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Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

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Page 1: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Projected-shell-model study for the structure oftransfermium nuclei

Yang SunShanghai Jiao Tong University

Beijing, June 9, 2009

Page 2: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

The island of stability

What are the next magic numbers, i.e. most stable nuclei? Predicted neutron magic number: 184 Predicted proton magic number: 114, 120, 126

Page 3: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Approaching the superheavy island

Single particle states in SHE Important for locating the island Little experimental information available

Indirect ways to find information on single particle states Study quasiparticle K-isomers in very heavy nuclei Study rotation alignment of yrast states in very heavy nuclei

Deformation effects, collective motions in very heavy nuclei

gamma-vibration Octupole effect

Page 4: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Single-particle states

R. Chasmanet al., Rev. Mod. Phys. 49, 833 (1977)R. Chasmanet al., Rev. Mod. Phys. 49, 833 (1977)

neutronsprotons

Page 5: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Nuclear structure models

Shell-model diagonalization method Most fundamental, quantum mechanical Growing computer power helps extending applications A single configuration contains no physics Huge basis dimension required, severe limit in applications

Mean-field method Applicable to any size of systems Fruitful physics around minima of energy surfaces No configuration mixing States with broken symmetry, cannot be used to calculate

electromagnetic transitions and decay rates

Page 6: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Bridge between shell-model and mean-field method

Projected shell model Use more physical states (e.g. solutions of a deformed mean-

field) and angular momentum projection technique to build shell model basis

Perform configuration mixing (a shell-model concept) • K. Hara, Y. Sun, Int. J. Mod. Phys. E 4 (1995) 637

The method works in between conventional shell model and mean field method, hopefully take the advantages of both

Page 7: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

The projected shell model

Shell model based on deformed basis

Take a set of deformed (quasi)particle states (e.g. solutions of HFB, HF + BCS, or Nilsson + BCS)

Select configurations (deformed qp vacuum + multi-qp states near the Fermi level)

Project them onto good angular momentum (if necessary, also particle number, parity) to form a basis in lab frame

Diagonalize a two-body Hamiltonian in projected basis

Page 8: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Model space constructed by angular-momentum projected states

Wavefunction:

with a.-m.-projector:

Eigenvalue equation:

with matrix elements:

Hamiltonian is diagonalized in the projected basis

IM K

IM Pf

DDdI

P IM K

IM K

28

12

0''

''

fENH II

'''''' I

KK

II

KK

I PNPHH

IM KP

Page 9: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Hamiltonian and single particle space

The Hamiltonian Interaction strengths

is related to deformation by

GM is fitted by reproducing moments of inertia

GQ is assumed to be proportional to GM with a ratio ~ 0.15

Single particle space Three major shells for neutrons or protons

For very heavy nuclei, N = 5, 6, 7 for neutrons

N = 4, 5, 6 for protons

PPGPPGQQHH QM

20

ppnn QQ 00

3/2

Page 10: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Building blocks: a.-m.-projected multi-quasi-particle states

Even-even nuclei:

Odd-odd nuclei:

Odd-neutron nuclei:

Odd-proton nuclei:

,0ˆ,0ˆ,0ˆ,0ˆ I

MKIMK

IMK

IMK PPPP

,0ˆ,0ˆ,0ˆ,0ˆ I

MKIMK

IMK

IMK PPPP

,0ˆ,0ˆ,0ˆ I

MKIMK

IMK PPP

,0ˆ,0ˆ,0ˆ I

MKIMK

IMK PPP

Page 11: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Recent developments in PSM

Separately project n and p systems for scissors mode Sun, Wu, Bhatt, Guidry, Nucl. Phys. A 703 (2002) 130

Enrich PSM qp-vacuum by adding collective d-pairs Sun and Wu, Phys. Rev. C 68 (2003) 024315

PSM Calculation for Gamow-Teller transition Gao, Sun, Chen, Phys. Rev, C 74 (2006) 054303

Multi-qp triaxial PSM for -deformed high-spin states Gao, Chen, Sun, Phys. Lett. B 634 (2006) 195 Sheikh, Bhat, Sun, Vakil, Palit, Phys. Rev. C 77 (2008) 034313

Breaking Y3 symmetry + parity projection for octupole band Chen, Sun, Gao, Phys. Rev, C 77 (2008) 061305

Real 4-qp states in PSM basis (from same or diff. N shell) Chen, Zhou, Sun, to be published

Page 12: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Very heavy nuclei: general features

Potential energy calculation shows deep prolate minimum A very good rotor, quadrupole + pairing interaction dominant Low-spin rotational feature of even-even nuclei can be well

described (relativistic mean field, Skyrme HF, …)

Page 13: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Yrast line in very heavy nuclei

No useful information can be extracted from low-spin g-band (rigid rotor behavior)

First band-crossing occurs at high-spins (I = 22 – 26)

Transitions are sensitive to the structure of the crossing bands

g-factor varies very much due to the dominant proton or neutron contribution

Page 14: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Band crossings of 2-qp high-j states

Strong competition between 2-qp i13/2 and 2qp j15/2 band crossings (e.g. in N=154 isotones)

Al-Khudair, Long, Sun, Phys. Rev. C 79 (2009) 034320

Page 15: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

MoI, B(E2), g-factor in Cf isotopes

-crossingdominant

-crossingdominant

-crossingdominant

-crossingdominant

Page 16: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

MoI, B(E2), g-factor in Fm isotopes

-crossingdominant

-crossingdominant

Page 17: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

MoI, B(E2), g-factor in No isotopes

-crossingdominant

-crossingdominant

-crossingdominant

Page 18: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

K-isomers in superheavy nuclei

K-isomer contains important information on single quasi-particles

e.g. for the proton 2f7/2–2f5/2 spin–orbit partners, strength of the spin–orbit interaction determines the size of the Z=114 gap

Information on the position of 1/2[521] is useful Herzberg et al., Nature 442 (2006) 896

K-isomer in superheavy nuclei may lead to increased survival probabilities of these nuclei

Xu et al., Phys. Rev. Lett. 92 (2004) 252501

Page 19: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Enhancement of stability in SHE by isomers

Occurrence of multi-quasiparticle isomeric states decreases the probability for both fission and decay, resulting in enhanced stability in superheavy nuclei.

Page 20: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

K-isomers in 254No

The lowest k = 8- isomeric band in 254No is expected at 1–1.5 MeV

Ghiorso et al., Phys. Rev. C7 (1973) 2032

Butler et al., Phys. Rev. Lett. 89 (2002) 202501

Recent experiments confirmed two isomers: T1/2 = 266 ± 2 ms and 184 ± 3 μs

Herzberg et al., Nature 442 (2006) 896

Page 21: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

What do we need for K-isomer description?

K-mixing – It is preferable to construct basis states with good angular momentum I and

parity , classified by K to mix these K-states by residual interactions at given I and to use resulting wavefunctions to calculate electromagnetic

transitions in shell-model framework

A projected intrinsic state can be labeled by K With axial symmetry: carries K

defines a rotational band associated with the intrinsic K-state

Diagonalization = mixing of various K-states

IMKP̂

III NHE /

Page 22: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

K-isomers in 254No - interpretation

Page 23: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Projected shell model calculation

A high-K band with K = 8- starts at ~1.3 MeV

A neutron 2-qp state:

(7/2+ [613] + 9/2- [734])

A high-K band with K = 16+ at 2.7 MeV

A 4-qp state coupled by two neutrons and two protons:

(7/2+ [613] + 9/2- [734]) +

(7/2- [514] + 9/2+ [624])

Herzberg et al., Nature 442 (2006) 896

Page 24: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Prediction: K-isomers in No chain

Positions of the isomeric states depend on the single particle states

Nilsson states used:

T. Bengtsson, I. Ragnarsson, Nucl. Phys. A 436 (1985) 14

Page 25: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Predicted K-isomers in 276SgPredicted K-isomers in 276Sg

Page 26: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

A superheavy rotor can vibrate

Take triaxiality as a parameter in the deformed basis and do 3-dim. angular-momentum-projection

Microscopic version of the -deformed rotor of

Davydov and Filippov, Nucl. Phys. 8 (1958) 237

’~0.1 (~22o)

Data: Hall et al., Phys. Rev. C39 (1989) 1866

Page 27: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

-vibration in very heavy nuclei

Prediction: -vibrations (bandhead below 1MeV) Low 2+ band cannot be explained by qp excitations

Sun, Long, Al-Khudair, Sheikh, Phys. Rev. C 77 (2008) 044307

Page 28: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Multi-phonon -bands

Multi-phonon -vibrational bands were predicted for rear earth nuclei

Classified by K = 0, 2, 4, … Y. Sun et al, Phys. Rev. C61

(2000) 064323

Multi-phonon -bands also predicted to exist in the heaviest nuclei

Show strong anharmonicity

Page 29: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Bands in odd-proton 249Bk

Nilsson parameters of T. Bengtsson-Ragnarsson

Slightly modifiedNilsson parameters

Ahmad et al., Phys. Rev. C71 (2005) 054305

Page 30: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Bands in odd-proton 249Bk

Page 31: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Nature of low-lying excited states

N = 150 Neutron states

N = 152 Proton states

Page 32: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Octupole correlation: Y30 vs Y32

Strong octupole effect known in the actinide region (mainly Y30 type: parity doublet band)

As mass number increases, starting from Cm-Cf-Fm-No, 2- band is lower

Y32 correlation may be important

Page 33: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Triaxial-octupole shape in superheavy nuclei

Proton Nilsson Parameters of T. Bengtsson and Ragnarsson

i13/2 (l = 6, j = 13/2), f7/2 (l = 3, j = 7/2) degenerate at the spherical limit

{[633]7/2; [521]3/2}, {[624]9/2; [512]5/2} satisfy l=j=3,K=2

Gap at Z=98, 106

Page 34: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Yrast and 2- bands in N=150 nuclei

Chen, Sun, Gao, Phys. Rev. C 77 (2008) 061305

Page 35: Projected-shell-model study for the structure of transfermium nuclei Yang Sun Shanghai Jiao Tong University Beijing, June 9, 2009

Summary

Study of structure of very heavy nuclei can help to get information about single-particle states.

The standard Nilsson s.p. energies (and W.S.) are probably a good starting point, subject to some modifications.

Testing quantities (experimental accessible) Yrast states just after first band crossing Quasiparticle K-isomers Excited band structure of odd-mass nuclei

Low-lying collective states (experimental accessible) -band Triaxial octupole band