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Page 1: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 11

Determination of thermal neutrons with LiF TLD

Determination of thermal Determination of thermal neutrons withneutrons with LiFLiF TLDTLD

ZeevZeev B.B. AlfassiAlfassiDepartment of Nuclear Department of Nuclear

engineeringengineering

Page 2: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 3: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 4: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 5: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 6: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 7: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 8: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 9: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 10: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 11: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 12: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 13: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 14: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 15: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 16: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1616

TTPstandard

long TTP for γirradiationlong TTP for thermal

neutrons irradiation

Page 17: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1717

0

1270

18-

ROI-67ROI-45

Page 18: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 1818

irradiation γ ROI(4+5) irradiationirradiation γγ ROI(4+5)ROI(4+5)

y = 0.3548x + 0.0502R2 = 0.9999

0

5

10

15

20

25

0 10 20 30 40 50 60

Dose (mSv)

RO

I 45

(mill

ions

of c

ount

s)

Page 19: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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irradiation γ ROI(6+7) irradiationirradiation γγ ROI(6+7)ROI(6+7)

y = 6.5176x + 4.3933R2 = 0.9998

050

100150200250300350400

0 10 20 30 40 50 60

Dose (mSv)

RO

I 67

(thou

sand

s of

cou

nts)

Page 20: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

200420042004 2020

Page 21: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 22: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Dose ROI-45 stdv (%) of ROI-67 stdv (%) of Normalized area/mSv***

(mSv) (*) ROI-45 (**) ROI-67 ROI-45 ROI-67

3 1.09 6.50 23.46 18.84 1.00 ± 0.07 1.00 ± 0.19 6 2.21 11.04 44.50 17.80 1.01 ± 0.11 0.95 ± 0.17 9 3.32 8.18 64.85 12.70 1.01 ± 0.08 0.92 ± 0.12 12 4.27 8.88 82.07 12.52 0.97 ± 0.09 0.87 ± 0.11 25 8.84 8.89 164.35 11.63 0.97 ± 0.09 0.84 ± 0.09 50 17.82 7.94 331.48 9.76 0.98 ± 0.08 0.85 ± 0.08

Table 1. The areas of the regions of interest of peaks 4+5 and 6+7 for different gamma ray doses from a 137Cs source.

(*) ROI-45 is the glow curve area in the region of peaks 4 and 5 in millions of counts. (**) ROI-67 is the glow curve area in the region of peaks 6 and 7 in thousands of counts. (***) Normalization of the area/mSv value to the value at 3mSv.

Page 23: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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6+4/7+5 66++44//77++55

Gamma rays

0,01

0,015

0,02

0,025

0,03

0 10 20 30 40 50 60Dose (mSv)

Rat

io o

f pea

ks 6

&7 /

4&5

Page 24: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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6+4/7+5 66++44//77++55

Thermal neutrons

0,1

0,15

0,2

0,25

0,3

0 2 4 6 8 10Irradiation time (hours)

Rat

io o

f pea

ks 6

&7 /

4&5

Page 25: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 26: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 27: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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0.1 1 100.00

0.05

0.10

0.15

0.20

0.25

Chi^2 = 3.3857E-6R^2 = 0.99927 P1 0.018 ± 0.00061P2 0.21533 ± 0.00106

A 67 /

A45

Dn / Dγγγγ

Page 28: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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0

2

4

6

8

10

12

25 50 75 100 125 150 200

Channel

Arb

itrary

scale

Normalized PTTL glow curves from TLD-600 . following neutron irradiation.

- - - - - - following gamma ray irradiation.

Page 29: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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y = 0.1663x + 0.6767R2 = 0.9962

y = 0.1549x + 0.4556R2 = 0.9968

y = 0.0718x + 0.2424R2 = 0.9966

y = 0.0714x + 0.251R2 = 0.9972

0

2

4

6

8

10

12

14

16

18

20

0 20 40 60 80 100 120 140

Original readout

PTTL

G3_TTP5G4_TTP5G3_TTP2G4_TTP2

PTTL vs. the original readout for thermal neutrons (mGy - 137Cs equivalent),for two readout times: - TTP2 : 20 seconds readout - TTP5 : 13.3 seconds readout.

Page 30: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Gamma ray exposure Neutron exposure Exposure (mSv) % PTTL Exposure (mSv) % PTTL

5 8.6 ± 1.0 1.5 36 ± 4 10 7.3 ± 0.9 2.5 30 ± 3 15 7.0 ± 0.8 4.2 29 ± 2

5.8 28 ± 1 7.7 31 ± 3

AVERAGE : Pg = 7.6 ± 1 % AVERAGE : Pn = 31 ± 3 %

Page 31: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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DTOT = DG + DN PTOT = (PG*DG + PN*DN ) / 100

DTOT - The total dose in a mixed field. DG - The gamma dose contribution. DN - The neutron dose contribution. PTOT - The total PTTL reading. PG - PTTL percent for gamma rays (7.6%). PN - PTTL percent for neutrons (31%).

100( ) /100

NTOT TOT

GN G

PD PD

P P

−=

−100

( ) /100

GTOT TOT

NN G

PP DD

P P

−=

Page 32: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 33: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 34: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 35: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 36: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 37: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 38: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 39: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 40: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 41: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 42: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 43: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 44: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 45: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 46: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 47: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 48: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 49: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 50: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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Page 51: Determination of thermal neutrons withneutrons with LiF ... neutrons.pdf · y = 0.0718x + 0.2424 R2 = 0.9966 y = 0.0714x + 0.251 R2 = 0.9972 0 2 4 6 8 10 12 14 16 18 20 0 20 40 60

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