crossover from bose-einstein condensed molecules to...
TRANSCRIPT
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Crossover from Bose-Einstein Condensed Molecules to
Cooper Pairs by Using Feshbach Resonance
Shu-Wei Chang
Department of Electrical and Computer Engineering,
University of Illinois at Urbana-Champaign, Urbana, IL 61801, USA
(Dated: May 6, 2004)
Abstract
At low temperature, fermionic atoms can either condense into a Bose-Einstein condensate (BEC)
by forming bosonic molecules or be loosely paired to form Cooper pairs described by Bardeen,
Cooper, and Schrieffer’s (BCS) microscopic theory. Experimentalists have claimed the observation
of the intermediate regime between BEC and BCS limits by tuning the scattering length with the
aid of Feshbach resonance. In this report, we will discuss the idea of using Feshbach resonance
to achieve the crossover. Some many-body formulation concerning this crossover will be briefly
introduced, but not in detail. The experimental results will be our main concerns and addressed
in this report.
1
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I. INTRODUCTION
After the successful demonstrations of Bose-Einstein condensation (BEC) of atomic
gas,[1, 2], the cooling down of atomic Fermi gas has also been achieved recently.[3, 4] Unlike
bosonic atoms, fermionic atoms cannot condense into a single state due to anti symmetriza-
tion of the macroscopic wave function. However, two fermionic atoms can be converted into
a bosonic molecule and condense into a BEC again.
Whether two fermionic atoms can form a bosonic molecule is closely related to the two-
body physics of the atoms. The sign of the s-wave scattering length between two identical
fermionic atoms in different internal quantum states, called an open channel, determines
whether the effective interaction in that channel between two fermions is repulsive or attrac-
tive at low temperature.[5] The sign of the s-wave scattering length has a close connection
with the near-by energy of the bound state in a closed channel of which threshold energy is
higher than that of the open channel. For fermionic atoms with the same internal quantum
states, the s-wave scattering cross section disappears due to anti-symmetrization of wave
functions, and one has to consider scattering lengths due to, for example, p-wave scatter-
ing. Experimentally, it will be more efficient to observe the change of the s-wave scattering
length in an open channel characterized by the scattering of the atoms with different internal
quantum numbers.[6, 7] However, if the physical environment favors the atoms of a single
internal quantum state, issues on p-wave scattering such as the analogy of p-wave pairing
in superconductivity then can be discussed.[8]
For atoms, the s-wave scattering length can be controlled by mechanisms such as the
interaction of magnetic moments with magnetic field[9] or Raman transition induced by
lasers.[10, 11] In either case, the energy of the bound state in the closed channel is swept
across the threshold energy of the open channel. It is possible to change the sign of the
scattering length and thus the property of the effective interaction. For fermionic atoms,
the controllability of the scattering length enables the formation of a correlated atom pair in
one limit and a tightly-bound molecule in the other, as will be discussed in the next section.
Experimentally, it is interesting to ask what happens to the pair of fermionic atoms at the
crossover between the two limits. Theoretically, it can also provide an analogue test for one
of the candidate theories of high temperature superconductivity, originated from Nozières
and Schmitt-Rink by considering electron pairs resonant with the molecular state.[12]
2
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Eb
E
Eth
Close Channel
Open Channel
Atomic Separation
FIG. 1: Feshbach resonance of a quasi-bound state with the open channel. Eb is the resonant
energy of the quasi-bound state. Eth is the threshold energy of the open channel. The blue part
indicates the continuum of the open channel.
II. FESHBACH RESONANCE
Feshbach is first discussed in nuclear physics.[13] In this section, emphasis will be put on
the Feshbach resonance using magnetic field. More details can be found in Ref. [5].
For fermionic atoms, Feshbach resonance is the change of the scattering length in an open
channel due to the coupling to a bound state in the closed channel. The state in the closed
channel will be a true bound state if either there is no coupling to the open channel, or the
energy of the state lies below the threshold energy of the open channel. On the other hand,
if the state has an energy lying in the continuum of the open channel and exhibits a finite
coupling to the open channel, it should be called a quasi-bound state since it is not a true
bound state. A quasi-bound state exhibits some sort of energy resonance just as a bound
state but is characterized by a finite decay width due to the coupling to the open channel.
Fig. 1 shows the Feshbach resonance of a quasi-bound state coupling to the open channel.
Write the general wave function |Ψ > as a superposition of the part in the open chan-
nel |Ψ1 > and the part in the closed channel |Ψ2 >. The two parts are orthogonal to each
other: < Ψ2|Ψ1 >= 0. The Hamiltonian describing both open and closed channels is de-
noted as H. Also, write the projection operator to the open and closed channels as P1 and
P2. We define various projected Hamiltonians as
Hij = PiHPj, i, j = 1, 2 (1)
3
-
After a close look, the effective Hamiltonian Heff describing the open channel is written as
Heff |Ψ1 >=[
H11 + H12(E − H22 + iδ)−1H21
]
|Ψ1 >= E|Ψ1 > (2)
where δ is a small number. We further write the projected Hamiltonian H11 as H11 = H0+U
where H0 is the noninteracting part of the Hamiltonian H11. The interaction term Ueff in
the effective Hamiltonian Heff is
Ueff = U + H12(E − H22 + iδ)−1H21 (3)
The effective s-wave scattering length is evaluated from equation (3) by Born’s approxima-
tion for the zero momentum state |ϕ0 > of the open channel. The energy of the state |ϕ0 >
is just the threshold energy Eth of the open channel. Denote a complete set of the eigenstates
of the projected Hamiltonian H22 as {|φn >, n = 1, 2, ...} with eigenenergies {En}. Due to
the fact that H12 = H†21 and the completeness relation 1 =
∑
n |φn >< φn| in the closed
channel, the s-wave scattering length as of this open channel can be written as
as =mr
4π~2< ϕ0|Ueff |ϕ0 >
=
as,1︷ ︸︸ ︷mr
4π~2< ϕ0|U |ϕ0 > +
mr4π~2
∑
n
| < φn|H21|ϕ0 > |2
Eth − En + iδ
=
[
as,1 +mr
4π~2
∑
n,En 6=Eb
| < φn|H21|ϕ0 > |2
Eth − En + iδ
]
︸ ︷︷ ︸
anr
+mr
4π~2| < φb|H21|ϕ0 > |
2
Eth − Eb + iδ(4)
where as,1 denotes the s-wave scattering length in the open channel; |φb > is the (quasi-)
bound state with energy Eb nearest to the threshold energy Eth; and ans is the nonresonant
part of the s-wave scattering length. The contribution from the state |φb > is separated from
the summation since it is the most significant. The denominator Eth −Eb in equation (4) is
a function of the applied magnetic field B. Denote the internal quantum numbers labeling
the two atoms in the open channel as α and β where α 6= β. Near a particular magnetic
field B0, the denominator can be expanded as
Eth − Eb ≈ (µb − µα − µβ)(B − B0) (5)
where µb, µα, and µβ are the magnetic moments of the (quasi-) bound state and the states la-
beled by internal quantum numbers α and β. If the nonresonant s-wave scattering length anr
does not vary too much with the magnetic field, equation (4) can be written as
4
-
B
as
anr
B0
FIG. 2: S-wave scattering length as a function of magnetic field.
as = anr(1 +∆B
B − B0 + iδB)
∆B =mr
4π~2anr
| < φb|H21|ϕ0 > |2
µb − µα − µβ(6)
where δB is an infinitesimal quantity. A typical s-wave scattering length as a function of
the magnetic field is shown in Fig. 2 for anr > 0 and ∆ − B > 0. The scattering length
diverges to plus and minus infinities as the magnetic field tends to B−0 and B+0 . Examples
include the s-wave scattering length for |F = 9/2,mF = −9/2 > +|F = 9/2,mF = −7/2 >
of 40K[6, 14, 15] and so on. Also, this scattering is an elastic one since the kinetic energy is
not lost during the scattering.
If the threshold energy Eth is slightly larger than Eb, the s-wave scattering length is
positive. Although the effective interaction potential corresponding to this positive elastic
scattering length is repulsive, two fermionic atoms can form a molecule when the magnetic
field is swept downward across the magnetic field B0. In this case, it is possible to form
BEC from these bosonic molecules. The energy difference between the two atoms and
molecule is brought away by three-body processes instead of the s-wave two-body inelastic
scattering which is believed to be absent.[8, 16–19] However, the molecules produced in this
way are usually highly vibrationally excited. The deexcitation of these molecules will cause
significant inelastic scattering, and the loss rate of these molecules is high.[6, 7, 20] On the
other hand, for the negative scattering length (attractive interaction), atoms in the open
channel cannot form a stable molecule described by a true bound state. They can interact
via the quasi-bound state and form a correlated pair, or may be viewed as molecules with
finite lifetime. This regime should be described by a generalized Bardeen, Cooper, and
Schrieffer’s (BCS) theory instead of BEC. Typically, the atoms in this regime have lower
loss rate than the molecules in the other side of the resonance. [6, 7, 20]
5
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III. ON THE MANY-BODY ASPECTS
In atomic gases, the presence of quasi-bound state is easily modeled by adding a coupling
term to a molecular state in the BCS Hamiltonian for fermionic atoms.[21–23]
H =∑
k
²k(a†k,↑ak,↑ + a
†k,↓ak,↓) + Ubg
∑
k1+...+k4=0
a†k1,↑a†k2,↓
ak3,↓ak4,↑
+g∑
k,q
(b†qaq/2+k,↑aq/2−k,↓ + bqa†
q/2−k,↓a†
q/2+k,↑) +∑
q
(ν + Eq)b†qbq (7)
where a (b) and a† (b†) are the annihilation and creation operators of atoms (molecules); ²k
and Eq are the the kinetic energies of atoms and molecules; ↑ and ↓ are pseudo spins indi-
cating the two different internal quantum states; Ubg is the background attractive potential
between atoms; µ is the bound-state energy relative to the threshold of the open channel
due to the magnetic field; and g describes the exchange between atoms and molecules. This
Hamiltonian describes the superfluidity of Fermi atoms in the BEC limit, BCS limit, and
the intermediate regime. The change of the scattering length is not obvious in equation (7)
but is implicitly included due to the coupling constant g. This model is a more rigorous
picture than the two-body one in the previous section because the corresponding effective
theory fails if the scattering length is large near the resonance.
Instead of going through the mathematical details, we only mention a few results of key
calculations. The detailed treatments of this Hamiltonian or its mutants for atomic Fermi
gas can be found in literatures.[21–25]
Fig. 3 shows the critical temperature, the chemical potential, and the fractions of atoms
and molecules at the emergence of superfluidity as a function of the bound-state energy.[23]
This result is obtained numerically by self-consistently solving the gap equation and the
conservation of particle number.
1 = (−Ubg +g2
ν − 2µ)∑
k
tanh[β(k2/2m − µ)/2]
2(k2/2m − µ)
N = 2∑
k
1
eβ(k2/2m−µ) + 1+ 2
∑
k
1
eβ(k2/4m+ν−µ) + 1−
1
β
∑
q
∂
∂µln[1 − χ(q, iω)] (8)
where µ is the chemical potential; N is the total particle number; and χ(q, iω) is a correction
function describing the number fluctuations of atoms and molecules. In Fig. 3(a), the
solid line shows the critical temperature calculated from equation (8). The dash line is
a calculation by substituting equation (6) into Ubg and solving the BCS gap equation. The
6
-
(a) (b) (c)
FIG. 3: Physical quantities at the emergence of superfluidity as a function of the bound-state
energy. (a) Critical temperature. Solid line is the result from equation (8). Dash-line is the result
from the reduced BCS theory. (b) Chemical Potential. (c) Fractions of atoms and molecules. Solid
line is the fraction of the fermions while the dot-dash line is the pair fraction. After Ref. [23]
critical temperature calculated from simple BCS gap equation diverges at the resonance
because the interaction energy Ubg calculated in this way diverges to minus infinity. The
solid line matches well with the simple BCS theory when the bound-state energy is above
the threshold. On the other hand, it approaches the critical temperature predicted by BEC
theory at the other limit. As the bound-state energy is tuned downward from the BCS side
toward the resonance, the critical temperature increases, which makes this model a candidate
for high-temperature superconductivity. There is an optimized critical temperature close
to the threshold energy. This critical temperature is around 0.26 TF , where TF is the
Fermi temperature of the atoms without any molecules. Similarly in Fig. 3(b), the chemical
potential is also a smooth connection between the two limits. In the BCS limit, the chemical
potential approaches that of the Fermi gas at critical temperature. In the BEC limit, the
chemical potential will tend to one half of the bound-state energy. This is an analogy to
that the chemical potential of pure bosons approach their ground energy as BEC occurs.
Fig. 3(c) shows the fractions of fermionic atoms and atom pairs. The fraction of fermions
approach zero as the system goes deep into BEC limit while the pair fraction shows the
opposite trend. The atom pairs resemble Cooper pairs above the resonance but are like
molecules below the resonance.
The calculation stated above is only related to the physical quantities when the super-
fluidity phase occurs. The question on whether there is a transition between BEC and
7
-
0
0.05
0.1
0.15
0.2
0.25
0.3
0.35
0.4
0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9
T/T
F
B-B0 (Gauss)
BEC BCS
TF=0.35 µK
(a)
0.1
0.15
0.2
00.2
0.40.6
0
0.03
0.06
T/TFB−B
0 (Gauss)
nm
c/n
m
(b)
FIG. 4: (a) The phase diagram of BCS-BEC transition. The upper dash line is the critical temper-
ature calculated from simple BCS theory. The lower dash line is the BCS-BEC boundary. (b) The
fraction of BEC condensate as a function of the magnetic field and temperature. After Ref. [26]
BCS limits, i.e., a boundary between BEC and BCS regimes in the phase diagram shown in
Fig. 4(a), is also interesting.[26] At zero temperature, write the pair wave function as the
superposition of the open and closed-channel wave functions χm(x, x′) and χaa(x, x
′),
√
Z(B)χm(x, x′)|closed > +
√
1 − Z(B)χaa(x, x′)|open > (9)
the question of BCS-BEC crossover becomes whether we can find a critical magnetic field
Bc(T = 0) such that the parameter Z(B < Bc(T = 0)) = 1 and Z(B > Bc(T = 0)) = 0. At
finite temperatures less than the critical temperature, the question becomes whether there is
a critical magnetic field Bc(T ) below which molecules begin to condense into the molecular
ground state, i.e., nm,BEC(B < Bc(T ), T )/nm(B < Bc(T ), T ) > 0. We first note that the
critical temperature calculated in Ref. [23] has a different shape from that calculated in
Ref. [26]. It may be a result of different approximations used in the calculations. Fig. 4(b)
shows the BEC fraction as a fraction of the magnetic field and temperature. At a given
temperature, there is a critical magnetic field Bc(T ) where the BEC condensate emerges.
These critical magnetic fields Bc(T ) deviate from B0 predicted by simple two-body physics.
A simple argument about these deviations is that molecules, though with a finite lifetime in
the BCS regime, will emerge from atomic Fermi sea when the shifted ground state energy
of molecules due to the coupling is roughly twice the chemical potential of the system.
This early formation of the molecular condensate before the exact resonance makes the
superfluidity at this crossover unusual.
8
-
(a)
3
2
1
0
N -
2 [10
-9]
6004002000Time [ms]
60
40
20
0
N -
1 [10
-6]
a)
b)
(b)
FIG. 5: (a) The scattering length of 40K. (b) The inelastic scattering rate of 6Li. The upper and
lower figure are the inverse and inverse square of the population as a function of time, indicating
the two-body and three-body processes. After Ref. [9, 14].
IV. EXPERIMENTS ON BCS-BEC CROSSOVER
Most of the experiments on BCS-BEC crossing are aimed at fermionic atoms 6Li and
40K.[2, 4, 6, 7, 9, 14, 15, 17–19] For 6Li, two hyperfine states |1/2, 1/2 > and |1/2,−1/2 >
are used while for 40K, two states |9/2,−7/2 > and |9/2,−9/2 > are used.
Fig. 5(a) shows the elastic scattering length of 40K as a function of magnetic field.[14]
The Feshbach resonance of 40K takes place at 224.18 G. The magnitude of the scattering
length is obtained from the extraction of rethermalization time by heating the atomic gas
when modulating the power of the optical trap.[9] The sign of the scattering length is
obtained by measuring the mean-filed shift of the transition |9/2,−9/2 >−→ |9/2,−5/2 >
.[15] The change of the scattering length is very significant as the magnetic field sweeps
across the resonance frequency, indicating the ability to control the effective interaction
between 40K atoms. Fig. 5(b) shows the inelastic loss rate of 6Li at 680 G.[17] There are two
Feshbach resonance peaks for 6Li–550 G and 822 G. The resonance at 822 G has a very broad
lineshape, and thus the inelastic scattering at 680 G is believed to be greatly influenced by
this resonance. The upper plot of Fig. 5(b) shows the inverse of the number of particles
remaining in the trap as a function of time. The nearly linear behavior seems to imply
that the two-body inelastic process dominates in the time scale observed. The lower plot
shows the inverse square of the population as a function of time. The three-body process will
dominate over the two-body process only when the population is high. The small linear part
at time close to zero thus indicates the three-body process. However, the inelastic two-body
9
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201 202 2030
20
40
60
80
100re
main
ing
ato
ms
(%)
B (gauss)
(a)
Ato
mic
Fra
ctio
n
Magnetic Field [G]
1.0
0.5
0.0
900850800750
(b)
FIG. 6: (a) The fraction of 40K atoms as a function of the magnetic field. (b) The fraction of 6Li
atoms as a function of the magnetic field. Cross: initial ramp-down speed=30 G/µs; circle: linear
ramp-down at 100 G/ms; triangle: linear ramp-down at12.5 G/ms. After Ref. [7, 19].
loss is believed to be suppressed. In Ref. [17], the author thus attributed the observed loss
rate to the three-body process simultaneously accompanying by the temperature change.
Fig. 6(a) and (b) show the fractions of fermionic atoms 40K at 224.18 G[19] and 6Li at
822 G[7] as a function of the magnetic field. In either case, the measurement begins from
the BEC side where bound molecules exist. The magnetic field is first swept up to a given
value. If the given magnetic field exceeds the resonant magnetic field, the molecules will
dissociate. During the sweeping which takes about more than ten milliseconds, the molecular
or atomic gas will expand so that the density of the gas is diluted. This action is performed
to avoid the unwanted interference from many-body effects and the reformation of molecules
at successive stage.[6, 7] After the expansion, the magnetic field is fast ramped down to zero.
The fraction of the atoms is then obtained at zero field by optical image method which only
detects the atoms because the transition of molecules does not match the frequency of the
incident light.[6, 14, 27] From Fig. 6(a) and (b), the fraction of atoms greatly increase as the
given magnetic field goes above the resonance, indicating the absence of molecules. Also, in
Fig. 6(b), the fraction of atoms corresponding to different speeds of ramping the magnetic
field down to zero are shown. This ramp-down speed has to be carefully chosen because the
resonant field B0 obtained in this way will shift due to the ramp-down speed.[7] However,
the ramp-down speeds used in the experiments do not significantly change the resonant field.
Fig. 7(a) and (b) show the fraction of the condensate of pair atoms (This term should
10
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-0.5 0 0.5 1.00
0.05
0.10
0.15
-9 -6 -3 0 3 16 18198
200
202
204
B(g
auss
)
t (ms)N
0/N
∆B (gauss)
(a)
Co
nd
en
sa
te F
ractio
n
Magnetic Field [G]
0.8
0.4
0.0
1000800600
(b)
FIG. 7: (a) The decay of 40K2 condensate fraction. Circle: 2 ms hold time; triangle: 30 ms hold
time (b) The decay of 6Li2 condensate fraction. Cross: 2 ms hold time; square: 100 ms hold time;
circle: 10 s hold time. After Ref. [6, 7].
stand for BEC molecules in the BCS side although its real meaning is a bit ambiguous in
these papers.) as a function of magnetic field for 40K[6] and 6Li.[7] Unlike Fig. 6(a) and (b),
the initial magnetic field is set at the BCS side and than brought slowly to a given magnetic
field to avoid the enhanced loss out of the optical trap due to rapid sweeping. No expansion
of atomic gas takes place at this stage. Furthermore, sometimes it is even necessary to in
crease optical power to enhance the confinement of the atomic gas.[7] The atomic gas is
held there for a period of time which is variable in the experiments. After the hold period,
the trap is turned off to allow the gas to expand. Simultaneously[6] or immediately after
the expansion,[7] the magnetic field is soon turned off. Unlike the experiments mentioned
previously, the atom in the gas will be adiabatically turned into molecules due to high
density. The fraction of molecular BEC condensate, which is assumed to be invariant before
and after the turn-off by some subtle argument, is then measured by mapping out the zero
momentum component[7] or Thomas-Fermi profile of the molecules.[6]
In Fig 7 (a) and (b), the fraction of the condensate decays as the hold time increases. As
mentioned in section II, the formation of molecules by sweeping the magnetic field across the
resonance creates vibrationlly-excited molecules. The deexcitation of these molecules will
cause the inelastic scattering and quench the fraction od the BEC condensate. The longer
the hold time is, the more thorough the quenching is. It accounts why significant decay is
observed at longer hold time. Close to the resonance and in the BCS side, the condensate
decays slowly while it decays faster farther away from the resonance in the BEC side because
the molecules are more tightly-bound. The extra bound energy has to be converted into
11
-
0
0.05
0.10
0.15
0.20
-0.4-0.2
00.2
0.40.6
0.8
-0.05
0
0.05
0.10
0.15
N /N0
T/TF
∆B (gauss)
(a)
0
0.2
0.4
0.6
Condensate
Fra
ction a
t 820 G
1000900800700Magnetic Field [G]
0.5
0.3
0.1
0.7
0.8
0.2
0.05
T/TF
(b)
FIG. 8: The fractions of (a) 40K2 BEC condensate and (b)6Li2 BEC condensate as a function of
the magnetic field and temperature. After Ref. [6, 7].
kinetic energy and reduces the condensate fraction.[28]
The argument that the condensate fraction measured in this way is just the condensate
fraction before the turn-off of the magnetic field is subtle. This argument will lead to the
conjecture that the BEC is present in the BCS side.[26] The argument is based on two
assumptions. The first one is that no BEC condensate is created when the magnetic field
drops to zero.[14] The second one is that slightly-correlated atoms tend to randomly pick up
a neighboring atom to form a molecule. Molecules formed in this way have finite momenta
and do not belong to the condensate. Therefore, the original condensate will be directly
projected to the condensate at zero magnetic field.[7] The condensate fraction as a function
of magnetic field and temperature for a given number of atoms is also measured.[6, 7] Fig. 8
(a) and (b) show the corresponding three-dimensional and contour plots for 40K2 and6Li2
molecules. Fig. 8 (a) can be directly compared with Fig. 4 (b) since this figure is an attempt
to fit the experimental data.
V. CONCLUSION
We have briefly surveyed the recent experiments on BEC-BCS crossover. Instead of going
into complicated calculations of many-body dynamics, we only look into those related to
thermal equilibrium. The interesting point of the cold fermionic atoms is the capability of
tuning the scattering length by magnetic field. BEC and BCS types of superfluidity can
thus be achieved in the same system by tuning this controllable parameter. Further, an
interesting regime of superfluidity between BEC and BCS has been opened. More future
work has to be devoted to explore the properties of the superfluidity phase in the regime.
12
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