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Synergetic use of mobile DOAS observation during CINDI-2 A. Merlaud, F. Tack, F. Hendrick, M. Van Roozendael (BIRA), D. Constantin, A. Rosu (UGal), K. Riffel, S. Donner, T. Wagner (MPIC), S. Schreier (Boku), A. Richter (IUP Bremen), H. Eskes (KNMI)

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Page 1: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Synergetic use of mobile DOAS observation during CINDI-2

A. Merlaud, F. Tack, F. Hendrick, M. Van Roozendael (BIRA), D. Constantin, A. Rosu (UGal), K. Riffel, S. Donner, T. Wagner (MPIC), S. Schreier (Boku), A. Richter (IUP Bremen), H. Eskes (KNMI)

Page 2: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Outline

• Status in Yokohama

• VCDs of Mobile DOAS vs BIRA Max-DOAS

• Azimuthal variability ?

• Comparison with models

• Comparison with OMI

Page 3: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Preliminary conclusions in September 2017

• Agreement between BIRA Mobile and MaxDOAS

• Good agreement between DOAS instruments and Lotos Euros on Sept 13

• seems less good on Sept 14, model > measurements in afternoon

• Measurements > model on Sept 15 all day

• What s next?

Page 4: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

5-sept 6-sept 7-sept 8-sept 9-sept 10-sept 11-sept

BOKU

BIRA_car

BIRA_bike

MPIC

UGAL

12-sept 13-sept 14-sept 15-sept 16-sept 17-sept 18-sept

BOKU

BIRA_car

BIRA_bike

MPIC

UGAL

19-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept

BOKU

BIRA_car

BIRA_bike

MPIC

UGAL

Overview of the measurements

Page 5: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Aeromobil vs BIRA Max-DOAS (13-14-15 September)

Page 6: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

BikeDOAS vs BIRA Max-DOAS (13-14-15 September)

Page 7: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

UGAL Mobile DOAS vs BIRA Max-DOAS (14-15-24 September)

Page 8: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

MPIC Mini MaxDOAS vs BIRA Max-DOAS (14-15-24 September)

Page 9: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

BOKU Mini MaxDOAS vs BIRA Max-DOAS (13-14-15 September)

Page 10: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Coordinated Mobile DOAS measurements during CINDI-2

Page 11: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

13/09/2016

14/09/2016

15/09/2016

8.4 – 8.48 UTC 14.42 – 14.48 UTC 8.92 – 8.98 UTC

Azimuthal variability in the VCDs seen with the BIRA Max-DOAS

Page 12: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Measurements vs Lotos Euros

-7 km resolution -surface to 3.5 km -O3, NO2, NO, SO2, CO, PM10, PM2.5

Page 13: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Measurements vs Lotos Euros 13 September 2016

Page 14: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Measurements vs Lotos Euros 14 September 2016

Page 15: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Measurements vs Lotos Euros 15 September 2016

Page 16: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Page 17: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Page 18: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Page 19: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Page 20: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Page 21: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Page 22: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Page 23: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Page 24: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Page 25: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Lotos Euros OMI

13 September 2016 at 12 UT

Page 26: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Can the model be used to reduce the representativeness error between the Mobile DOAS and OMI ?

Page 27: Synergetic use of mobile DOAS observation during CINDI-219-sept 20-sept 21-sept 22-sept 23-sept 24-sept 25-sept BOKU BIRA_car BIRA_bike MPIC UGAL Overview of the measurements . Aeromobil

Conclusions

• Dataset of mobile doas vcds consistent with Max-DOAS

• Limited azimuthal variability on Sept 13-14-15

• Including additional measurements confirms earlier comparisons with Lotos Euros on Sept 13-14-15

• Higher VCDs on 15 September correlated with transport from most polluted areas

• For comparison with satellite, how do mobile measurements reduce the representativeness error? Does it help to include a model-based correction?

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