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Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy Elements at the S3-LEB Rafael Ferrer KU Leuven, Instituut voor Kern- en Stralingsfysica Belgium

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Page 1: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy

Elements at the S3-LEB

Rafael FerrerKU Leuven Instituut voor Kern- en Stralingsfysica

Belgium

Outline

bull Motivation for Laser Spectroscopy of Heavy Elements

bull The In-Gas Laser Ionization and Spectroscopy (IGLIS) technique

Off-line characterization studies

bull IGLIS studies of exotic nuclei at S3-LEB (GANIL)

bull Summary amp Outlook

2R Ferrer NuSPRASEN 2019

3

Optical Spectroscopy Actinides Status

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

Important nuclear ground- and isomeric-state properties to understand underlying nuclear structure and improve predictive power of nuclear theories

Deduced observables dltr2gt m Q I

(model independent)

Shapedeform ParametersSinglefew particle config

R Ferrer NuSPRASEN 2019

4

Optical Spectroscopy Actinides Challenges

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

Laser spectroscopy after fusion evaporation reactions

Low production rates of actinides impose highly sensitive and efficient laser spectroscopy technique

amp High spectral resolution to resolve hyperfine structure

R Ferrer NuSPRASEN 2019

5

In Gas Laser Ionization and Spectroscopy (IGLIS)

spectrometerHI beam

gas cell

CD nozzle RFQ ion guide

detectorstation

-40 -20 0 20 400

100

200

300

gas cell

gas jet

c

ou

nts

in 5

0 s

Detuning (GHz)

215Ac (T

12= 170 ms)

R F et al Nat Commun 8 (2017) 14520

In-Cell vs In-Jet Spectroscopy

ejet~eGC

R Ferrer NuSPRASEN 2019

6

Performance of IGLIS on Actinides

Characterizationoptimization offline IGLIS laboratory

R F et al Nat Commun 8 (2017) 14520 Y Kudryavtsev et al NIM B297 (2013) 7S Raeder et al NIM B 376 (2016) 382

bull collisions Δϑρ~T119895119890119905

T293K

03lowast ρjet

bull temperature Δ120599Doppler~1205990 Τ119879119895119890119905

119860

jet

in cell

in jet

R Ferrer NuSPRASEN 2019

7

IGLIS laboratory KU Leuven (off-line studies)

- High power high rep laser system

- New gas cell design

- RFQ Ion Guides

Jet properties with CD nozzles

R Ferrer NuSPRASEN 2019

50 mm

119875119887119892 ge 119875119895119890119905ICCD camera

Jet visualization the PLIF technique

laser

8

bull Information on velocity temperature and density distributions in the gas jet

Freqshift vFWHM TAmp rel density

63Cu

laser

Gas cell

Gas jet

laser

R Ferrer NuSPRASEN 2019

Central jet line Pbg asymp Popt

P0 = 380 mbar Pbg = 15 mbarQuasi-uniform jet

Characterization of jets formed by de Laval nozzles

L

9A Zadvornaya et al Phys Rev X 8 041008 (2018)R Ferrer NuSPRASEN 2019

Qu

asi-u

niform

je

t

CFD Module

PLIF

T0 = 500 K P0 = 379 mbar Pbg = 146 mbar

FWHM

Doppler shift

Characterization of jets formed by de Laval nozzles II

10A Zadvornaya et al Phys Rev X 8 041008 (2018)

Density

R Ferrer NuSPRASEN 2019

11

Nozzle (Mgt 5)

Characterization of the flow parameters by PLIFS and RIS and comparison with results from simulations

bull precision inner contour ~ 5 mmbull surface finishing Ra=01 mm

Shortcomings

bull Calculations considering inviscid flow software limitations

bull Precise (CNC) machining inner contour and surface finishing

New nozzle contour using advanced simulation code from Aeronautics and Aerospace Department (von Karman Institute for Fluid Dynamics)

Radia

l dis

tan

ce (

mm

)

Distance from nozzle throat (mm)

R Ferrer NuSPRASEN 2019

12

Characterization of jets by RIS

R Ferrer NuSPRASEN 2019

13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 2: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

Outline

bull Motivation for Laser Spectroscopy of Heavy Elements

bull The In-Gas Laser Ionization and Spectroscopy (IGLIS) technique

Off-line characterization studies

bull IGLIS studies of exotic nuclei at S3-LEB (GANIL)

bull Summary amp Outlook

2R Ferrer NuSPRASEN 2019

3

Optical Spectroscopy Actinides Status

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

Important nuclear ground- and isomeric-state properties to understand underlying nuclear structure and improve predictive power of nuclear theories

Deduced observables dltr2gt m Q I

(model independent)

Shapedeform ParametersSinglefew particle config

R Ferrer NuSPRASEN 2019

4

Optical Spectroscopy Actinides Challenges

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

Laser spectroscopy after fusion evaporation reactions

Low production rates of actinides impose highly sensitive and efficient laser spectroscopy technique

amp High spectral resolution to resolve hyperfine structure

R Ferrer NuSPRASEN 2019

5

In Gas Laser Ionization and Spectroscopy (IGLIS)

spectrometerHI beam

gas cell

CD nozzle RFQ ion guide

detectorstation

-40 -20 0 20 400

100

200

300

gas cell

gas jet

c

ou

nts

in 5

0 s

Detuning (GHz)

215Ac (T

12= 170 ms)

R F et al Nat Commun 8 (2017) 14520

In-Cell vs In-Jet Spectroscopy

ejet~eGC

R Ferrer NuSPRASEN 2019

6

Performance of IGLIS on Actinides

Characterizationoptimization offline IGLIS laboratory

R F et al Nat Commun 8 (2017) 14520 Y Kudryavtsev et al NIM B297 (2013) 7S Raeder et al NIM B 376 (2016) 382

bull collisions Δϑρ~T119895119890119905

T293K

03lowast ρjet

bull temperature Δ120599Doppler~1205990 Τ119879119895119890119905

119860

jet

in cell

in jet

R Ferrer NuSPRASEN 2019

7

IGLIS laboratory KU Leuven (off-line studies)

- High power high rep laser system

- New gas cell design

- RFQ Ion Guides

Jet properties with CD nozzles

R Ferrer NuSPRASEN 2019

50 mm

119875119887119892 ge 119875119895119890119905ICCD camera

Jet visualization the PLIF technique

laser

8

bull Information on velocity temperature and density distributions in the gas jet

Freqshift vFWHM TAmp rel density

63Cu

laser

Gas cell

Gas jet

laser

R Ferrer NuSPRASEN 2019

Central jet line Pbg asymp Popt

P0 = 380 mbar Pbg = 15 mbarQuasi-uniform jet

Characterization of jets formed by de Laval nozzles

L

9A Zadvornaya et al Phys Rev X 8 041008 (2018)R Ferrer NuSPRASEN 2019

Qu

asi-u

niform

je

t

CFD Module

PLIF

T0 = 500 K P0 = 379 mbar Pbg = 146 mbar

FWHM

Doppler shift

Characterization of jets formed by de Laval nozzles II

10A Zadvornaya et al Phys Rev X 8 041008 (2018)

Density

R Ferrer NuSPRASEN 2019

11

Nozzle (Mgt 5)

Characterization of the flow parameters by PLIFS and RIS and comparison with results from simulations

bull precision inner contour ~ 5 mmbull surface finishing Ra=01 mm

Shortcomings

bull Calculations considering inviscid flow software limitations

bull Precise (CNC) machining inner contour and surface finishing

New nozzle contour using advanced simulation code from Aeronautics and Aerospace Department (von Karman Institute for Fluid Dynamics)

Radia

l dis

tan

ce (

mm

)

Distance from nozzle throat (mm)

R Ferrer NuSPRASEN 2019

12

Characterization of jets by RIS

R Ferrer NuSPRASEN 2019

13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 3: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

3

Optical Spectroscopy Actinides Status

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

Important nuclear ground- and isomeric-state properties to understand underlying nuclear structure and improve predictive power of nuclear theories

Deduced observables dltr2gt m Q I

(model independent)

Shapedeform ParametersSinglefew particle config

R Ferrer NuSPRASEN 2019

4

Optical Spectroscopy Actinides Challenges

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

Laser spectroscopy after fusion evaporation reactions

Low production rates of actinides impose highly sensitive and efficient laser spectroscopy technique

amp High spectral resolution to resolve hyperfine structure

R Ferrer NuSPRASEN 2019

5

In Gas Laser Ionization and Spectroscopy (IGLIS)

spectrometerHI beam

gas cell

CD nozzle RFQ ion guide

detectorstation

-40 -20 0 20 400

100

200

300

gas cell

gas jet

c

ou

nts

in 5

0 s

Detuning (GHz)

215Ac (T

12= 170 ms)

R F et al Nat Commun 8 (2017) 14520

In-Cell vs In-Jet Spectroscopy

ejet~eGC

R Ferrer NuSPRASEN 2019

6

Performance of IGLIS on Actinides

Characterizationoptimization offline IGLIS laboratory

R F et al Nat Commun 8 (2017) 14520 Y Kudryavtsev et al NIM B297 (2013) 7S Raeder et al NIM B 376 (2016) 382

bull collisions Δϑρ~T119895119890119905

T293K

03lowast ρjet

bull temperature Δ120599Doppler~1205990 Τ119879119895119890119905

119860

jet

in cell

in jet

R Ferrer NuSPRASEN 2019

7

IGLIS laboratory KU Leuven (off-line studies)

- High power high rep laser system

- New gas cell design

- RFQ Ion Guides

Jet properties with CD nozzles

R Ferrer NuSPRASEN 2019

50 mm

119875119887119892 ge 119875119895119890119905ICCD camera

Jet visualization the PLIF technique

laser

8

bull Information on velocity temperature and density distributions in the gas jet

Freqshift vFWHM TAmp rel density

63Cu

laser

Gas cell

Gas jet

laser

R Ferrer NuSPRASEN 2019

Central jet line Pbg asymp Popt

P0 = 380 mbar Pbg = 15 mbarQuasi-uniform jet

Characterization of jets formed by de Laval nozzles

L

9A Zadvornaya et al Phys Rev X 8 041008 (2018)R Ferrer NuSPRASEN 2019

Qu

asi-u

niform

je

t

CFD Module

PLIF

T0 = 500 K P0 = 379 mbar Pbg = 146 mbar

FWHM

Doppler shift

Characterization of jets formed by de Laval nozzles II

10A Zadvornaya et al Phys Rev X 8 041008 (2018)

Density

R Ferrer NuSPRASEN 2019

11

Nozzle (Mgt 5)

Characterization of the flow parameters by PLIFS and RIS and comparison with results from simulations

bull precision inner contour ~ 5 mmbull surface finishing Ra=01 mm

Shortcomings

bull Calculations considering inviscid flow software limitations

bull Precise (CNC) machining inner contour and surface finishing

New nozzle contour using advanced simulation code from Aeronautics and Aerospace Department (von Karman Institute for Fluid Dynamics)

Radia

l dis

tan

ce (

mm

)

Distance from nozzle throat (mm)

R Ferrer NuSPRASEN 2019

12

Characterization of jets by RIS

R Ferrer NuSPRASEN 2019

13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 4: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

4

Optical Spectroscopy Actinides Challenges

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

Laser spectroscopy after fusion evaporation reactions

Low production rates of actinides impose highly sensitive and efficient laser spectroscopy technique

amp High spectral resolution to resolve hyperfine structure

R Ferrer NuSPRASEN 2019

5

In Gas Laser Ionization and Spectroscopy (IGLIS)

spectrometerHI beam

gas cell

CD nozzle RFQ ion guide

detectorstation

-40 -20 0 20 400

100

200

300

gas cell

gas jet

c

ou

nts

in 5

0 s

Detuning (GHz)

215Ac (T

12= 170 ms)

R F et al Nat Commun 8 (2017) 14520

In-Cell vs In-Jet Spectroscopy

ejet~eGC

R Ferrer NuSPRASEN 2019

6

Performance of IGLIS on Actinides

Characterizationoptimization offline IGLIS laboratory

R F et al Nat Commun 8 (2017) 14520 Y Kudryavtsev et al NIM B297 (2013) 7S Raeder et al NIM B 376 (2016) 382

bull collisions Δϑρ~T119895119890119905

T293K

03lowast ρjet

bull temperature Δ120599Doppler~1205990 Τ119879119895119890119905

119860

jet

in cell

in jet

R Ferrer NuSPRASEN 2019

7

IGLIS laboratory KU Leuven (off-line studies)

- High power high rep laser system

- New gas cell design

- RFQ Ion Guides

Jet properties with CD nozzles

R Ferrer NuSPRASEN 2019

50 mm

119875119887119892 ge 119875119895119890119905ICCD camera

Jet visualization the PLIF technique

laser

8

bull Information on velocity temperature and density distributions in the gas jet

Freqshift vFWHM TAmp rel density

63Cu

laser

Gas cell

Gas jet

laser

R Ferrer NuSPRASEN 2019

Central jet line Pbg asymp Popt

P0 = 380 mbar Pbg = 15 mbarQuasi-uniform jet

Characterization of jets formed by de Laval nozzles

L

9A Zadvornaya et al Phys Rev X 8 041008 (2018)R Ferrer NuSPRASEN 2019

Qu

asi-u

niform

je

t

CFD Module

PLIF

T0 = 500 K P0 = 379 mbar Pbg = 146 mbar

FWHM

Doppler shift

Characterization of jets formed by de Laval nozzles II

10A Zadvornaya et al Phys Rev X 8 041008 (2018)

Density

R Ferrer NuSPRASEN 2019

11

Nozzle (Mgt 5)

Characterization of the flow parameters by PLIFS and RIS and comparison with results from simulations

bull precision inner contour ~ 5 mmbull surface finishing Ra=01 mm

Shortcomings

bull Calculations considering inviscid flow software limitations

bull Precise (CNC) machining inner contour and surface finishing

New nozzle contour using advanced simulation code from Aeronautics and Aerospace Department (von Karman Institute for Fluid Dynamics)

Radia

l dis

tan

ce (

mm

)

Distance from nozzle throat (mm)

R Ferrer NuSPRASEN 2019

12

Characterization of jets by RIS

R Ferrer NuSPRASEN 2019

13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 5: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

5

In Gas Laser Ionization and Spectroscopy (IGLIS)

spectrometerHI beam

gas cell

CD nozzle RFQ ion guide

detectorstation

-40 -20 0 20 400

100

200

300

gas cell

gas jet

c

ou

nts

in 5

0 s

Detuning (GHz)

215Ac (T

12= 170 ms)

R F et al Nat Commun 8 (2017) 14520

In-Cell vs In-Jet Spectroscopy

ejet~eGC

R Ferrer NuSPRASEN 2019

6

Performance of IGLIS on Actinides

Characterizationoptimization offline IGLIS laboratory

R F et al Nat Commun 8 (2017) 14520 Y Kudryavtsev et al NIM B297 (2013) 7S Raeder et al NIM B 376 (2016) 382

bull collisions Δϑρ~T119895119890119905

T293K

03lowast ρjet

bull temperature Δ120599Doppler~1205990 Τ119879119895119890119905

119860

jet

in cell

in jet

R Ferrer NuSPRASEN 2019

7

IGLIS laboratory KU Leuven (off-line studies)

- High power high rep laser system

- New gas cell design

- RFQ Ion Guides

Jet properties with CD nozzles

R Ferrer NuSPRASEN 2019

50 mm

119875119887119892 ge 119875119895119890119905ICCD camera

Jet visualization the PLIF technique

laser

8

bull Information on velocity temperature and density distributions in the gas jet

Freqshift vFWHM TAmp rel density

63Cu

laser

Gas cell

Gas jet

laser

R Ferrer NuSPRASEN 2019

Central jet line Pbg asymp Popt

P0 = 380 mbar Pbg = 15 mbarQuasi-uniform jet

Characterization of jets formed by de Laval nozzles

L

9A Zadvornaya et al Phys Rev X 8 041008 (2018)R Ferrer NuSPRASEN 2019

Qu

asi-u

niform

je

t

CFD Module

PLIF

T0 = 500 K P0 = 379 mbar Pbg = 146 mbar

FWHM

Doppler shift

Characterization of jets formed by de Laval nozzles II

10A Zadvornaya et al Phys Rev X 8 041008 (2018)

Density

R Ferrer NuSPRASEN 2019

11

Nozzle (Mgt 5)

Characterization of the flow parameters by PLIFS and RIS and comparison with results from simulations

bull precision inner contour ~ 5 mmbull surface finishing Ra=01 mm

Shortcomings

bull Calculations considering inviscid flow software limitations

bull Precise (CNC) machining inner contour and surface finishing

New nozzle contour using advanced simulation code from Aeronautics and Aerospace Department (von Karman Institute for Fluid Dynamics)

Radia

l dis

tan

ce (

mm

)

Distance from nozzle throat (mm)

R Ferrer NuSPRASEN 2019

12

Characterization of jets by RIS

R Ferrer NuSPRASEN 2019

13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 6: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

6

Performance of IGLIS on Actinides

Characterizationoptimization offline IGLIS laboratory

R F et al Nat Commun 8 (2017) 14520 Y Kudryavtsev et al NIM B297 (2013) 7S Raeder et al NIM B 376 (2016) 382

bull collisions Δϑρ~T119895119890119905

T293K

03lowast ρjet

bull temperature Δ120599Doppler~1205990 Τ119879119895119890119905

119860

jet

in cell

in jet

R Ferrer NuSPRASEN 2019

7

IGLIS laboratory KU Leuven (off-line studies)

- High power high rep laser system

- New gas cell design

- RFQ Ion Guides

Jet properties with CD nozzles

R Ferrer NuSPRASEN 2019

50 mm

119875119887119892 ge 119875119895119890119905ICCD camera

Jet visualization the PLIF technique

laser

8

bull Information on velocity temperature and density distributions in the gas jet

Freqshift vFWHM TAmp rel density

63Cu

laser

Gas cell

Gas jet

laser

R Ferrer NuSPRASEN 2019

Central jet line Pbg asymp Popt

P0 = 380 mbar Pbg = 15 mbarQuasi-uniform jet

Characterization of jets formed by de Laval nozzles

L

9A Zadvornaya et al Phys Rev X 8 041008 (2018)R Ferrer NuSPRASEN 2019

Qu

asi-u

niform

je

t

CFD Module

PLIF

T0 = 500 K P0 = 379 mbar Pbg = 146 mbar

FWHM

Doppler shift

Characterization of jets formed by de Laval nozzles II

10A Zadvornaya et al Phys Rev X 8 041008 (2018)

Density

R Ferrer NuSPRASEN 2019

11

Nozzle (Mgt 5)

Characterization of the flow parameters by PLIFS and RIS and comparison with results from simulations

bull precision inner contour ~ 5 mmbull surface finishing Ra=01 mm

Shortcomings

bull Calculations considering inviscid flow software limitations

bull Precise (CNC) machining inner contour and surface finishing

New nozzle contour using advanced simulation code from Aeronautics and Aerospace Department (von Karman Institute for Fluid Dynamics)

Radia

l dis

tan

ce (

mm

)

Distance from nozzle throat (mm)

R Ferrer NuSPRASEN 2019

12

Characterization of jets by RIS

R Ferrer NuSPRASEN 2019

13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 7: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

7

IGLIS laboratory KU Leuven (off-line studies)

- High power high rep laser system

- New gas cell design

- RFQ Ion Guides

Jet properties with CD nozzles

R Ferrer NuSPRASEN 2019

50 mm

119875119887119892 ge 119875119895119890119905ICCD camera

Jet visualization the PLIF technique

laser

8

bull Information on velocity temperature and density distributions in the gas jet

Freqshift vFWHM TAmp rel density

63Cu

laser

Gas cell

Gas jet

laser

R Ferrer NuSPRASEN 2019

Central jet line Pbg asymp Popt

P0 = 380 mbar Pbg = 15 mbarQuasi-uniform jet

Characterization of jets formed by de Laval nozzles

L

9A Zadvornaya et al Phys Rev X 8 041008 (2018)R Ferrer NuSPRASEN 2019

Qu

asi-u

niform

je

t

CFD Module

PLIF

T0 = 500 K P0 = 379 mbar Pbg = 146 mbar

FWHM

Doppler shift

Characterization of jets formed by de Laval nozzles II

10A Zadvornaya et al Phys Rev X 8 041008 (2018)

Density

R Ferrer NuSPRASEN 2019

11

Nozzle (Mgt 5)

Characterization of the flow parameters by PLIFS and RIS and comparison with results from simulations

bull precision inner contour ~ 5 mmbull surface finishing Ra=01 mm

Shortcomings

bull Calculations considering inviscid flow software limitations

bull Precise (CNC) machining inner contour and surface finishing

New nozzle contour using advanced simulation code from Aeronautics and Aerospace Department (von Karman Institute for Fluid Dynamics)

Radia

l dis

tan

ce (

mm

)

Distance from nozzle throat (mm)

R Ferrer NuSPRASEN 2019

12

Characterization of jets by RIS

R Ferrer NuSPRASEN 2019

13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 8: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

50 mm

119875119887119892 ge 119875119895119890119905ICCD camera

Jet visualization the PLIF technique

laser

8

bull Information on velocity temperature and density distributions in the gas jet

Freqshift vFWHM TAmp rel density

63Cu

laser

Gas cell

Gas jet

laser

R Ferrer NuSPRASEN 2019

Central jet line Pbg asymp Popt

P0 = 380 mbar Pbg = 15 mbarQuasi-uniform jet

Characterization of jets formed by de Laval nozzles

L

9A Zadvornaya et al Phys Rev X 8 041008 (2018)R Ferrer NuSPRASEN 2019

Qu

asi-u

niform

je

t

CFD Module

PLIF

T0 = 500 K P0 = 379 mbar Pbg = 146 mbar

FWHM

Doppler shift

Characterization of jets formed by de Laval nozzles II

10A Zadvornaya et al Phys Rev X 8 041008 (2018)

Density

R Ferrer NuSPRASEN 2019

11

Nozzle (Mgt 5)

Characterization of the flow parameters by PLIFS and RIS and comparison with results from simulations

bull precision inner contour ~ 5 mmbull surface finishing Ra=01 mm

Shortcomings

bull Calculations considering inviscid flow software limitations

bull Precise (CNC) machining inner contour and surface finishing

New nozzle contour using advanced simulation code from Aeronautics and Aerospace Department (von Karman Institute for Fluid Dynamics)

Radia

l dis

tan

ce (

mm

)

Distance from nozzle throat (mm)

R Ferrer NuSPRASEN 2019

12

Characterization of jets by RIS

R Ferrer NuSPRASEN 2019

13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 9: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

Central jet line Pbg asymp Popt

P0 = 380 mbar Pbg = 15 mbarQuasi-uniform jet

Characterization of jets formed by de Laval nozzles

L

9A Zadvornaya et al Phys Rev X 8 041008 (2018)R Ferrer NuSPRASEN 2019

Qu

asi-u

niform

je

t

CFD Module

PLIF

T0 = 500 K P0 = 379 mbar Pbg = 146 mbar

FWHM

Doppler shift

Characterization of jets formed by de Laval nozzles II

10A Zadvornaya et al Phys Rev X 8 041008 (2018)

Density

R Ferrer NuSPRASEN 2019

11

Nozzle (Mgt 5)

Characterization of the flow parameters by PLIFS and RIS and comparison with results from simulations

bull precision inner contour ~ 5 mmbull surface finishing Ra=01 mm

Shortcomings

bull Calculations considering inviscid flow software limitations

bull Precise (CNC) machining inner contour and surface finishing

New nozzle contour using advanced simulation code from Aeronautics and Aerospace Department (von Karman Institute for Fluid Dynamics)

Radia

l dis

tan

ce (

mm

)

Distance from nozzle throat (mm)

R Ferrer NuSPRASEN 2019

12

Characterization of jets by RIS

R Ferrer NuSPRASEN 2019

13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 10: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

Qu

asi-u

niform

je

t

CFD Module

PLIF

T0 = 500 K P0 = 379 mbar Pbg = 146 mbar

FWHM

Doppler shift

Characterization of jets formed by de Laval nozzles II

10A Zadvornaya et al Phys Rev X 8 041008 (2018)

Density

R Ferrer NuSPRASEN 2019

11

Nozzle (Mgt 5)

Characterization of the flow parameters by PLIFS and RIS and comparison with results from simulations

bull precision inner contour ~ 5 mmbull surface finishing Ra=01 mm

Shortcomings

bull Calculations considering inviscid flow software limitations

bull Precise (CNC) machining inner contour and surface finishing

New nozzle contour using advanced simulation code from Aeronautics and Aerospace Department (von Karman Institute for Fluid Dynamics)

Radia

l dis

tan

ce (

mm

)

Distance from nozzle throat (mm)

R Ferrer NuSPRASEN 2019

12

Characterization of jets by RIS

R Ferrer NuSPRASEN 2019

13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 11: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

11

Nozzle (Mgt 5)

Characterization of the flow parameters by PLIFS and RIS and comparison with results from simulations

bull precision inner contour ~ 5 mmbull surface finishing Ra=01 mm

Shortcomings

bull Calculations considering inviscid flow software limitations

bull Precise (CNC) machining inner contour and surface finishing

New nozzle contour using advanced simulation code from Aeronautics and Aerospace Department (von Karman Institute for Fluid Dynamics)

Radia

l dis

tan

ce (

mm

)

Distance from nozzle throat (mm)

R Ferrer NuSPRASEN 2019

12

Characterization of jets by RIS

R Ferrer NuSPRASEN 2019

13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 12: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

12

Characterization of jets by RIS

R Ferrer NuSPRASEN 2019

13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

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13

Results of flow parameters using RIS

R Ferrer NuSPRASEN 2019

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 14: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

Ground state properties(mass size moments spins)

REGLIS3 setup

Low Energy

Branch

Atomic physics

FISIC setup

Fast Ion Slow

Ion Collisions

Electron exchange

S3 Experimental Techniques

In-beam spectroscopyTwo step reactions

EXOGAM2AGATA

PARIS

MUST2GASPARD

Delayed spectroscopy

SIRIUS setup

Implantation-decay

station at the mass

dispersive plane

Primary beam + EVR

from

LINAG

SPIRAL2 Phase1- Increase the intensity of stable beams- High intense neutron source(HIle 1015 pps p-Ni)

48Ca 25 pmicroA

R Ferrer NuSPRASEN 2019

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 15: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

15

REGLIS3 SPIRAL2S3- LEB Layout

diff pumpingmRFQ

QMF (mDm ~ 100)

RFQ buncher

90o bender

gas inlet

l12

l2 l1

EVRs

Neutralized EVRs

Photoions

gas cell

S-shape RFQ

from S3

SEASONdetector station

MR ToF MS(mDm ~ 105)

in-gas-cell

ionization

in-gas-jet

ionization

R F et al NIM B 317 (2013) 570

Y Kudryavtsev et al NIM B297 (2013) 7

Spectrally resolved hyperfine structure

RIBs (isomeric) of high purity for low energy experiments

VHERefractory

N=Z

P Chauveau et al NIM B 376 (2016) 211

towards DESIR

Phase 1+

R Ferrer NuSPRASEN 2019

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 16: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

Offline commissioning at LPC

16

PILGRIM

P Chauveau PhD

RFQsbull Characterization ion guides QMF MR ToF MSbull Study photodisotiation of moleculesbull Neutralization of ions in the gas cellbull Implement narrow-bandwidth injection-locked

Tisa laser

Courtesy N LecesneR Ferrer NuSPRASEN 2019

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 17: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

First experimental campaigns S3-LEB

17

10 pre-proposals for laser spectroscopy and MR-ToF

mass spectrometry of N=Z and actinide nuclei

P Campbell ID Moore MR Pearson Prog Part Nucl Phys 86 (2015) 127-180

R Ferrer NuSPRASEN 2019

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

Page 18: Supersonic Gas Jets for Laser Ionization Spectroscopy of Heavy … · 2019. 3. 11. · nozzle RFQ ion guide detector station-40 -20 0 20 40 0 100 200 300 gas cell gas jet nts in 50

18

197Au(20Ne xn)210-213Ac

bull Extend high-resolution laser spectroscopy studies

bull Refine atomic and nuclear structure predictions

206208Pb(48Ca xn)252-255No

bull Understand nuclear structure around and

at the N=152

bull IGLIS on K isomers -gt single-particle states

178180Hf(40Ar xn)213215216Th

bull Check magicity of N=126 shell closure

observed to vanish in the uranium isotopes

bull Probe nuclear structure near the proton drip line

First REGLIS3 experiments (1 puA)209Bi(48Ca xn)255Lr

bull Look for atomic levels

First experimental campaigns S3-LEB (Actinides)

In the meantime RADRIS-Jet SHIP (GSI) (approved beam time 2019-2020)

R Ferrer NuSPRASEN 2019

Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

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Summary

19

bull The In-Gas-Jet method is being optimized to study fusion evaporation reaction products

bull IGLIS combines good efficiency and spectral resolution and is well suitedfor the study of heavy elements

bull PLIF has been implemented and can be used to characterize local flow parameters find the best nozzles for IGLIS studies

bull Considering RIS as an alternative method to characterize flow parameters (higher efficiency)

bull Commissioning of REGLIS3 at LPC Caen is ongoing A full off-line characterization of the setup along with a further optimization of the IGLIS technique are planned

R Ferrer NuSPRASEN 2019

20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France

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20

Acknowledgments

THANK YOU ALL FOR YOUR ATTENTION

Collaborators

S3-LEBM Authier2 F Boumard3 L Caceres1 J-F Cam3 S Damoy1 P Delahaye1 P Desrue3 A Drouart2 P Duchesne5 X Fleacutechard3 S Franchoo5 P Gangnant1 R de Groote7 N Lecesne1 R Leroy1 J Lory3 F Lutton1 Y Merrer3 I Moore7 B Osmond1 J Piot1 O Pochon5 B-M Retailleau1 H Savajols1 E Traykov8 J Uusitalo7 C Vandamme3 M Vandebrouck2 and K Wendt6

GSI H Grawe S Raeder

K Dockx M Huyse S Kraemer Yu Kudryavtsev V Manea M Nabuurs P Van den Bergh D Reynaerts J Romans S Sels P Van Duppen M Verlinde E Verstraelen A Zadvornaya

KU Leuven

JoGu and Helmholtz-Institut MainzM Block P Chhetri R Heinke M Laatiaoui T Murboumlck P Naubereit S Nothhelfer F Schneider K Wendt

1GANIL CEADRF-CNRSIN2P3 BP 55027 14076 Caen France 2IRFU CEA-Saclay 91191 Gif-sur-Yvette France 3LPC Caen Normandie Univ ENSICAEN UNICAEN CNRSIN2P3 14000 Caen France 5IPNO Universiteacute Paris-Sud 11 CNRSIN2P3 91406 Orsay France 6Institut fuumlr Physik Johannes Gutenberg-Universitaumlt Mainz 55128 Mainz Germany 7Department of Physics University of Jyvaumlskylauml PO Box 35 (YFL) Jyvaumlskylauml FI-40014 Finland 8IPHC Universiteacute de Strasbourg 67037 Strasbourg France