experiments of sto synchronization by electrical connection · (mattana, af et al) as in this...
TRANSCRIPT
trilayer 1
1.0 1.1 1.2 1.30.0
0.1
0.2
0.3
0.4
0.5
0.6
po
we
r (p
W/G
Hz/m
A2
)
frequency (GHz)
- 9 mA
-12.4 mA
increasing I
1.0 1.1 1.2 1.3
0.0
0.1
0.2
0.3
0.4
0.5
0.6
po
we
r (p
W/G
Hz/m
A2)
frequency (GHz)
-11.00mA
-9.80mA
Idc Ihf1+
trilayer 2
Ihf2+
hf circuit
Ihf1+ Ihf2
Idc
Experiments of STO synchronization by electrical connection
(B.Georges, AF et al, CNRS/Thales and LPN-CNRS, preliminary results)
Spintronique avec semi-conducteurs
et molécules
GaMnAs (Tc→170K) and R.T. FS
Electrical control of ferromagnetism
TMR, TAMR, spin transfer (GaMnAs)
Field-induced metal/insulator transition
Spintronics with semiconductors
Magnetic metal/semiconductor
hybrid structures
Example: spin
injection from
Fe into LED
(Mostnyi et al,
PR. B 68, 2003)
Ferromagnetic
semiconductors (FS)
GaMnAs (Tc→170K) and R.T. FS
Electrical control of ferromagnetism
TMR, TAMR, spin transfer (GaMnAs)
Field-induced metal/insulator transition
Spintronics with semiconductors
Magnetic metal/semiconductor
hybrid structures
Example: spin
injection from
Fe into LED
(Mostnyi et al,
PR. B 68, 2003)
Ferromagnetic
semiconductors (FS)
F1 F2
Semiconductor
channel
V
Spin Field Effect Transistor ?
Semiconductor channel between
spin-polarized source and draintransforming spin information into
large (?) and tunable (by gate voltage) electrical signal
Nonmagnetic lateral channel between spin-polarized source and drain
Semiconductor channel:
« Measured effects of the order of 0.1-1% have been reported for the change in
voltage or resistance (between P and AP)…. », from the review article
« Electrical Spin Injection and Transport in Semiconductors » by BT Jonker
and ME Flatté in Nanomagnetism (ed.: DL Mills and JAC Bland, Elsevier 2006)
F1 F2
Semiconductor channel
PAP
Nonmagnetic lateral channel between spin-polarized source and drain
Semiconductor channel:
« Measured effects of the order of 0.1-1% have been reported for the change in
voltage or resistance (between P and AP)…. », from the review article
« Electrical Spin Injection and Transport in Semiconductors » by BT Jonker
and ME Flatté in Nanomagnetism (ed.: DL Mills and JAC Bland, Elsevier 2006)
Carbon nanotubes:
LSMO LSMO
LSMO = La2/3Sr1/3O3
nanotube
1.5 µµµµm
L.Hueso, N.D. Mathur,A.F. et al, Nature 445, 410, 2007
F1 F2
Semiconductor channel
PAP
Nonmagnetic lateral channel between spin-polarized source and drain
Semiconductor channel:
« Measured effects of the order of 0.1-1% have been reported for the change in
voltage or resistance (between P and AP)…. », from the review article
« Electrical Spin Injection and Transport in Semiconductors » by BT Jonker
and ME Flatté in Nanomagnetism (ed.: DL Mills and JAC Bland, Elsevier 2006)
Carbon nanotubes:
∆∆∆∆R/R ≈≈≈≈ 60-70%, VAP-VP ≈≈≈≈ 60 mV
APAPAPAP
PPPP PPPPLSMO LSMO
LSMO = La2/3Sr1/3O3
nanotube
1.5 µµµµm
L.Hueso, N.D. Mathur,A.F. et al, Nature 445, 410, 2007
F1 F2
Semiconductor channel
PAP
60%
MR=72 %
Nonmagnetic lateral channel between spin-polarized source and drain
Semiconductor channel:
« Measured effects of the order of 0.1-1% have been reported for the change in
voltage or resistance (between P and AP)…. », from the review article
« Electrical Spin Injection and Transport in Semiconductors » by BT Jonker
and ME Flatté in Nanomagnetism (ed.: DL Mills and JAC Bland, Elsevier 2006)
Carbon nanotubes:
∆∆∆∆R/R ≈≈≈≈ 60-70%, VAP-VP ≈≈≈≈ 60 mV
LSMO LSMO
LSMO = La2/3Sr1/3O3
nanotube
1.5 µµµµm
L.Hueso, N.D. Mathur,A.F. et al, Nature 445, 410, 2007
F1 F2
Semiconductor channel
PAP
AF and Jaffrès
PR B 2001
+cond-mat
0612495, +
IEEE Tr.El.Dev. 54,5,921,2007
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
sfbn
b
sfnP
rfor
raszerotodrops
R
R
ττ
ττγγ
>>∝
+−
=∆
*
*
22
/1
/1
)1/(
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
v
rL
vt
L
timedwell
b
r
n
*
*
2∝=τ
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
L
NsfNN
b
lr
r
ρ
γ
=
=
∝=
resistance interface theofasymmetry spin
teff1/trans.coresist.interfaceareaunit **r
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
F1 F2
Semiconductor
channel
V
L
F1 F2
Semiconductor
channel
V
L
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
LInterface resistance rb*
in most experimentsNsf
l
LNrbr <<*
Two interface
spin transportproblem (diffusive regime)
sfn ττ >>..,*ei
L
lrr
Nsf
Nb >>
AF and Jaffrès
PR B 2001
+cond-mat
0612495, +
IEEE Tr.El.Dev. 54,5,921,2007
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
al)etAF(Mattana,
examplethisinas
raszerotodrops
R
R
b
sfnP
*
22
/1
/1
)1/(
ττγγ
+−
=∆
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
L
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
F1 F2
Semiconductor
channel
V
L
F1 F2
Semiconductor
channel
V
L
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
L
Nsf
l
LNrbr <<*
Two interface spin transport
problem (diffusive regime)
b
Magnetic field (Oe)
1E-3 0.01 0.10
10
20
30
40
50
T=4K
GaAs QW=6nm
1.95nm1.45nm1.7nm
MR ( % )
b
Magnetic field (Oe)
1E-3 0.01 0.10
10
20
30
40
50
T=4K
GaAs QW=6nm
1.95nm1.45nm1.7nm
MR ( % )
)( 2* cmr b Ω
GaMnAs/AlAs/GaAs/AlAs/GaMnAs vertical structure
v
rL
vt
L
timedwell
b
r
n
*
*
2∝=τ
Carbon nanotubes between spin-polarized sources and drains
La2/3Sr1/3MnO3(LSMO)
La2/3Sr1/3MnO
3 (LSMO)
MR=72 %
PPPP PPPP
MR=60 %
L ≈ 1-2 µm
NanotubesNanotubesNanotubesNanotubes ((((also graphenealso graphenealso graphenealso graphene, , , , other moleculesother moleculesother moleculesother molecules) :) :) :) :
)(long2
)/10(long 317
sfr
n
sf
istv
Lsmallisvbut
cmelnforbecan
ττ
τ
>>=→
≈SemiconductorsSemiconductorsSemiconductorsSemiconductors::::
sfnsfn
Pif
R
RP
P
ττττγγ
<+
−=
∆
===
largeis,/1
)1/(),off(Aand(on)Pbetweencontrastthe:
Sinjectionγlifetime,spinτtime,dwellτ:drainandsourceSPbetweenTransport
22
sfn
)50(2
CNT)in50ns(long
sfr
n
sf
nsshortrelativelyistv
Lvvelocityhigh
islifetimespinorbitspinsmall
ττ
τ
≈≈=→
≈→−
NanotubesNanotubesNanotubesNanotubes ((((also graphenealso graphenealso graphenealso graphene, , , , other moleculesother moleculesother moleculesother molecules) :) :) :) :
)50(2
CNT)in50ns(long
sfr
n
sf
nsshortrelativelyistv
Lvvelocityhigh
islifetimespinorbitspinsmall
ττ
τ
≈≈=→
≈→−
)(long2
)/10(long 317
sfr
n
sf
istv
Lsmallisvbut
cmelnforbecan
ττ
τ
>>=→
≈SemiconductorsSemiconductorsSemiconductorsSemiconductors::::
Solution for semiconductors:
shorter L ?, larger transmission tr ?
sfnsfn
Pif
R
RP
P
ττττγγ
<+
−=
∆
===
largeis,/1
)1/(),off(Aand(on)Pbetweencontrastthe:
Sinjectionγlifetime,spinτtime,dwellτ:drainandsourceSPbetweenTransport
22
sfn
NanotubesNanotubesNanotubesNanotubes ((((also graphenealso graphenealso graphenealso graphene, , , , other moleculesother moleculesother moleculesother molecules) :) :) :) :
)(long2
)/10(long 317
sfr
n
sf
istv
Lsmallisvbut
cmelnforbecan
ττ
τ
>>=→
≈SemiconductorsSemiconductorsSemiconductorsSemiconductors::::
Solution for semiconductors:
shorter L ?, larger transmission tr ?
Potential of molecular
spintronics (nanotubes,
graphene and others)
sfnsfn
Pif
R
RP
P
ττττγγ
<+
−=
∆
===
largeis,/1
)1/(),off(Aand(on)Pbetweencontrastthe:
Sinjectionγlifetime,spinτtime,dwellτ:drainandsourceSPbetweenTransport
22
sfn
)50(2
CNT)in50ns(long
sfr
n
sf
nsshortrelativelyistv
Lvvelocityhigh
islifetimespinorbitspinsmall
ττ
τ
≈≈=→
≈→−
NanotubesNanotubesNanotubesNanotubes ((((also graphenealso graphenealso graphenealso graphene, , , , other moleculesother moleculesother moleculesother molecules) :) :) :) :
)(long2
)/10(long 317
sfr
n
sf
istv
Lsmallisvbut
cmelnforbecan
ττ
τ
>>=→
≈SemiconductorsSemiconductorsSemiconductorsSemiconductors::::
Solution for semiconductors:
shorter L ?, larger transmission tr ?
Potential of molecular
spintronics (nanotubes,
graphene and others)
Next challenge for molecules:
spin control by gate
sfnsfn
Pif
R
RP
P
ττττγγ
<+
−=
∆
===
largeis,/1
)1/(),off(Aand(on)Pbetweencontrastthe:
Sinjectionγlifetime,spinτtime,dwellτ:drainandsourceSPbetweenTransport
22
sfn
)50(2
CNT)in50ns(long
sfr
n
sf
nsshortrelativelyistv
Lvvelocityhigh
islifetimespinorbitspinsmall
ττ
τ
≈≈=→
≈→−
MR of LSMO/Alq3/Co structures (preliminary results)
Collaboration CNRS/Thales [C. Barraud, P. Seneor et al) and CNR Bologna (Dediu et al)]
Alq3 (50nm)
LSMO
Co
resist
1- 4 nm
Co nanocontact
≈≈≈≈10 nm
LSMO Co
Alq3
LUMO
HOMOAlq3 = π - conjugated 8-hydroxy-quinoline aluminium
ELECTRONIQUE
SPINTRONIQUE
Summary
¤Already important aplications of GMR/TMR (HDD, MRAM..) and now promising new fields
-Spin transfer formagnetic switching and microwave generation
-Spintronics with semiconductors, molecules or nanoparticles
M. Anane, C. Barraud, A. Barthélémy, H. Bea, A. Bernand-
Mantel, M. Bibes, O. Boulle, K.Bouzehouane, O. Copi, V.Cros,
C. Deranlot, B. Georges, J-M. George, J.Grollier, H. Jaffrès, S.
Laribi, J-L. Maurice, R. Mattana, F. Petroff, P. Seneor, M.
Tran F. Van Dau, A. Vaurès
Université Paris-Sud and Unité Mixte de Physique CNRS-Thales, Orsay, France
P.M. Levy, New York University, A.Hamzic, Zagreb University
B. Lépine, A. Guivarch and G. Jezequel
Unité PALMS, Université de Rennes , Rennes, France
G. Faini, R. Giraud, A. Lemaître: CNRS-LPN, Marcoussis, France
L. Hueso, N.Mathur, Cambridge
J. Barnas, M. Gimtra, I. Weymann, Poznan University
Acknowledgements to
J↑↑↑↑-J↓↓↓↓
J↑↑↑↑+J↓↓↓↓*
*
bNF
bF
rrr
rr
++
+=
γβDeviations from at large current density (drift effect)
= low current limit
current density
= deviations from
the low current limit (nondegenerate
semiconductor)
from Jaffrès and A.F.
(see also Yu and Flatté)
NMNMNMNM = = = = semiconductorsemiconductorsemiconductorsemiconductor
EF↑
Rasbah, PR B 2000
A.F-Jaffrès, PR B 2001
Spin accumulation ∆µ∆µ∆µ∆µ= EF↑↑↑↑-EF↓↓↓↓
NMsfl
FMsfl
z
EF↑
Current Spin Polarization (J↑↑↑↑-J↓↓↓↓)/(J↑↑↑↑+J↓↓↓↓)
FMFMFMFMspin dependent. interf.
resist. (ex:tunnel barrier)
EF↓↓↓↓
EF↑↑↑↑
Spin dependent drop of the
electro-chemical potential
Discontinuity increases the
spin accumulation in NM
re-balanced spin relaxations
in F and NM
extension of the spin-
polarized current into the
semiconductor
e-
NsfNNb lrr ρ=≈*
NsfNNb lrr ρ=>>*
Spin injection/extraction at a Semiconductor/FM interface
AF and Jaffrès
PR B 2001
+cond-mat
0612495, +
IEEE Tr.El.Dev. 54,5,921,2007
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
sfbn
b
sfnP
rfor
raszerotodrops
R
R
ττ
ττγγ
>>∝
+−
=∆
*
*
22
/1
/1
)1/(
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
v
rL
tv
L
timedwell
b
r
n
*
*
2∝=τ
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
L
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
LInterface resistance rb*
in most experiments
with semiconductors
and lateral channel
Nsf
l
LNrbr <<*
Two interface
spin transportproblem (diffusive regime)
NanotubesNanotubesNanotubesNanotubes::::
)(2
50ns)(long
sfr
n
sf
shortistv
Lvvelocityhigh
islifetimespinorbitspinsmall
ττ
τ
<=→
≈→−sfn ττ >>
AF and Jaffrès
PR B 2001
+cond-mat
0612495, +
IEEE Tr.El.Dev. 54,5,921,2007
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
sfbn
b
sfnP
rfor
raszerotodrops
R
R
ττ
ττγγ
>>∝
+−
=∆
*
*
22
/1
/1
)1/(
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
v
rL
tv
L
timedwell
b
r
n
*
*
2∝=τ
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
L
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
LInterface resistance rb*
in most experiments
with semiconductors
and lateral channel
Nsf
l
LNrbr <<*
Two interface
spin transportproblem (diffusive regime)
)(long2
)/10(long 317
sfr
n
sf
istv
Lsmallisvbut
cmelnforbecan
ττ
τ
>>=→
≈
SemiconductorsSemiconductorsSemiconductorsSemiconductors::::sfn ττ >>
AF and Jaffrès
PR B 2001
+cond-mat
0612495, +
IEEE Tr.El.Dev. 54,5,921,2007
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
sfbn
b
sfnP
rfor
raszerotodrops
R
R
ττ
ττγγ
>>∝
+−
=∆
*
*
22
/1
/1
)1/(
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
v
rL
tv
L
timedwell
b
r
n
*
*
2∝=τ
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
L
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
LInterface resistance rb*
in most experiments
with semiconductors
and lateral channel
Nsf
l
LNrbr <<*
Two interface
spin transportproblem (diffusive regime)
Solution for semiconductors:
shorter L ?, larger transmission tr ? sfb
r
nv
rL
tv
Lττ >>∝=
*
*
2
AF and Jaffrès
PR B 2001
+cond-mat
0612495, +
IEEE Tr.El.Dev. 54,5,921,2007
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
sfbn
b
sfnP
rfor
raszerotodrops
R
R
ττ
ττγγ
>>∝
+−
=∆
*
*
22
/1
/1
)1/(
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
v
rL
tv
L
timedwell
b
r
n
*
*
2∝=τ
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
L
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
LInterface resistance rb*
in most experiments
with semiconductors
and lateral channel
Nsf
l
LNrbr <<*
Two interface
spin transportproblem (diffusive regime)
sfb
r
nv
rL
tv
Lττ >>∝=
*
*
2Potential of molecular
spintronics (nanotubes,
graphene and others)
AF and Jaffrès
PR B 2001
+cond-mat
0612495, +
IEEE Tr.El.Dev. 54,5,921,2007
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
sfbn
b
sfnP
rfor
raszerotodrops
R
R
ττ
ττγγ
>>∝
+−
=∆
*
*
22
/1
/1
)1/(
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
v
rL
tv
L
timedwell
b
r
n
*
*
2∝=τ
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
L
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
LInterface resistance rb*
in most experiments
with semiconductors
and lateral channel
Nsf
l
LNrbr <<*
Two interface
spin transportproblem (diffusive regime)
Next challenge for molecules:
spin control by gate
sfn ττ >>Potential of molecular
spintronics (nanotubes,
graphene and others)
NMNMNMNM FMFMFMFM
zone of spin accumulation
NMsfl
FMsfl
EF↑
EF↑↑↑↑(z)
Spin accumulation
∆µ∆µ∆µ∆µ= EF↑↑↑↑-EF↓↓↓↓
Spin current
= J↑↑↑↑-J↓↓↓↓
z
z
J↑↑↑↑-J↓↓↓↓
F Ms fl = spin diffusion length in F
= spin diffusion length in NMN Ms fl
N Ms fl
FMsfl
EF↓↓↓↓(z)
E
2/111)](3/[
−↓
−↑
+= λλλFsf
2/1)6/(
NNsf
λλ=
Description* : Boltzmann-type equation with a
distribution function in which the equilibrium
chemical potential is replaced by
, function of σσσσ and z
which leads to macroscopic equations**relating the charge and spin currents to a spin
dependent electro-chemical potential
µµµµσσσσ(z)= eV(z) + EFσσσσ(z)
to finally,after having also introduced the
interface resistance boundary counditions,
derive the profiles of the spin accumulation
and spin↑↑↑↑(spin↓↓↓↓) currents
*Valet and Fert, PR B 48, 7099, 1993.** the same as in Silsbee-Johnson and van Son et al
)(zEFσ0FE
Spin injection/extraction at a NM/FM interface (beyond ballistic range)
I < 0I < 0I < 0I < 0
Standard behavior (initial state = P, I < 0)
¤ switching at low field
¤ precession regime at high field
0.1
0.2
0 0.5 1
ϕ/πϕ/πϕ/πϕ/π
ττττ ϕϕ ϕϕ/(ħ
|I0|/|e
|)
P AP
Standard Standard Standard Standard angularangularangularangular dependencedependencedependencedependence(ex: (ex: (ex: (ex: CoCoCoCo////CuCuCuCu////CoCoCoCo))))
fixedfixedfixedfixed MMMM
mmmmϕϕϕϕ
APAPAPAP
PPPP
I < 0 , H = 0I < 0 , H = 0I < 0 , H = 0I < 0 , H = 0Switching Switching Switching Switching
from from from from P to APP to APP to APP to AP
I < 0I < 0I < 0I < 0
I > 0I > 0I > 0I > 0
APP
Torque on the free layer (Py) as a function of the angle between m(m(m(m(PyPyPyPy)))) and M(Co) for
Shorter SDL in the free layer, ex: Co8(fixed)/Cu10/Py8(free)
I < 0I < 0I < 0I < 0
I > 0I > 0I > 0I > 0
APP
J. J. J. J. BarnasBarnasBarnasBarnas, A. , A. , A. , A. FertFertFertFert. et al, . et al, . et al, . et al, Phys. Rev. B 2005, Mat.Sc.Eng. B126,271,2006
Spin transfer torque
I < 0I < 0I < 0I < 0
I > 0I > 0I > 0I > 0
APP
Shorter SDL in the free layer, ex: Co8(fixed)/Cu10/Py8(free)
I < 0I < 0I < 0I < 0
I > 0I > 0I > 0I > 0
APP
J. J. J. J. BarnasBarnasBarnasBarnas, A. , A. , A. , A. FertFertFertFert. et al, . et al, . et al, . et al, Phys. Rev. B 2005, Mat.Sc.Eng. B126,271,2006
Spin transfer torque
fixedfixedfixedfixed MMMM
mmmmϕϕϕϕ
APAPAPAP
PPPP
0.1
0.2
0 0.5 1
ϕ/πϕ/πϕ/πϕ/π
ττττ ϕϕ ϕϕ/(ħ
|I0|/|e
|)
P AP
Standard Standard Standard Standard angularangularangularangular dependencedependencedependencedependence(ex: (ex: (ex: (ex: CoCoCoCo////CuCuCuCu////CoCoCoCo))))
I < 0 , H = 0I < 0 , H = 0I < 0 , H = 0I < 0 , H = 0Switching from Switching from Switching from Switching from
P to APP to APP to APP to AP
I < 0I < 0I < 0I < 0
I < 0 , I < 0 , I < 0 , I < 0 , inactiveinactiveinactiveinactive
fixedfixedfixedfixed MMMM
mmmmϕϕϕϕ
APAPAPAP
PPPP
I >0 , H = 0 I >0 , H = 0 I >0 , H = 0 I >0 , H = 0 precessionprecessionprecessionprecession
fixedfixedfixedfixed MMMM
mmmmϕϕϕϕ
APAPAPAP
PPPP
inversion
-6 -4 -2 0 2
14.4
15.0
dV
/dI
( ΩΩ ΩΩ)
I (mA)
High field (H>Hc)
Low field (H<Hc)
I>0
Switching from
AP to P
I<0
Switching from
P to AP
VSD
VG
e∆V = 25-500 meV
>> Coulomb energy
and level spacing,
K< T <120 K
drainsource
nanotube
Quasi-continuous DOS, same conditions
as for semiconductor or metallic channel
drainsource
nanotube
Uc=e2/2C
δE+Uc
e∆V ≈ 1 meV
Usual
conditions:
small bias
voltage
experiments
LSMO/CNT/LSMO:
higher voltage
experiments thanks to
large interface
resistances and small
V2/R heating at large V
Oscillatory variation of the conductance,
different signs of theMR depending on the
bias voltage and from sample to sample
PAP
MR=60% AP
P P
Vbias=25 mV
T = 5 K
CNT instead of semiconductor : LSMO/CNT/LSMO (Hueso, Mathur, Fert et al,
Nature,445, 440, 2007)
LSMO LSMO
LSMO = La2/3Sr1/3O3
Carbon nanotube (CNT)1.5 µµµµm (multi-wall)
MR=72 %
MR=45 %MR=54 %
other samples
MR=60%
MR
/MR
(5K
, 25
m)
rb* ≅≅≅≅70 MΩΩΩΩ
AF and Jaffrès
PR B 2001
+cond-mat
0612495, +
IEEE Tr.El.Dev. 54,5,921,2007
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
al)etAF(Mattana,
examplethisinas
raszerotodrops
R
R
b
sfnP
*
22
/1
/1
)1/(
ττγγ
+−
=∆
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
v
rL
tv
L
timedwell
b
r
n
*
*
2∝=τ
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
L
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
F1 F2
Semiconductor
channel
V
L
F1 F2
Semiconductor
channel
V
L
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
L
Nsf
l
LNrbr <<*
Two interface
spin transportproblem (diffusive regime)
b
Magnetic field (Oe)
1E-3 0.01 0.10
10
20
30
40
50
T=4K
GaAs QW=6nm
1.95nm1.45nm1.7nm
MR ( % )
b
Magnetic field (Oe)
1E-3 0.01 0.10
10
20
30
40
50
T=4K
GaAs QW=6nm
1.95nm1.45nm1.7nm
MR ( % )
)( 2* cmr b Ω
GaMnAs/AlAs/GaAs/AlAs/GaMnAs vertical structure
AF and Jaffrès
PR B 2001
+cond-mat
0612495, +
IEEE Tr.El.Dev. 54,5,921,2007
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
sfbn
b
sfnP
rfor
raszerotodrops
R
R
ττ
ττγγ
>>∝
+−
=∆
*
*
22
/1
/1
)1/(
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
v
rL
tv
L
timedwell
b
r
n
*
*
2∝=τ
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
L
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
10-4
10-2
100
102
104
0.00
0.05
0.10
0.15
0.20
0.25
0.30
0.35
N
lSF=2µm
tN=20nm
tN=2µm
tN=200nm
rb
*////rN
∆∆ ∆∆R/R
P
Condition
dwell time ττττn < spin lifetime ττττsf
Condition for
spin injection
Nb rr /*
∆R
/RP
1−∝L
lwindow
sf
1.6
1.2
0.8
0.4
0.0
L=20nmL
LInterface resistance rb*
in most experiments
with semiconductors
and lateral channel
Nsf
l
LNrbr <<*
Two interface
spin transportproblem (diffusive regime)
sfn ττ >>F1 F2
Semiconductor
channel
V
L
F1 F2
Semiconductor
channel
V
L