the utilization of thorium for long-life small thermal reactors without on-site refueling

5
The utilization of thorium for long-life small thermal reactors without on-site refueling Iyos Subki a, * , Asril Pramutadi b ,S.N.M. Rida b , Zaki Su’ud b , R. Eka Sapta a,b , S. Muh. Nurul a,b , S. Topan a,b , Yuli Astuti a,b , Sedyartomo Soentono a a  National Atomic Energy Agency (BATAN) Indonesia b  Nuclear and Reactor Physics Laboratory, ITB, Bandung , Indones ia Abstract Thorium cycle has many advantages over uranium cycle in thermal and intermediate spectrum nuclear reactors. In addition to large amount of resou rces in the world which up to now still not utiliz ed optimally , thoriu m based thermal reactors may have high inter nal conversion ratio so that they are very potential to be designed as long-life reactors without on-site refueling based on thermal spectrum cores. In this study prelim- inary study for application of thorium cycle in some of thermal reactors has been performed. We applied thorium cycle for small long-life high temperature gas reactors without on-site refueling. Calculation results using SRAC code show that 10 years lifetime without on-site refueling can be achieved with excess reactivity of about 10% dk/k. The next application of thorium cycle has been employed in long-life small and medium PWR cores without on-site refueling. Relatively high fuel volume fraction is also applied to get relatively hard spectrum, small size, and high internal conversion ratio. In the current study we have been able to reach more than 10 years lifetime without on-site refueling for 20 e300 MWth PWR with maximum excess reactivity of a few %dk/k. The last application of thorium cycle has been employed in long-life BWR cores without on-site refueling. Relatively high fuel volume fraction is applied to get relatively hard spectrum, small size, and high internal conversion ratio. In the current study we have been able to reach more than 10 years lifetime without on-site refueling for 100e600 MWth BWR with maximum excess reactivity of a few %dk/k. Ó 2007 Published by Elsevier Ltd.  Keywords: Thorium cycle; Long-life thermal reactors; High internal conversion ratio; SRAC code; Hard spectrum; Excess reactivity 1. Introduction Thorium cycle in general has better conversion ratio than uranium cycle in the thermal spectrum. In this study, thorium cycle is used to extend the thermal reactor operation cycle without on-site refueling. Basically we have to adjust the mod- erating ratio and fuel enrichment to be able to improve internal conversion ratio. And by geometrical optimization process we can get the design of small long-life high temper ature gas cooled reactors (HTGR) without on-site fueling, small long- life pressurized water reactors (PWR) witho ut on-site fuelin g, and small boil ing wa ter reactors (BWR) without on-sit e fueling. 2. Design concept In order to extend the refueling cycle without excessive re- activity swing in high temperature gas cooled reactors we need rea ctor core wit h hig h internal con ver sion rat io, in gen eral around unity. In thermal reactors such as HTGR, proper com- bination of 232 The 233 U cycle gives high possibility to achieve such objective. Adjusting moderation ratio by appropriately set ting the gra phi te mod era tor and fue l compos iti on is one of important strategy to get harder neutron spectrum so that much better conversion ratio can be reached. Here we performed many parametric surveys to understand the inuence of many parameters such as moderating ratio, * Corresponding author.  E-mail address es: [email protected] (I. Subki ), szaki@.itb.ac.id (Z. Su’ud). 0149-1970/$ - see front matter Ó 2007 Published by Elsevier Ltd. doi:10.1016/j.pnucene.2007.10.029  Available online at www.sciencedirect.com Progress in Nuclear Energy 50 (2008) 152e156 www.elsevier.com/locate/pnucene

Upload: topan-setiadipura

Post on 30-May-2018

219 views

Category:

Documents


0 download

TRANSCRIPT

Page 1: The Utilization of Thorium for Long-life Small Thermal Reactors Without on-site Refueling

8/14/2019 The Utilization of Thorium for Long-life Small Thermal Reactors Without on-site Refueling

http://slidepdf.com/reader/full/the-utilization-of-thorium-for-long-life-small-thermal-reactors-without-on-site 1/5

The utilization of thorium for long-life small thermalreactors without on-site refueling

Iyos Subki a,*, Asril Pramutadi b, S.N.M. Rida b, Zaki Su’ud b, R. Eka Sapta a,b,S. Muh. Nurul a,b, S. Topan a,b, Yuli Astuti a,b, Sedyartomo Soentono a

a  National Atomic Energy Agency (BATAN) Indonesiab  Nuclear and Reactor Physics Laboratory, ITB, Bandung, Indonesia

Abstract

Thorium cycle has many advantages over uranium cycle in thermal and intermediate spectrum nuclear reactors. In addition to large amount of 

resources in the world which up to now still not utilized optimally, thorium based thermal reactors may have high internal conversion ratio so

that they are very potential to be designed as long-life reactors without on-site refueling based on thermal spectrum cores. In this study prelim-

inary study for application of thorium cycle in some of thermal reactors has been performed.

We applied thorium cycle for small long-life high temperature gas reactors without on-site refueling. Calculation results using SRAC code

show that 10 years lifetime without on-site refueling can be achieved with excess reactivity of about 10% dk/k.

The next application of thorium cycle has been employed in long-life small and medium PWR cores without on-site refueling. Relatively high

fuel volume fraction is also applied to get relatively hard spectrum, small size, and high internal conversion ratio. In the current study we have

been able to reach more than 10 years lifetime without on-site refueling for 20e300 MWth PWR with maximum excess reactivity of a few %dk/k.

The last application of thorium cycle has been employed in long-life BWR cores without on-site refueling. Relatively high fuel volume

fraction is applied to get relatively hard spectrum, small size, and high internal conversion ratio. In the current study we have been able to reach

more than 10 years lifetime without on-site refueling for 100e

600 MWth BWR with maximum excess reactivity of a few %dk/k.Ó 2007 Published by Elsevier Ltd.

 Keywords: Thorium cycle; Long-life thermal reactors; High internal conversion ratio; SRAC code; Hard spectrum; Excess reactivity

1. Introduction

Thorium cycle in general has better conversion ratio than

uranium cycle in the thermal spectrum. In this study, thorium

cycle is used to extend the thermal reactor operation cycle

without on-site refueling. Basically we have to adjust the mod-erating ratio and fuel enrichment to be able to improve internal

conversion ratio. And by geometrical optimization process we

can get the design of small long-life high temperature gas

cooled reactors (HTGR) without on-site fueling, small long-

life pressurized water reactors (PWR) without on-site fueling,

and small boiling water reactors (BWR) without on-site

fueling.

2. Design concept

In order to extend the refueling cycle without excessive re-activity swing in high temperature gas cooled reactors we need

reactor core with high internal conversion ratio, in general

around unity. In thermal reactors such as HTGR, proper com-

bination of 232The233U cycle gives high possibility to achieve

such objective. Adjusting moderation ratio by appropriately

setting the graphite moderator and fuel composition is one

of important strategy to get harder neutron spectrum so that

much better conversion ratio can be reached.

Here we performed many parametric surveys to understand

the influence of many parameters such as moderating ratio,

* Corresponding author.

  E-mail addresses: [email protected] (I. Subki), [email protected]

(Z. Su’ud).

0149-1970/$ - see front matter Ó 2007 Published by Elsevier Ltd.

doi:10.1016/j.pnucene.2007.10.029

 Available online at www.sciencedirect.com

Progress in Nuclear Energy 50 (2008) 152e156www.elsevier.com/locate/pnucene

Page 2: The Utilization of Thorium for Long-life Small Thermal Reactors Without on-site Refueling

8/14/2019 The Utilization of Thorium for Long-life Small Thermal Reactors Without on-site Refueling

http://slidepdf.com/reader/full/the-utilization-of-thorium-for-long-life-small-thermal-reactors-without-on-site 2/5

fuel enrichment, linear power, etc. to the infinite multiplica-

tion factors pattern during burn-up. Using the results of para-

metric survey we can then perform optimization in the core

level.

Similar approach is used for long-life small pressurized

water reactors without on-site refueling and long-life small

long-life BWR without on-site refueling and here we apply

tight lattice concept to get small core with relatively high

internal conversion ratio.

3. Computational method

For computation method we used SRAC code system to

calculate cell calculation and cell burn-up. Whole core

SRAC PUBLIC LIBRARY

JENDL-3.2,

SRAC USER LIBRARY

Flux, Microscopic,,

Macroscopic

CELL CALCULATION.,

BURNUP

START

HOMOGENISATION

& COLLAPSING

CORE

CALCULATION

(CITATION)

CALCULATION

RESULT

END

Fig. 1. Computation scheme in this study.

1.00000E+00

1.05000E+00

1.10000E+00

1.15000E+00

1.20000E+00

1.25000E+00

1.30000E+00

1.35000E+00

1.40000E+001.45000E+00

1.50000E+00

0 2 4 6 8 10

      K   -      i    n

      f

Time (year)

K-inf vs Time of fuel element

3.00% 3.30% 3.60% 3.90% 4.50% 4.90%

5.10% 5.40% 5.70% 6.00% 6.30% 6.60%

Fig. 2. Infinite multiplication change during burn-up for various enrichment of  233U in the fuel.

153  I. Subki et al. / Progress in Nuclear Energy 50 (2008) 152e156 

Page 3: The Utilization of Thorium for Long-life Small Thermal Reactors Without on-site Refueling

8/14/2019 The Utilization of Thorium for Long-life Small Thermal Reactors Without on-site Refueling

http://slidepdf.com/reader/full/the-utilization-of-thorium-for-long-life-small-thermal-reactors-without-on-site 3/5

calculation is performed using CITATION or FI-ITBCH

codes. For SRAC code system calculation the calculation

scheme is shown in Fig. 1.

When we calculate the whole core calculation using

FI-ITBCH code, interpolation for linear power parameter is

performed to get relatively accurate results with optimal com-

putation time.

4. Simulation results and discussion

 4.1. Small long-life high temperature gas cooled reactors

without on-site refueling

Fig. 2 shows the results of cell-burn-up parametric survey

for different fuel enrichments (233U) during 10 years burn-up

without refueling.

From Fig. 2 it is shown that in general higher enrichment

gives longer lifetime but also higher reactivity swing. Core en-

richment of 3% gives smaller infinite multiplication constant

drop after 10 years of burn-up. This trend can be thought as

an influence of higher internal conversion ratio in fuel with

lower enrichment 233U Fig. 3.

As the next steps we performed core optimization and as

one of the optimal results we can see the combination shown

in Table 1 as follows.

So as shown in the above table we used various values of 

fuel enrichment (233U) in core optimization. The effective

multiplication factor change during burn-up for the above

core configuration is shown in Fig. 4.

Fig. 4 shows that during 10 years of burn-up without

refueling, the core composition shown in Table 1 in which

30 column of fuel were filled give excess reactivity of about12% dk/k.

 4.2. Small long-life pressurized water reactors (PWR)

without on-site refueling

Similar method to that of long-life HTGR was applied to

the long-life PWR without on-site refueling. After some opti-

mizations we get the following pattern for 100 MWth long-life

PWR without on-site refueling based on thorium cycle. Fig. 5

Fig. 3. Core lay-out of small long-life high temperature gas cooled reactors

without on-site refueling.

Table 1

One example of core level optimization results of long-life small high temper-

ature gas cooled reactors without on-site refueling

Position of 

fuel block 

(from above)

Fuel characteristics No. of fuel zone

1 2 3 4

1 Uranium-233 enrichment (wt%) 5 .4 6.0 6.3 6.6

Number of fuel pins 33 33 31 31

Type of burnable poisson H-I H-I H-I H-I

2 Uranium-233 enrichment (wt%) 4 .5 5.1 5.7 6.0

Number of fuel pins 33 33 31 31

Type of burnable poisson H-II H-II H-II H-II

3 Uranium-233 enrichment (wt%) 3 .6 4.5 4.9 5.1

Number of fuel pins 33 33 31 31

Type of burnable poisson H-II H-II H-II H-II

4 Uranium-233 enrichment (wt%) 3 .0 3.3 3.6 3.9

Number of fuel pins 33 33 31 31

Type of burnable poisson H-I H-I H-I H-I

5 Uranium-233 enrichment (wt%) 3 .0 3.3 3.6 3.9

Number of fuel pins 33 33 31 31

Type of burnable poisson H-I H-I H-I H-I

K-eff vs Time at 30 column for a,b,c,d,e core combination

8.50000E-01

9.00000E-01

9.50000E-01

1.00000E+00

1.05000E+00

1.10000E+00

1.15000E+00

1.20000E+00

0 1 2 3 4 5 6 7 8 9 10

Time (year)

      K   -    e

      f      f

a b c d e

Fig. 4. Effective multiplication factor change during burn-up and the combination shown in Table 1 correspond to the ‘a’ line.

154 I. Subki et al. / Progress in Nuclear Energy 50 (2008) 152e156 

Page 4: The Utilization of Thorium for Long-life Small Thermal Reactors Without on-site Refueling

8/14/2019 The Utilization of Thorium for Long-life Small Thermal Reactors Without on-site Refueling

http://slidepdf.com/reader/full/the-utilization-of-thorium-for-long-life-small-thermal-reactors-without-on-site 4/5

shows a pattern of multiplication factor change for 100 MWth

10 years long-life PWR without on-site fueling. Detail param-

eters are shown in Table 2 as follows.

 4.3. Small long-life boiling water reactors (BWR)

without on-site refueling

Similar process to the long-life PWR was applied to the

long-life BWR and some results are shown as follows.

Fig. 6 shows infinite multiplication pattern change during

burn-up for thorium cycle for various enrichment of  233U.

It is shown that high enrichment fuel (around 6%) giveshigher initial infinite multiplication factor but the value

decreases much faster than that of lower enrichments. On

the other hand, very low enrichment gives low initial infinite

multiplication factor value but then increases. Using the above

0.99000

1.00000

1.01000

1.02000

1.03000

1.04000

1.05000

1.06000

1.07000

1.08000

0 2 4 6 8 10 12

Burnup(year)

      K   -    e      f

      f

Fig. 5. Effective multiplication factor change during burn-up for the core configuration shown in Table 2.

Table 2

Design Specification of long-life PWR 100 MWth

Parameter Specification

Power (thermal) 100 MWth

Refueling 10 years

Core type Tall

Radial 90e100 cm

Axial 216e266 cm

Fuels Thoriumeuranium dioxide (Th,U)O2

Structure Zircalloy

Coolant Light water (H2O)

Cell type Square cell

Smear density 90% T.D.

Enrichment 1.5e3% 233U

Density (Th,U)O2 9.64 g/cm3

Fuel fraction 60%

Pin size

Clad thickness 0.07 cm

Pitch 1.4 cm

K-inf vs Time for Different Enrichment

0.75

0.8

0.85

0.9

0.95

1

1.05

1.1

1.15

1.2

0 1 2 3 4 5 6 7 8 9

Time (Year)

      K   -      i    n

      f

2.10%2.300%2.500%2.700%2.900%3.100%

3.300%3.500%3.700%3.900%4.100%4.300%4.500%4.700%4.900%5.100%5.300%5.500%5.700%5.900%6.100%

Fig. 6. Infinite multiplication factor change during burn-up for various enrichment of  233U in thorium cycle tight lattice core.

155  I. Subki et al. / Progress in Nuclear Energy 50 (2008) 152e156 

Page 5: The Utilization of Thorium for Long-life Small Thermal Reactors Without on-site Refueling

8/14/2019 The Utilization of Thorium for Long-life Small Thermal Reactors Without on-site Refueling

http://slidepdf.com/reader/full/the-utilization-of-thorium-for-long-life-small-thermal-reactors-without-on-site 5/5

parametric survey results and after some optimization pro-

cesses we could get some designs which can be operated for

10 years of burn-up without on-site fueling with excess

reactivity less than 5%.

5. Conclusion

The thorium cycle has been successfully applied to design

long-life high temperature gas cooled reactor without on-site

refueling, long-life pressurized water reactors without on-site

refueling, and long-life boiling water reactors without

on-site refueling. For small long-life high temperature gas

reactors without on-site refueling. Calculation results show

that 10 years lifetime without on-site refueling can be achieved

with excess reactivity of about 10% dk/k.

For long-life PWR and BWR relatively high fuel volume

fraction is applied to get relatively hard spectrum, small

size, and high internal conversion ratio. For long-life small

PWR without on-site fueling, 10 years lifetime without on-site refueling for 20e300 MWth PWR have been reached

with maximum excess reactivity of a few %dk/k. Similarly

for long-life BWR without on-site refueling, in the current

study we have been able to reach more than 10 years lifetime

without on-site refueling for 100e600 MWth BWR with

maximum excess reactivity of a few %dk/k.

156 I. Subki et al. / Progress in Nuclear Energy 50 (2008) 152e156