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Science and Techniques of Ultra- Fast Electron and Photon Sources ... ... the laser-driven approach Stefan Karsch MPI for Quantum Optics & LMU Munich Hans-Kopfermann-Straße 1 D-85748 Garching PAC 09, Vancouver, May 8, 2009

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Page 1: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Science and Techniques of Ultra-Fast Electron and Photon Sources ...

... the laser-driven approach

Stefan Karsch

MPI for Quantum Optics & LMU MunichHans-Kopfermann-Straße 1

D-85748 Garching

PAC 09, Vancouver, May 8, 2009

Page 2: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

- Attosecond sources - state of the art- Detour - ultra-high intensity lasers- New approaches to high-intensity

few-femtosecond and attosecond sources

➡ relativistic high-harmonic generation➡ ultrashort electron beams➡ undulator and FEL radiation

OUTLINE

Page 3: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Standard technology limits for XUV intensity

Nonlinear self-phase modulation in noble gas

below ionization threshold

20 fs, mJ 40 fs, 100‘s µJ

Broadband compression using chirped mirrors

5 fs, 100‘s µJ

attosecond production by recollission in noble gas at

ionization threshold

100 as, 104-105 photons

Limited per-shot photon numberHigh repetition rate necessary,

scanning techniques

Page 4: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

6565

7575

8585

elec

tron

kin

etic

ene

rgy

[eV]

elec

tron

kin

etic

ene

rgy

[eV]

delay [fs]delay [fs] 00 44-4-4 88

E. Goulielmakis et al, Science 305, 1267 (2004)

experimental evidence for the existence of a single sub-femtosecond xuv pulse and for the sampling of light waves in real time

Page 5: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Freezing of atomic motion by short exposure timeFreezing of atomic motion by short exposure time↓↓

XFEL pulses with 10XFEL pulses with 101212 photonsphotons in <10 fs are highly desirablein <10 fs are highly desirable

Single Molecule imaging:Coulomb explosion of a protein moleculeLysozyme with 137 structural waters

Neutze, R., Wouts, R., van der Spoel, D., Weckert, E. Hajdu, J., Nature 406, 752 (2000)

t =20fst =-2fs t =2fs t =5fs t =10fs t =50fs

Page 6: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

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benötigt.

Zur Anzeige wird der QuickTime™ Dekompressor „“

benötigt.

Zur Anzeige wird der QuickTime™ Dekompressor „“

benötigt.

Zur Anzeige wird der QuickTime™ Dekompressor „“

benötigt.

steering bound electrons with controlled light fields: the birth of an attosecond pulse

3D-solution of the Schrödinger equation for hydrogen: Armin Scrinzi animation: Barbara Ferus, Matthias Uiberacker

Page 7: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

electrons released and returning within the central wave cycle of a near-single-cycle light wave recollide with highest energy and produce an

isolated sub-fs pulse at the highest photon energies emitted

Page 8: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

00

momentum change∆p along the EL vectormomentum change∆p along the EL vector

-500 as-500 as 00 500 as500 as

laser electric field, EL(t)laser electric field, EL(t)

t7t7t2t2 t3t3 t4t4 t5t5 t6t6

Drescher et al, Science 291, 1923 (2001)J. Itatani et al, PRL 88, 173903 (2002)

M. Kitzler et al, PRL 88, 173904 (2002)

electron release timeelectron release time

incident x-rayintensity

electronmomentumdistribution

optical-field-driven streak camera optical-field-driven streak camera

t1t1

steering freed electrons with controlled light fields: the measurement of an attosecond

pulse

Page 9: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

00

momentum changealong the EL vectormomentum changealong the EL vector

-500 as-500 as 00 500 as500 asDrescher et al, Science 291, 1923 (2001)

J. Itatani et al, PRL 88, 173903 (2002)M. Kitzler et al, PRL 88, 173904 (2002)

electron release timeelectron release time

optical-field-driven streak camera optical-field-driven streak camera

steering freed electrons with controlled light fields: the measurement of an attosecond

pulse

electronmomentumdistribution

electronmomentumdistribution

incident x-rayintensity

laser electric field, EL(t)laser electric field, EL(t)

Page 10: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

00

momentum changealong the EL vectormomentum changealong the EL vector

-500 as-500 as 00 500 as500 as electron release timeelectron release time

optical-field-driven streak camera optical-field-driven streak camera

steering freed electrons with controlled light fields: the measurement of an attosecond

pulse

laser electric field, EL(t)laser electric field, EL(t)

Drescher et al, Science 291, 1923 (2001)J. Itatani et al, PRL 88, 173903 (2002)

M. Kitzler et al, PRL 88, 173904 (2002)

Page 11: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Q-switching

modelocking

chirped pulse amplification

classical plasma physics

relativistic optics

relativistic ions

nonlinear damage

nonlinear QED

historical development of delivered laser intensities

Necessary laser power:

Focusing to 3 µm x 3 µm: P = 1 PW for 1022 W/cm2

Page 12: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Images: NASA/Apollo 17MPI f. Astronomie

How to generate 1022 W/cm2

r=re=6371 km

solar constant: 1367 W/m2

total radiation power hitting the earth: 1.7x1017 W

⇒ focused to 50µm ∅: I =1022 W/cm2

lens: focal length 17 mm, diameter=12700 km...

Page 13: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

or: using lasers

focusability of coherent light:

w = 1.22 λ F

f

D F = f/D = O(1..10)

λ = 0.8 µmw ≈ 3 µm = 10-7 cm2

for 1022 W/cm2 one needs 1015 W = 1PW!

Page 14: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

picture: AP

1 PW?

........106 x

Atomic power plant: 109 W

1 PW continuously is obviously

hard to realize...

pulsed laser: expensiveexpensive

limited by laser materiallimited by laser material

Page 15: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Our Laser Suite

ATLAS Ti:Sa laser30-100 TW

20-35 fs5-10 Hz

etawatt Field Synthesizer (PFS)OPCPA system

5 fs, >500 TW1-10 Hz

LWS-20 OPCPA system20 TW7-8 fs10 Hz

Page 16: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

EL > 1014 V/mBL > 106 T

L=2.7 fsL = 2.35 PHz

Strength of light fields

energy flux (Poynting vector)

Intensity

Page 17: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Interaction with matter

classical velocity of an electron after half a laser periodrelativistic effects have to be taken into account when the energy gain in a half period equals its rest mass: i.e. when dimensionless amplitude a0≥1,

above 1018 W/cm2 for 1µm light

Equation of motion for an electron in a plane, monochromatic light

wave

Potential difference across an atom: 1 Å Matter is instantly ionized!

Page 18: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

solid target In filter

ATLAS:45 fs

800 nm25 TW

parabola

Si wafers

split mirror

He gas jet

time-of-flight spectrometer

coarse scan

fine scan

2.0

1.5

1.0

0.5

0.0-100 -50 0 50 100

delay [fs]

ion

sign

al [a

rb. u

nits

]

2.5

1.5

1.0

0.5

0.0

ion

sign

al [a

rb. u

nits

] 2.0

-4 -2 0 2 4delay [fs]

Y. Nomura, R. Hörlein, S. Rykovanov, Zs. Major, J. Osterhoff, S. Karsch, L. Veisz, G. D. Tsakiris– in collaboration with D. Droomey, M. Zepf, P. Tzallas, D. Charalambidis

Y. Nomura, R. Hörlein, S. Rykovanov, Zs. Major, J. Osterhoff, S. Karsch, L. Veisz, G. D. Tsakiris– in collaboration with D. Droomey, M. Zepf, P. Tzallas, D. Charalambidis

harmonics emitted from a relativistic interaction are phased yielding a train of sub-fsec pulses of XUV light

harmonics emitted from a relativistic interaction are phased yielding a train of sub-fsec pulses of XUV light

Attosecond autocorrelation of XUV pulse train by 2-photon ionization of helium

Page 19: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

after a long, hard journey...

A. Modena et al., Nature 377, 606 (1995): (self-modulated wakefield)

from long laser pulses....

...to shorter ones...

Mangles et al., Geddes et al., Faure et al. Nature 2004

...where the laser pulses are much shorter than the plasma period

Page 20: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

courtesy L. Veisz

Basic mechanism

Page 21: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

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Acceleration gradients scale as ne1/2 ⇒ higher density preferrableHowever:

speed of light in plasma decreases for higher density ⇒ electrons and drive pulse dephase

Page 22: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Single shotsSingle shots Summed shotsSummed shots

Lase

r pol

ariz

atio

n ax

isLa

ser p

olar

izat

ion

axis

1.1 m behind electron source1.1 m behind electron source

2 cm2 cm

2 cm2 cm

Divergence, beam pointing stabilityDivergence, beam pointing stabilityDivergence, beam pointing stability

2 cm2 cm

2 cm2 cm

Pointing stability in x-direction 2.2 mrad RMS

y-direction 1.4 mrad RMS

Pointing stability in x-direction 2.2 mrad RMS

y-direction 1.4 mrad RMS

averaged over 100 shots

averaged over 100 shots

xx

yy yy

xx

Page 23: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

towards applications - beam transport: Focusing with mini-quadrupole lenses

field gradient: 500 T/m

sourcedipole

mini quadrupole doublet

Lanex

with F. Grüner, M. Fuchs, R. Weingartner, S. Becker,

U.Schramm

Lenses• focus the beam• improve spectrometer resolution• strongly reduce pointing

fluctuations

Page 24: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Real energy spread

Screen 2

→ Essential property forfuture table-top FEL operation

1.1% peak energy fluctuation !

E ≈ 169.7 ± 2.0 MeV

150 MeV

175 MeV

Ene

rgy

1 2 3 4 5 6 7 8Shots

ΔE/E ≈ 1.76±0.26% RMS

See also:LOA: C. Rechatin et al., PRL 102, 164801 (2009): 3.1 % RMS spread

Nebraska: S. Banerjee et al., 0.8 % energy spread

Source size image: provides emittance measurement,

given the resolution can be improved

Page 25: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Stability and control by external injectionJ. Faure et al, Nature 444, 737 (2006)

Page 26: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

A two-screen spectrometer unambiguously measures the energy and deflection of the electron beams

Courtesy: D. Froula, LLNL

Page 27: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Laser wakefield acceleration in the matched parameter regime

University of Nebraska• Guiding: only relativistic (no

pre-formed channel)• 1-10 mm He supersonic jet• Laser parameters (intensity,

pulse duration, focal spot-size) all matched with plasma

Electron Beam MeasurementEnergy 50-600 MeVΔE/E 10%Charge per bunch 100-600 pCDivergence angle 2-5 mradPointing & energy stability 1% (>30 shots)

Laser Parameter MeasurementPeak power < 140 TWRepetition rate 10 HzCentral wavelength 805 nmPulse duration < 30 fsPulse energy 3.5 JEnergy stability 0.8% rmsStrehl ratio 0.95Pointing stability 3.5 μrad

Courtesy: S. Banerjee, UNL

Page 28: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central
Page 29: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

→ Pulse-front tilted beams drive asymmetric wakes

Page 30: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Pulse duration?

1st measurement: Tilborg et al. PRL 96 014801 (2006)

EO sampling, t < 50 fs RMS, limited by detection system resolution

Page 31: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

ENLITE 2009, Dresden Alexander Debus April 2nd 2009

Simulated vs. measured cross-correlator signal• Delay between electron

bunch distributions

= 370

• Long bunch @ FWHM

long = 650 ± 25 fs

• Short bunch @ FWHM

short = 49

• Laser probe distance from axis is compatible with

doff-axis = 600 ± 25 µmt [ps]

822

fs+-

510

fs+-

norm

. cro

ss-c

orre

lato

r int

ensi

tySingle shot EO measurement, RAL ASTRA

Courtesy: A. Debus, FZD

Page 32: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Courtesy: S. Wesch, DESY

Page 33: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Courtesy: S.F. Martins, IST& UCL

Page 34: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

X-ray generation: Undulator radiation towards FEL

Page 35: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

as-HHG seed

Laser-driven FEL amplifier

ultra-compact as-X-ray FEL

Future dreams:

Page 36: Science and Techniques of Ultra- Fast Electron and Photon … · 2010. 12. 4. · animation: Barbara Ferus, Matthias Uiberacker . electrons released and returning within the central

Coworkers

D.Habs group (LMU)G. Tsakiris group (MPQ)S.Hooker group (Oxford)L.O‘Silva group (Lisbon)

J. Hein (Jena)

Main collaborators: