overview of fusion neutronics activities at jaeri/fns in 2004

18
Overview of Fusion Neutronics A ctivities at JAERI/FNS in 2004 Presented by T. NISHITANI Japan Atomic Energy Research Institute, Tokai-mura, 319-1195, Jap an IEA Fusion Neutronics Subtask Workshop Sala del Consiglio, the Giorgio Cini Foun dation, Venice 21th September 2004

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Overview of Fusion Neutronics Activities at JAERI/FNS in 2004. Presented by T. NISHITANI Japan Atomic Energy Research Institute, Tokai-mura, 319-1195, Japan IEA Fusion Neutronics Subtask Workshop Sala del Consiglio, the Giorgio Cini Foundation, Venice 21th September 2004. - PowerPoint PPT Presentation

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Page 1: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Overview of Fusion Neutronics Activities at JAERI/FNS in 2004

Presented by T. NISHITANI

Japan Atomic Energy Research Institute, Tokai-mura, 319-1195, Japan

IEA Fusion Neutronics Subtask Workshop Sala del Consiglio, the Giorgio Cini Foundation, Venice

21th September 2004

Page 2: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Verification of Tritium Production through Integral Experiments on the Mock-up

REALITY SIMULATION

Reactor Spectrum

Two main components:

I. High Energy 1n0 from D-T Plasma

II. Low Energy Backward Scattering 1n0

Blanket Module Blanket Mock-up

Source Spectrum

• Point D-T Source;

• Point D-T Source with a Reflector;

Bulk Beryllium Assembly

One Breeder Layer Behind the Fist Wall

Two Breeder LayersSandwiched by Be

Page 3: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Experiment Strategy for Verification of Tritium Breeding

Type Mock-up /

Neutron Spectrum

Motivation

Clean Beryllium /

D-T source

C/E ?

Neutron Transport

Design-Oriented

One Breeder Layer Behind the Fist Wall

D-T source

C/E ?

for TPR-6

One Breeder Layer Behind the First Wall

D-T source & Reflector

Impact of Neutrons from a Reflector

W & One Breeder Layer Behind the First Wall

D-T source & Reflector

Impact of Armor Layer

Two Breeder Layers Sandwiched by Beryllium

D-T source

C/E ?

for TPR-6

Page 4: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Experiment on the Bulk Beryllium Assembly

6

28 m

m

355.6 mm

1.E-27

1.E-26

1.E-25

1.E-24

0 70 140 210 280 350

Distance, mmR

ea

cti

on

ra

te, 1

/nu

cl./

s.n

.

6Li(n, )3H

32S(n,p)32P, x 103

0.8

1.0

1.2

1.4

0 70 140 210 280 350Distance, mm

Ca

lc. /

Ex

p. 6Li(n, )3H

C/E ~ 1.04

0.8

1.0

1.2

1.4

0 70 140 210 280 350Distance, mm

Ca

lc. /

Ex

p. 32S(n,p)32P

C/E ~ 1.03

Page 5: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Source Reflector, SS316

Assembly Encloser, SS316

F82H (16) / Li2TiO3 (12) / Be (200)

Experiments on the One-Breeder Layer Blanket Mock-up -- TPR-6 data --

1.E-28

1.E-27

1.E-26

0 5 10 15Distance, mm

TP

R-6

, 1/6 L

i nu

cl./

s.n

.

D-T Source

D-T Source&

Reflector

0.8

1.0

1.2

1.4

0 4 8 12Distance, mm

Ca

lc. /

Ex

p. D-T Source & Reflector

C/E ~ 1.14

0.8

1.0

1.2

1.4

0 4 8 12Distance, mm

Ca

lc. /

Ex

p. D-T Source

C/E ~ 1.02

Page 6: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Source Reflector, SS316

Assembly Encloser, SS316

W (12.6) / F82H (16) / Li2TiO3 (12) / Be (200)

Experiments on the One-Breeder Layer Blanket Mock-up with W Armor

1.E-28

1.E-27

1.E-26

0 5 10 15Distance, mm

TP

R-6

, 1/6

Li n

ucl

./s.n

. Mock-upwithout

W armor

Mock-upwith

W (12.6 mm)

0.8

1.0

1.2

1.4

0 4 8 12Distance, mm

Cal

c. /

Exp

.

C/E ~ 1.18

0.8

1.0

1.2

0 4 8 12Distance, mm

RR

rat

io

W (12.6mm) Effect on TPR-6RR Ratio ~ 0.98

Page 7: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Li2TiO3 (12) / Be (100)

Experiment on the Mock-up with Two-Breeder Layers Sandwiched by Beryllium

TP

R-6

, 1/6 L

i nu

cl./s

.n.

3.E-27

5.E-27

7.E-27

9.E-27

1.E-26

1.E-26

0 4 8 12

Distance, mm

First Layer

1.E-27

3.E-27

5.E-27

7.E-27

9.E-27

1.E-26

0 4 8 12

Distance, mm

Second Layer

0.8

1.0

1.2

1.4

0 4 8 12Distance, mm

Ca

lc. /

Ex

p. First Layer

C/E ~ 1.02

0.8

1.0

1.2

1.4

0 4 8 12Distance, mm

Ca

lc. /

Ex

p. Second Layer

C/E ~ 1.05

Page 8: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

The JAERRI/FNS activity for tritium benchmark measurement

We obtained the complete result of tritium benchmark by means of HTO sample.

690.0± 3%

69.0± 3%

13.8± 3%

330.0 ± 3%

1.505± 0.76%

18.44± 0.75%

91.4± 0.73%

1.505± 0.76%

18.52± 0.75%

91.3± 0.73

347.3± 3%

36.97± 3%

3.84± 3%

13.26± 3%

Theoretical value

Bq/g

1.01

1.01

1.01

-----

1.06

1.04

0.97

-----

-----

-----

1.00

1.00

1.00

1.00

Ratio

0.98

0.99

1.00

0.99

-----

-----

-----

1.00

1.01

1.01

1.01

1.01

1.03

1.02

Ratio

1.02

1.02

1.04

0.95

1.00

1.00

1.00

1.00

1.00

1.00

0.98

0.97

0.98

0.97

Ratio

678.0 (2.4%)

68.4 (4.3%)

13.9 (5.7%)

328.0 (3.0%)

---------

---------

---------

1.5 (3.8%)

18.7 (3.5%)

92.0 (3.4%)

352.0 (2.4%)

37.2 (4.6%)

4.0 (5.7%)

13.5 (5.2%)

TUD measurement Bq/g

(Total uncertainty %)

702.0 (1.0%)

70.4 (1.2%)

14.3 (1.4%)

315.0 (1.0%)

1.5 (9.2%)

18.6 (1.4%)

91.4 (1.2%)

1.5 (9.2%)

18.6 (1.4%)

91.4 (1.2%)

342.0 (1.5%)

35.7 (1.3%)

3.8 (4.4%)

12.8 (2.1%)

ENEA measurement Bq/g

(Total uncertainty %)

694.0 (3.3%)

70.0 (3.4%)

13.9 (3.5%)

----------

1.6 (4..3%)

19.2 (2.7%)

94.0 (2.3%)

---------

---------

---------

347.8 (3.4%)

36.84 (3.4%)

3.84 (3.4%)

13.26 (3.4%)

JAERI measurement Bq/g

(Total uncertainty %)

VKTA-A

VKTA-B

VKTA-C

VKTA-D (Blind)

TUD

ENEA02

ENEA12 (Blind)

ENEA22

ENEA04

ENEA14

ENEA24 (Blind)

ENEA

HTO-01

HTO-02

HTO-03

HTO-04 (Blind)

JAERI

HTO waterPrepared

690.0± 3%

69.0± 3%

13.8± 3%

330.0 ± 3%

1.505± 0.76%

18.44± 0.75%

91.4± 0.73%

1.505± 0.76%

18.52± 0.75%

91.3± 0.73

347.3± 3%

36.97± 3%

3.84± 3%

13.26± 3%

Theoretical value

Bq/g

1.01

1.01

1.01

-----

1.06

1.04

0.97

-----

-----

-----

1.00

1.00

1.00

1.00

Ratio

0.98

0.99

1.00

0.99

-----

-----

-----

1.00

1.01

1.01

1.01

1.01

1.03

1.02

Ratio

1.02

1.02

1.04

0.95

1.00

1.00

1.00

1.00

1.00

1.00

0.98

0.97

0.98

0.97

Ratio

678.0 (2.4%)

68.4 (4.3%)

13.9 (5.7%)

328.0 (3.0%)

---------

---------

---------

1.5 (3.8%)

18.7 (3.5%)

92.0 (3.4%)

352.0 (2.4%)

37.2 (4.6%)

4.0 (5.7%)

13.5 (5.2%)

TUD measurement Bq/g

(Total uncertainty %)

702.0 (1.0%)

70.4 (1.2%)

14.3 (1.4%)

315.0 (1.0%)

1.5 (9.2%)

18.6 (1.4%)

91.4 (1.2%)

1.5 (9.2%)

18.6 (1.4%)

91.4 (1.2%)

342.0 (1.5%)

35.7 (1.3%)

3.8 (4.4%)

12.8 (2.1%)

ENEA measurement Bq/g

(Total uncertainty %)

694.0 (3.3%)

70.0 (3.4%)

13.9 (3.5%)

----------

1.6 (4..3%)

19.2 (2.7%)

94.0 (2.3%)

---------

---------

---------

347.8 (3.4%)

36.84 (3.4%)

3.84 (3.4%)

13.26 (3.4%)

JAERI measurement Bq/g

(Total uncertainty %)

VKTA-A

VKTA-B

VKTA-C

VKTA-D (Blind)

TUD

ENEA02

ENEA12 (Blind)

ENEA22

ENEA04

ENEA14

ENEA24 (Blind)

ENEA

HTO-01

HTO-02

HTO-03

HTO-04 (Blind)

JAERI

HTO waterPrepared

Results of tritium -ray counting (Bq/g) in used HTO samples

Page 9: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

The JAERRI/FNS activity for tritium benchmark measurement

As the next step, JAERI/FNS carried out the D-T neutrons irradiation by means of the 6Li and 7Li enriched pellets.

Li2CO3 pellet( 13mm x 2mm, Li-6 : 99.7 atom%)

DT neutron1.5 x 10 11 n/sec

TiT target

FNS 80deg. Beam line

Beryllium assembly60 x 35 cm3

200 mm 102 mm

Li2CO3 pellet( 13mm x 2mm, Li-6 : 99.7 atom%)

DT neutron1.5 x 10 11 n/sec

TiT target

FNS 80deg. Beam line

Beryllium assembly60 x 35 cm3

200 mm 102 mm

5 r.p.m.

DT neutron1.5 x 10 11 n/sec

TiT targetLi2CO3 pellet

( 13mm x 2mm, Li-7:99.9 atom%)

Aluminum disk

Motor

Si detector for neutron counting

FNS 80deg. Beam line350 keV, 1mA Deuteron

Water line for cooling

5 r.p.m.

DT neutron1.5 x 10 11 n/sec

TiT targetLi2CO3 pellet

( 13mm x 2mm, Li-7:99.9 atom%)

Aluminum disk

Motor

Si detector for neutron counting

FNS 80deg. Beam line350 keV, 1mA Deuteron

Water line for cooling

We obtained preliminary results of the tritium activities (Bq/cc) in the irradiated pellets. We will discuss the results in depth within this conference term.

Schematic drawing of Li-7 enrichedLi2CO3 irradiation experiments with JAERI/FNS

Schematic drawing of Li-6 enrichedLi2CO3 irradiation experiments with JAERI/FNS

Page 10: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

FNS Rotatingtritium target(TiT target 37TBq)

D+ beam350 keV, ~20mA

Pre-collimator

Shield wall

2nd Target room

Accelarator Room

F.C.Th-232

Shield wall

Collimator assembly

1st Target room at JAERI/FNS

F.C.U-238

Experimental chamber

Step-backshielding door

Experimental movable deck

1.8 m 2.0 m

Neutron beam

Experimental chamber

Schematic view of JAERI/FNS D-T neutron beam assembly and the experimental chamber.

Differential cross section measurement of (n,CP) reactioncollaborating with Osaka University

Page 11: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Differential cross section measurement of (n,CP) reaction

We obtained the DDXs and ADXs of 9Be(n,x) and 9Be(n,t) reactions

The measured ADX of the 9Be(n,t) and and the evaluated value (ENDF-B/VI).

0

1

2

3

4

0 0.2 0.4 0.6 0.8 1

9Be(n,t)

[cosine unit]

Evaluated value

lab= 70 deg

45 deg

30 deg

15 deg

The measured ADX of the 9Be(n,x) and the evaluated nuclear data (JENDL-3.3 and ENDF-B/VI).

JENDL3.3

ENDF/B-VI

1

10

100

1000

-1 -0.5 0 0.5 1

Experiment

ADX

[mb/

sr]

Scattering angle [cos unit]

Page 12: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

In 2004, 51V(d,x) 49Cr, natFe(d,x) 55,56Co , natNi(d,x) 55Co , 60,61Cu , and 181Ta(d,x)178,180Ta cross sections have been measured.

natFe(d,x)56Co natNi(d,x)61Cu

1.0E+01

1.0E+02

1.0E+03

0 10 20 30 40 50Deuteron Energy [MeV]

Cro

ss S

ect

ion

[m

b] Present

Takacs('01)

1.0E+00

1.0E+01

1.0E+02

0 10 20 30 40 50Deuteron Energy [MeV]

Cro

ss S

ect

ion

[m

b] Present

Takacs('01)

Measurements of (d,x) reaction cross sections for IFMIF

Page 13: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Heat Load Analysis of NBI Duct

Evaluation of nuclear heating and surface heat load due to bremsstrahlung by MCNP as ITER ITA task

D-NBI duct

NBI duct

Duct wall with facing surface

Blanket

NBI duct

Blanket

Vacuum vessel

TF coil

PF coil

Cryostat

Biological shield

NBI duct

Vacuum vessel

Duct wall with hidden surface

Page 14: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Heat Load Analysis of NBI Duct

1

10

0 50 100 150 200

Facing SurfaceHidden Surface

Distance from the FW surface (cm)

1

10

0 50 100 150 200

Hidden SurfaceFacing Surface

Distance from the FW surface (cm)

Page 15: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Hydrogen Isotope Analysis of the TFTR Tile

Nuclear Reaction Analysis with below 350-keV deuteronDepth profiles of Tritium, Deuterium and Lithium

Rutherford Backscattering Spectroscopy with 350-keV deuteron Carbon density of the matrix and some high Z impurities (W etc.)

Imaging Plate methodsTritium intensity and spatial distributions in the matrix

Activation Analysis with FNS D-T neutron sourceMedium Z metals (Fe, Ni, Co etc.)

Gas flow methodThe number of tritium and carbon-14

Our main objectives is to measure the tritium retention on the TFTR-PFM

In 1993, the TFTR had the series of the D-T discharge experiments.The absolute measurement of tritium depth profile in the order of m on the surface of the plasma facing material (4D-CFC) has been left.

Page 16: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Tritium Depth Profile on the Surface of the TFTR tile

T-Retention7.2 x 1015 T/cm2 (up to 1.2m)

NE213

JAERI/FNS80deg. LineD+, 1A150~380 keV

SSD

We mainly observed charged particles induced with T-d, D-d, 6Li-d and 7Li-d reactions by means of nuclear reaction analysis.

Schematic view of the FNS-NRA system

1.0E+00

1.0E+01

1.0E+02

1.0E+03

1.0E+04

1.0E+05

0 3 6 9 12

Energy MeV

Cou

nts

/Ch

ann

el/m

C

6Li(d,2)

D(d,p)TT(d,n)

7Li(d,2n)

3.0E+19

6.0E+19

9.0E+19

1.2E+20

-0.2 0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4

Depth (m)

Tri

tium

den

sity

(c

m-3

)

Tritium profile on the surface, Activity=12.9 MBq/cm2. Density peak 1 x 1020cm-3 at near 0.5 m depth.

Page 17: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Tritium Depth Profile on the Surface of the TFTR tile

3.0E+19

6.0E+19

9.0E+19

1.2E+20

-0.2 0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4

Depth (m)

Tri

tium

den

sity

(c

m-3

)

T-Retention7.2 x 1015 T/cm2 (up to 1.2m)

Tritium profile on the surface, Activity=12.9 MBq/cm2. Density peak 1 x 1020cm-3 at near 0.5 m depth.

We mainly observed charged particles induced with T-d, D-d, 6Li-d and 7Li-d reactions by means of nuclear reaction analysis.

NE213

JAERI/FNS80deg. LineD+, 1A150~380 keV

SSD

Schematic view of the FNS-NRA system

A piece at the corner of block in KC-16 was sampled

Page 18: Overview of Fusion Neutronics Activities at JAERI/FNS  in 2004

Plan in 2004-2005

Integral Study on Structural/Blanket Materials Benchmark experiment for the blanket assembly with pebbles Benchmark experiment for the blanket assembly with the coolant panel.

Low Activation Materials Induced Radioactivity Experiments Charged particle production cross section measurement for 6Li and 7Li. Activation cross section measurement of (d,X) reactions for IFMIF ma

terials,Ta, Fe, Ni and V, in the energy range of 20-35 MeV. Others

ITER-ITA task : Nuclear heat analyses for NB and DNB ports. Neutron Elastic Scattering Analysis of D and T in TFTR and JT-60 car

bon tiles.