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First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC WSU KNMI NIWA Univ. Leicester PSI TNO RIVM KNMI

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 CIMEL sunphotometer (TNO) → AOD at different wavelengths & ssalb, phase-function  Nephelometer (PSI,TNO) → surface extinction & ssalb, phase-function  Ramen LIDAR (RIVM) → aerosol extinction profiles  Ceilometer (KNMI) → boundary layer height  Backscatter lidar (RIVM) → boundary layer height The participants:  …

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Page 1: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

First results of the aerosol profiling group

IUP HeidelbergBIRA-IASBMPIC MainzIUP BremenJAMSTEC

WSUKNMINIWAUniv. Leicester

PSITNORIVMKNMI

Page 2: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

The participants: MAX-DOAS

JAMSTEC → aerosol extinction profiles → VIS → 1km grid;

parameterized

IUP HDB → aerosol extinction profiles → VIS → 200m grid

BIRA → aerosol extinction profiles → UV and VIS → 200m grid

MPI → aerosol extinction profiles → UV → AOD + surface ext. + layer

height + f=0.9 IUP Bremen → AOD → VIS → ?; parameterized

Page 3: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

CIMEL sunphotometer (TNO)

→ AOD at different wavelengths & ssalb, phase-function

Nephelometer (PSI,TNO) → surface extinction & ssalb, phase-function

Ramen LIDAR (RIVM) → aerosol extinction profiles

Ceilometer (KNMI) → boundary layer height

Backscatter lidar (RIVM) → boundary layer height

The participants:

Page 4: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

Results; BIRA

Page 5: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

AOD time series

Page 6: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

AOD time series

Page 7: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

AOD MAXDOAS vs. CIMEL

Page 8: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

AOD MAXDOAS vs. CIMEL

Measured O4 DSCD are reduced by ~20% for BIRA, MPI, IUP HDBNot for JAMSTEC and IUP Bremen

Page 9: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

With correction Without correction

AOD MAXDOAS vs. CIMEL

Page 10: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

Correcting the O4 DSCD

Page 11: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

Case: 30° elevation , pointing north, clear-sky , AOD<0.15

Correcting the O4 DSCDBased on the Beijing dataset

→ Measured and simulated O4 DSCD should be equal

But sim. O4 DSCDs = meas. O4 DSCDs * 0.80.1

Page 12: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

12

Measured DS SCDO4 is within 2% of the simulated using Hermans et al. cross section at room T (477 nm).

1.02

1.01

1.00

0.99

0.98

Rat

io [s

im S

CD

/ m

easu

red

SCD

]

181614121086UTC

23-JUNE-2009

3.0

2.5

2.0

1.5

1.0

0.5

0.0

DS

O2-

O2

dSC

D x

1043

3.53.02.52.01.5Direct sun AMF

DIRECT SUN O2-O2: Coefficient values ± sigma SCDref = -1.53e+43 ± 8.55e+40 VCDmeas = 1.32e+43 ± 4.58e+40 VCDsim = 1.31e+43 Teff = 266 K

23-JUNE-2009

Direct sun results VIS; Elena Spinei

Page 13: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

Correcting the O4 DSCD? Are we really sure that the simulations are correct .That the differences are not caused by errors in other forward model parameters

Aerosol optical properties, … Error in measured O4 DSCD

Error in the spectra Error in DOAS fit

? O4 cross-section

No Yes

or

?

?

Page 14: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

Influence of ssalb and g

Page 15: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

BIRA VIS Heidelberg VIS

JAMSTEC VIS

Contour plots

Page 16: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

BIRA UV MPI UV

Contour plots

Page 17: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

BIRA VIS

Heidelberg VIS

JAMSTEC VIS

Contour plots; identical scales

Page 18: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

BIRA UV

MPI UV

But; better results for f=1.1Uplifted aerosol layer

Contour plots; identical scales

Page 19: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

BIRA VIS

Heidelberg VIS

JAMSTEC VIS

Contour plots

Page 20: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

BIRA UV MPI UV

Contour plots

Page 21: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

BIRA VIS

Heidelberg VIS

JAMSTEC VIS

Contour plots; identical scales

Page 22: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

BIRA UV

MPI UV

Contour plots; identical scales

Page 23: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

Aerosol inter-comparisons: plans for the future

Retrieving synthetic profiles:

BIRA will provide O4 DSCDs and relative intensities at 4 wavelengths for 4 aerosol cases: low AOD and high AOD; surface layer and up-lifted layer

Try to retrieve the profiles using your best settings; the settings agreed on for the real data.

MAXDOAS

→ Focus on both AOD and profiles

Page 24: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

+ Sensitivity tests concerning ssalb, phase function,…

Aerosol inter-comparisons: plans for the future

Real data On your own data set On the Heidelberg dataset (data until October the 5th) Retrievals using your own best settings Retrievals using settings as similar as possible

Apriori extinction: exponential profile, SH=1km, AOD=0.1; Height grid for the simulations: 200m grid to 4km. Covariance matrix: 100% of apriori; 100m or 500m (HDB suggestion). Atmosphere (P,T): USstandard O3+NO2: USstandard Lambertian surface albedo: 5% Aerosol: optical properties are based on mean Nephelometer: g=0.65 and single scattering albedo = 0.95; wavelengths: 360, 477, 577, 630nm if possible

Page 25: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

MAXDOAS vs other instruments

Insitu data, nephelometer (Paul Zieger)

Aerosol extinction from Raman LIDAR (Arnoud Apituley)

Paper on MAXDOAS intercomparison and the Nephelometer paper by June-July

→ deadline for data submission: end March

Aerosol inter-comparisons: plans for the future

Page 26: First results of the aerosol profiling group IUP Heidelberg BIRA-IASB MPIC Mainz IUP Bremen JAMSTEC…

Summary The agreement between the different aerosol retrievals has already improved compared to the previous workshop

Questions

What’s up with the O4 DSCD?What can we actually achieve?(what is our sensitivity, how sensitive are we towards forward model parameters and towards a-priori information, can we obtain “substitute aerosol profiles” for clouds,…)

Conclusion for now

We are making progress

But we still have a lot of work to do; a lot of questions to answer

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