice intensity

Lattice modulation experiments

where

-3 -2 -1 0 1 2 3

-3

-2

-1

0

1

2

3

• Equal energy

contours

Resonantly exciting quasiparticles with

Enhancement close to the bananatips due to coherence factors

Page 33: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Distribution of quasi-particles

after lattice modulation

experiments (1/4 of zone)

Momentum distribution of

fermions after lattice modulation

(1/4 of zone)

Can be observed in TOF experiments

Lattice modulation as a probe of d-wave superfluids

Page 34: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

number of quasi-particles density-density correlations

• Peaks at wave-vectors connecting tips of bananas

• Similar to point contact spectroscopy

• Sign of peak and order-parameter (red=up, blue=down)

Lattice modulation as a probe of d-wave superfluids

Page 35: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Scanning tunneling spectroscopy of high Tc cuprates

Page 36: Condensed Matter Theory at Harvard University - Lattice ...cmt.harvard.edu/demler/2008_talks/2008_eth.pdfwith fermions in optical lattice. Mott state Related theory work: Kollath et

Conclusions

Experiments with fermions in optical lattice open

many interesting questions about dynamics of the

Hubbard model

Thanks to:

Harvard-MIT