measurement of nuclear reaction cross sections of rare

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lOO-Ab-LOSbf-L-DNd PNC TJ9607 97-001 80 PNC-TJ9607-97-001 am*# JP9709020 # ± © s r m m m © ay m -m (mz>F - 1 9 9 7 # 3 m iiimnn 330025188® * JK I* ± ^

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Page 1: Measurement of nuclear reaction cross sections of rare

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Inquiries about copyright and reproduction should be addressed to : Technology

Management Section Oarai Engineering Center, Power Reactor and Nuclear Fuel

Development Corporation 4002 Narita-cho, 0-arai-machi, Higashi-Ibaraki,

Ibaraki-Ken, 311-13, Japan

thjj'lp • (Power Reactor and Nuclear Fuel Development

Corporation)1997

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Page 4: Measurement of nuclear reaction cross sections of rare

PNC TJ9607 97-001 MARCH. 199 7

Measurement of Nuclear Reaction Cross Sections of Rare Earth Nuclides-H

Masayuki Igashira* *

Abstract

When minor actinides (MA) are returned to a core of fast breeder reactor for the purpose of incineration of them, rare earth nuclides and so on(RE) are also returned to the core because the separation of MA from RE is difficult at present. Then, accurate neutron cross section data of RE become necessary for investigating the characteristics of the core.

Therefore, the measurement of keV-neutron capture cross sections of l43Nd and 14lNd were performed to obtain the accurate data. The measurement was relative to the standard capture cross sections of 1,7Au. A neutron time-of-flight method was adopted with a ns-pulsed neutron source by a Pelletron accelerator and a large anti -Compton NaI(Tl) gamma-ray detector. As a result, the capture cross sections of those nuclides were obtained with the error of about 4 % in an incident neutron energy re­gion of 10 to 560 keV.

A comparison between the present data and the evaluated values of JENDL-3.2 showed that JENDL-3.2 provided good evaluations for 14SNd, but underestimated the capture cross sections of 14*Nd by 10-20 % at neutron energies below 30 keV and overestimated them by about 20 % at 560 keV, whereas it provided good evaluations in the energy re­gion of 40-70 keV. The discrepancy is caused by the weak dependency of evaluated cross sections on the incident neutron energy.

Work performed by Tokyo Institute of Technology under contract with Power Reactor and Nuclear Fuel Development Corporation

PNC Liaison : Toshio Wakabayashi, Core Physics Research Section, Advanced Technology Division

* : Research Laboratory for Nuclear Reactors, Tokyo Institute of Technology

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Page 21: Measurement of nuclear reaction cross sections of rare

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Page 22: Measurement of nuclear reaction cross sections of rare

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Page 23: Measurement of nuclear reaction cross sections of rare

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Page 30: Measurement of nuclear reaction cross sections of rare

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Page 33: Measurement of nuclear reaction cross sections of rare

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Page 35: Measurement of nuclear reaction cross sections of rare

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- 30 -

Page 36: Measurement of nuclear reaction cross sections of rare

2. 7 m%.

143NdS.UJ145NdWi^^(O^S^oV'T, *&Jf-^;V3I-5~8 0 k e5 5 0 k e V 'itz 0 5~8 0 k e VOlel^-eiJ, ® 7~ 1 3 k e V (TO 1IkeV) ,©14~25keV (TO 2 0 k e V) , © 2 6 ~ 3 4 k e V (TO 3 0 k e V) , ®3 5~4 5 k e V (W4 0keV) ,®46~54keV ffi^50keV) ,©55~6 5 k e V (TO 6 0 k e V) , S.U5© 66~78keV (TO 7 2 k e V) <D 7

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Page 37: Measurement of nuclear reaction cross sections of rare

m3

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- 32 -

Page 38: Measurement of nuclear reaction cross sections of rare

#4 h^SrS*)£LfclS50&fl=

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33 -

Page 39: Measurement of nuclear reaction cross sections of rare

3

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34 -

Page 40: Measurement of nuclear reaction cross sections of rare

Cou

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35 -

Page 41: Measurement of nuclear reaction cross sections of rare

Cou

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Page 42: Measurement of nuclear reaction cross sections of rare

Elh-»

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Energy (keV)

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Page 44: Measurement of nuclear reaction cross sections of rare

0.020

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r| (1

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Page 46: Measurement of nuclear reaction cross sections of rare

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Page 47: Measurement of nuclear reaction cross sections of rare

Coun

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42 -

Page 48: Measurement of nuclear reaction cross sections of rare

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Page 49: Measurement of nuclear reaction cross sections of rare

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Page 50: Measurement of nuclear reaction cross sections of rare

I

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Page 52: Measurement of nuclear reaction cross sections of rare

- LV -

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Page 53: Measurement of nuclear reaction cross sections of rare

101 -r

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Page 54: Measurement of nuclear reaction cross sections of rare

Cou

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Page 55: Measurement of nuclear reaction cross sections of rare

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Page 56: Measurement of nuclear reaction cross sections of rare

3 • 3 M9E4' — K

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Page 57: Measurement of nuclear reaction cross sections of rare

rsd)w(i)

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Page 58: Measurement of nuclear reaction cross sections of rare

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53 -

Page 59: Measurement of nuclear reaction cross sections of rare

n :

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Page 60: Measurement of nuclear reaction cross sections of rare

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Page 61: Measurement of nuclear reaction cross sections of rare

E5

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DW2 DW3 DW4 DW5 DW6 DW7

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- 56 -

Page 62: Measurement of nuclear reaction cross sections of rare

4

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Page 63: Measurement of nuclear reaction cross sections of rare

me xwftx-nbtitz’ptemmmfcfomffim (mb)

Ed(keV) 143Nd 145Nd

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Page 64: Measurement of nuclear reaction cross sections of rare

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Page 67: Measurement of nuclear reaction cross sections of rare

1) G. Zeisel: Acta. Phys. Austr. , 23, 5223 (1966).

2) L. A. McVey, R. L. Brodzinski, and T. M. Tanner: J. Radio. Chem., 76, 131 (1983).3) H. Harada, T. Sekine, Y. Hatsukawa, N. Shigeta, K. Kobayashi, T. Ohtsuki, and

T. Katoh: J. Nucl. Sci. Technol., 31, 173 (1994).4) Mughabghab S.F. and Garber D.I.: BNL 325, 3rd ed., vol.l (1973).5) Igashira M. , Kitazawa H., and Yamamuro N. : Nucl. Instr. and Meth., A245, 432

(1986).

6) Meads R.E. and Mclldowie J.E.G. "• Nucl.Phys. , 33, 502 (1962).

7) Choa C.Y. , Tollestrup A.V., Fowler W.A. and Lauritsen C.C.: Phys.Rev. , 79, 108

(1950).8) Anttia A., Keinonen J., Hautala M. and Forsbrom I.: Nucl. Instr. and Meth., 147,

501 (1977).

9) Kendrick H. and Sperling S.M.: GA-9882 (1970).

10) Macklin R.L. and Gibbons J.H.: Phys. Rev. 159, 1007 (1967).

11) K. Senoo, Y. Nagai, T. Shima, T. Ohsaki, and M. Igashira: Nucl. Instr. and Meth., A339, 556 (1994).

12) CAGSS2M: Kitazawa Laboratory, Tokyo Institute of Technology, unpublished.13) ENDF/B-V1 data file for 197Au (MAT=7925), evaluated by P. G. Young (1984).14) M. Kawai, T. Nakagawa, S. Chiba, Y. Nakajima, T. Sugi, Y. Kikuchi, T. Watanabe,

A. Zukeran, and H. Matsunobu: Proc. Int. Conf. on Nuclear Data for Science and

Technology, Gatlinburg, Tennessee, May 9-13, 1994, p.727, edited by J. K. Dickens,

American Nuclear Society, 1994.15) A. R. de L. Musgrove, B. J. Allen and J. W. Bo 1 deman, Proc. Int. Conf. on Neutron

Physics and Nuclear Data for Reactors and Other Applied Purposes, AERE Harwell,

1978, p.449.16) M. V. Bokhovko, L. E. Kazakov, V. N. Kononov, E. D. Poletaev, V. M. Timokhov, and

A. A. Voevodskiy, Yaderye Konstanty, 3 (1985) 12.17) Y. Nakajima, A. Asami, Y. Kawarasaki and Y. Furuta, Proc. Int. Conf. on Neutron

Physics and Nuclear Data for Reactors and Other Applied Purposes, AERE Harwell,

1978, p.438.

18) R. W. Hockenbury, W. R. Koste and R. A. Shaw, Bull. Am. Phys. Soc. 20 (1975) 560.

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Page 68: Measurement of nuclear reaction cross sections of rare

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