Transcript
Page 1: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Quantum Spin Hall Effect

- A New State of Matter ? -

Naoto Nagaosa

Dept. Applied Phys. Univ. Tokyo

Collaborators:

M. Onoda (AIST), Y. Avishai (Ben-Grion)

Aug. 1, 2006 @Banff

Page 2: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Bmagnetic field

Voltage

Hall effect

Page 4: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

(Integer) Quantum Hall Effect

Quantized Hall conductance in the unit of h

e2

Plateau as a function of magnetic field

pure case

Disorder effect and localization

Page 5: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

pure case

Localized states do not contribute to xy

Extended states survive only at discrete energies

(Integer) Quantum Hall Effect

Page 6: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Anderson Localization of electronic wavefunctions

xx

ximpurity

Extended Bloch waveLocalized state

EELeGLg d /)/()( 22 Thouless number= Dimensionless conductance

E

L

E

Periodic boundary condition

Anti-periodic boundary condition

quantum interference betweenscattered waves.

Page 7: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Scaling Theory of Anderson Localization

)/),(()( LdLLgfdLLg The change of the Thouless numberIs determined only by the Thouless number Itself.

In 3D there is a metal-insulator transition

In 1D and 2D all the states are localized for any finite disorder !!

Page 8: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Symplectic class with Spin-orbit interaction

Universality classes of Anderson Localization

Orthogonal: Time-reversal symmetric system without the spin-orbit interaction

Symplectic: Time-reversal symmetric system with the spin-orbit interaction

Unitary: Time-reversal symmetry broken Under magnetic field or ferromagnets Chern number extended states

Universality of critical phenomena Spatial dimension, Symmetry, etc. determine the critical exponents.

Page 9: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

xx k/

yy k/

0 2

2wave function

Chern number

cckk

kdi

Cheyx

xy .|4

)//( 22

Page 10: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)
Page 11: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Chern number is carried only by extended states.

Topology “protects” extended states.

Page 12: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Chiral edge modes

Page 13: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

M

vy

x

-e

-e

-e

-eE

Anomalous Hall Effect

magnetization

Electricfield

Hall, Karplus-Luttinger, Smit,Berger, etc.

Berry phase

Page 14: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Electrons with ”constraint”

Projection onto positive energy stateSpin-orbit interaction

as SU(2) gauge connection

Dirac electrons

doublydegenerate

positive energy states.

E

k

Bloch electrons

Projection onto each bandBerry phase

of Bloch wavefunction

k

E

Page 15: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Berry Phase Curvature in k-space

Bloch wavefucntion )()( ruer nkikr

nk

nkknkn uuikA ||)( Berry phase connection in k-space

)()( kAikArx nknii i covariant derivative

)())()((],[ kiBkAkAiyx nznxknyk yx Curvature in k-space

y

VkB

m

k

y

Vyxi

m

kHxi

dt

tdxnz

xx

)(],[],[)(

xk yk

zk

Anomalous Velocity andAnomalous Hall Effect

New Quantum Mechanics !!Non-commutative Q.M.

knku| nku|

k

Page 16: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

dt

tkdkB

k

k

dt

trdn

n )()(

)()(

dt

trdrB

r

rV

dt

tkd )()(

)()(

Duality between Real and Momentum Spaces

k- space curvature

r- space curvature

Page 17: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Gauge flux density

M.Onoda, N.N.J.P.S.P. 2002

Chern #'s : (-1, -2, 3, -4, 5 -1)

Chern number = Integral of the gauge fluxover the 1st BZ.

Distribution of momentum space “magnetic field” in momentum spaceof metallic ferromagnet with spin-orbit interaction.

Page 18: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

M.Onoda-N.N. 2003

Localization in Haldane model -- Quantized anomalous Hall effect

Page 19: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

vy

x

-e

-e

-e

E

Spin Hall Effect

Electric field

v-e

-e

-e

spin currenttime-reversal even

D’yakonov-Perel (1971)

Page 20: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Spin current induced by an electric field

x: current direction y: spin directionz: electric field

SU(2) analog of the QHE• topological origin• dissipationless • All occupied states in the valence ba

nd contribute.• Spin current is time-reversal even

zsLF

HF

zxy E

ekk

eEj

2

1

4 2

GaAs

E

x

y

z

S.Murakami-N.N.-S.C.ZhangJ.Sinova-Q.Niu-A.MacDonald

Page 21: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Let us extend the wave-packet formalism to the case with time-reversal symmetry.

Adiabatic transport = The wave-packet stays in the same band, but can transform inside the Kramers degeneracy.

Wave-packet formalism in systems with Kramers degeneracy

),(),,(),(),,(),()( 22113 LHntxqtqatxqtqaqdt cncnn

),(

),(1

),(

),(

2

1

22

212

1

tqa

tqa

aatqz

tqz

zAkiz

LHnzFzkk

Ex

Eek

n

nljj

l

n

l

,

Eq. of motion

Page 22: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Wunderlich et al.   2004

Experimental confirmation of spin Hall effect in GaAs D.D.Awschalom (n-type)    UC Santa Barbara J.Wunderlich (p-type ) Hitachi Cambridge

Y.K.Kato,et.al.,Science,306,1910(2004)

n-type p-type

Page 23: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Recent focus of theories

Quantum spin Hall effect - A New State of Matter ?

Page 24: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Spin Hall Insulator with real Dissipationless spin current

Zero/narrow gap semiconductors

S.Murakami, N.N., S.C.Zhang (2004)

Rocksalt structure: PbTe, PbSe, PbSHgTe, HgSe, HgS, alpha-Sn

s

Bernevig-S.C.ZhangKane-Mele

rryxrryxr

rryrrxr

rrr

cccc

cccc

cMcH

H.c.3232

H.c.33

)(

52

33

52

33

52

4252

42

521

Quantum spin Hall GenericSpin Hall InsulatorM.Onoda-NN (PRL05)

0

Finite spin Hall conductance but not quantized

No edge modesfor generic spinHall insulator

Page 25: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Two sources of “conservation law”

Rotational symmetry Angular momentumGauge symmetry Conserved current

Topology winding number

Page 26: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Quantum Hall Problem

Quantized Hall Conductance

Localization problem

Topological Numbers

ChernEdge modes

TKNN

2-param. scalin

g

Gauge invariance

TKNN

Conserved charge current and U(1) gauge invariance

Landauer

Page 27: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Issues to be addressed

Spin Hall Conductance

Localization problem

Topological Numbers

Spin Chern, Z2Edge modes

No conserved spin current !!

Kane-MeleXu-MooreWu-Bernevig-ZhangQi-Wu-Zhang

Sheng-Weng-Haldane

Page 28: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Kane-Mele 2005

Kane-Mele Model of quantum spin Hall system

Stability of edge modes Z2 topological number = # of helical edge mode pairs

kk HH Lattice structureand/or inversion symmetry breakingGraphene, HgTe at interface, Bi surface       (Bernevig-S.C.Zhang) (Murakami)

Pfaffian

time-reversal operation

Page 29: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)
Page 30: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

1st BZ

K

K

K

K’

K’

K’

Two Dirac Fermions at K and K’ 8 components

helical edge modes

SU(2) anomaly (Witten) ?

Stability against the T-invariant disorder due to Kramer’s theorem

Kane-Mele, Xu-Moore, Wu-Bernevig-Zhang

Page 31: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Sheng et al. 2006Qi et al. 2006

Chern Number Matrix

CC : spin Chern number

Page 32: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Generalized twisted boundary condition Qi-Wu-

Zhang(2006)

nn 4or 24 Spin Chern number

Page 33: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Issues to be addressed

Spin Hall Conductance

Localization problem

Topological Numbers

Spin Chern, Z2Edge modes

?

No conserved spin current !!

Kane-MeleXu-MooreWu-Bernevig-ZhangQi-Wu-Zhang

Sheng-Weng-Haldane

Page 34: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Two decoupled Haldane model(unitary)

Chern number =0

Chern number =1,-1

Z2 trivialZ2 non-trivial

xh

Generalized Kane-Mele Model

Page 35: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Numerical study of localization MacKinnon’s transfer matrix method and finite size scaling

M

L

Localization length ),( WM

/),1( LeLG

MWMWM /),(),(

Page 36: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

(a-1)

(b-1)

(a-2) (a-3)

(b-2) (b-3)

(c-1) (c-2) (c-3)

2 copies of Haldane model

increasing disorder strength W

Page 37: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Two decoupled unitary modelwith Chern number +1,-1

Symplectic model

Page 38: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

xh

Disappearance of the extended states in unitary model

hybridizes positive andnegative Chern number statesxh

Page 39: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

xh

Disappearance of the extended states in trivial symplectic model

Page 40: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Scaling Analysis of the localization/delocalization transition

73.2symplectic 33.2unitary

Page 41: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Conjectures

Spin Hall Conductance

Localization problem

Topological Numbers

Spin Chern, Z2Helical Edge modes

No conserved spin current !!

No quantized spin Hall conductancenor plateau

Page 42: Quantum Spin Hall Effect - A New State of Matter ? - Naoto Nagaosa Dept. Applied Phys. Univ. Tokyo Collaborators: M. Onoda (AIST), Y. Avishai (Ben-Grion)

Conclusions

Rich variety of Bloch wave functions in solids Symmetry classification Topological classification Anomalous velocity makes the insulator an active player.

Quantum spin Hall systems: No conserved spin current but Analogous to quantum Hall systems characterized by spin Chern number/Z2 number

Novel localization properties influenced by topology New universality class !? Graphene, HgTe, Bi (Murakami) Stability of the edge modes

Spin Current physics Spin pumping and ME effect

EE


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