determination of thermal neutrons withneutrons with lif ... neutrons.pdf · y = 0.0718x + 0.2424 r2...

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2004 2004 2004 1 1 Determination of thermal neutrons with LiF TLD Determination of thermal Determination of thermal neutrons with neutrons with LiF LiF TLD TLD Zeev Zeev B. B. Alfassi Alfassi Department of Nuclear Department of Nuclear engineering engineering

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Page 1: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 11

Determination of thermal neutrons with LiF TLD

Determination of thermal Determination of thermal neutrons withneutrons with LiFLiF TLDTLD

ZeevZeev B.B. AlfassiAlfassiDepartment of Nuclear Department of Nuclear

engineeringengineering

Page 2: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 22

Page 3: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 33

Page 4: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 44

Page 5: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 55

Page 6: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 66

Page 7: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 77

Page 8: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 88

Page 9: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 99

Page 10: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1010

Page 11: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1111

Page 12: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1212

Page 13: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1313

Page 14: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1414

Page 15: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1515

Page 16: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1616

TTPstandard

long TTP for γirradiationlong TTP for thermal

neutrons irradiation

Page 17: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1717

0

1270

18-

ROI-67ROI-45

Page 18: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1818

irradiation γ ROI(4+5) irradiationirradiation γγ ROI(4+5)ROI(4+5)

y = 0.3548x + 0.0502R2 = 0.9999

0

5

10

15

20

25

0 10 20 30 40 50 60

Dose (mSv)

RO

I 45

(mill

ions

of c

ount

s)

Page 19: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1919

irradiation γ ROI(6+7) irradiationirradiation γγ ROI(6+7)ROI(6+7)

y = 6.5176x + 4.3933R2 = 0.9998

050

100150200250300350400

0 10 20 30 40 50 60

Dose (mSv)

RO

I 67

(thou

sand

s of

cou

nts)

Page 20: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 2020

Page 21: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 2121

Page 22: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 2222

Dose ROI-45 stdv (%) of ROI-67 stdv (%) of Normalized area/mSv***

(mSv) (*) ROI-45 (**) ROI-67 ROI-45 ROI-67

3 1.09 6.50 23.46 18.84 1.00 ± 0.07 1.00 ± 0.19 6 2.21 11.04 44.50 17.80 1.01 ± 0.11 0.95 ± 0.17 9 3.32 8.18 64.85 12.70 1.01 ± 0.08 0.92 ± 0.12 12 4.27 8.88 82.07 12.52 0.97 ± 0.09 0.87 ± 0.11 25 8.84 8.89 164.35 11.63 0.97 ± 0.09 0.84 ± 0.09 50 17.82 7.94 331.48 9.76 0.98 ± 0.08 0.85 ± 0.08

Table 1. The areas of the regions of interest of peaks 4+5 and 6+7 for different gamma ray doses from a 137Cs source.

(*) ROI-45 is the glow curve area in the region of peaks 4 and 5 in millions of counts. (**) ROI-67 is the glow curve area in the region of peaks 6 and 7 in thousands of counts. (***) Normalization of the area/mSv value to the value at 3mSv.

Page 23: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 2323

6+4/7+5 66++44//77++55

Gamma rays

0,01

0,015

0,02

0,025

0,03

0 10 20 30 40 50 60Dose (mSv)

Rat

io o

f pea

ks 6

&7 /

4&5

Page 24: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 2424

6+4/7+5 66++44//77++55

Thermal neutrons

0,1

0,15

0,2

0,25

0,3

0 2 4 6 8 10Irradiation time (hours)

Rat

io o

f pea

ks 6

&7 /

4&5

Page 25: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 2525

Page 26: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 2626

Page 27: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 2727

0.1 1 100.00

0.05

0.10

0.15

0.20

0.25

Chi^2 = 3.3857E-6R^2 = 0.99927 P1 0.018 ± 0.00061P2 0.21533 ± 0.00106

A 67 /

A45

Dn / Dγγγγ

Page 28: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 2828

0

2

4

6

8

10

12

25 50 75 100 125 150 200

Channel

Arb

itrary

scale

Normalized PTTL glow curves from TLD-600 . following neutron irradiation.

- - - - - - following gamma ray irradiation.

Page 29: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 2929

y = 0.1663x + 0.6767R2 = 0.9962

y = 0.1549x + 0.4556R2 = 0.9968

y = 0.0718x + 0.2424R2 = 0.9966

y = 0.0714x + 0.251R2 = 0.9972

0

2

4

6

8

10

12

14

16

18

20

0 20 40 60 80 100 120 140

Original readout

PTTL

G3_TTP5G4_TTP5G3_TTP2G4_TTP2

PTTL vs. the original readout for thermal neutrons (mGy - 137Cs equivalent),for two readout times: - TTP2 : 20 seconds readout - TTP5 : 13.3 seconds readout.

Page 30: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 3030

Gamma ray exposure Neutron exposure Exposure (mSv) % PTTL Exposure (mSv) % PTTL

5 8.6 ± 1.0 1.5 36 ± 4 10 7.3 ± 0.9 2.5 30 ± 3 15 7.0 ± 0.8 4.2 29 ± 2

5.8 28 ± 1 7.7 31 ± 3

AVERAGE : Pg = 7.6 ± 1 % AVERAGE : Pn = 31 ± 3 %

Page 31: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 3131

DTOT = DG + DN PTOT = (PG*DG + PN*DN ) / 100

DTOT - The total dose in a mixed field. DG - The gamma dose contribution. DN - The neutron dose contribution. PTOT - The total PTTL reading. PG - PTTL percent for gamma rays (7.6%). PN - PTTL percent for neutrons (31%).

100( ) /100

NTOT TOT

GN G

PD PD

P P

−=

−100

( ) /100

GTOT TOT

NN G

PP DD

P P

−=

Page 32: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 3232

Page 33: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 3333

Page 34: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 35: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 36: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 37: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 38: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 39: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 40: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 4040

Page 41: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 42: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 43: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 44: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 45: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 46: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 47: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 48: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 49: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 50: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 5050

Page 51: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 52: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 5252

Page 53: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 5353