grain-size analysis of the neogene red clay formation in the pannonian basin
TRANSCRIPT
ORIGINAL PAPER
Grain-size analysis of the Neogene red clay formationin the Pannonian Basin
Janos Kovacs
Received: 11 April 2006 / Accepted: 4 August 2006 / Published online: 13 December 2006� Springer-Verlag 2006
Abstract The red clay is a significant deposit under-
lying the Pleistocene loess-paleosols sequence in the
Pannonian Basin. The sedimentary processes involved
and the origin of the materials remain controversial. In
order to determine the depositional processes of the
Pliocene red clay formation we studied many red clay
sections in Hungary. Here, we present results of grain-
size analyses of the red clay from representative sites.
In particular their grain-size distribution is compared
with that of typical Pleistocene eolian loess-paleosols,
as well as lacustrine and fluvial sediments. It appears
from the sedimentological data that the majority of the
red clay is of a wind-blown origin. The red clay might
be transported by weak westerly winds and has been
modified by post-depositional alteration.
Keywords Sedimentology � Neogene � Red clay �Pannonian Basin � Grain size
Introduction
Over the past decade abundant information about var-
ious aspects of the loess was obtained, but little attention
has been paid to the red clay in the Pannonian Basin. Full
investigation of the formation is needed, particularly
regarding its geographic distribution, stratigraphy,
chronology and paleoclimate reconstruction. At the first
stage of this investigation, it is critical to determine the
manner of deposition of the red clay deposits.
Different views on the formation, properties and
distribution of red clays in the Pannonian Basin have
been published by several authors. Early scientists
described the red clay as a variety of loess, sediment
formed by the deposition of wind-blown silt (Loczy
1886; Treitz 1904; Sumeghy 1944). At that time other
researcher e.g. Szabo and Molnar (1866) and Balle-
negger (1917) agreed that the red clay formed by the
weathering of volcanic material. After the 1950s dif-
ferent ideas have developed about the distribution of
red clay. Many geologists draw parallels between red
clays and bauxites (Vadasz 1956; Vendl 1957; Bardossy
and Aleva 1990).
In the last decade investigations have focused on
geology, mineralogy and pedology (Fekete et al. 1997;
Nemeth et al. 1999; Fekete 2002; Foldvari and Kovacs-
Palffy 2002; Viczian 2002a, b; Berenyi-Uveges et al.
2003; Koloszar and Marsi 2005). Complex investigation
including geology, geomorphology, mineralogy and
geochemistry was carried out only a few authors like
Schweitzer and Szo}or (1997) and Kovacs (2003). None
of these recent investigations discussed the deposi-
tional process of the red clay.
The most remarkable progress made on the red clay
research worldwide is that sedimentology, geochemis-
try, geomorphology and field survey all demonstrate a
wind-blown origin for the red clay (Ding et al. 1998;
Sun et al. 2002, 2004; Lu et al. 2001; Yang and Ding
2004; Kovacs 2006), like the overlying Pleistocene and
Holocene loess. However, the stratigraphy of the
whole Pliocene is still far from being understood,
mainly because of the efficient coverage of the terrain
by the terrestrial alluvial fan systems.
Important key formations in the stratigraphy are
the red (silty) clays. Litho-, bio-, chemo- and
J. Kovacs (&)Department of Geology, University of Pecs,Ifjusag u. 6, Pecs, Baranya 7624, Hungarye-mail: [email protected]
123
Int J Earth Sci (Geol Rundsch) (2008) 97:171–178
DOI 10.1007/s00531-006-0150-2
magnetostratigraphic data show that they formed in
different periods (Schweitzer and Szo}or 1997; Kovacs
2003). The youngest one the red paleosol (or reddish
clay) is of Early Pleistocene age. The older one (red
clay) was formed probably in the Zanclean–Piacenzian
(4.6–3.2 Ma) under a warm, humid subtropical mon-
soon-like climatic conditions (Kretzoi 1987; Pecsi 1985;
Schweitzer and Szo}or 1997; Kovacs 2003).
Geological setting
The investigated sections selected for this study are
located mainly on the foothills of Hungarian moun-
tains (Fig. 1). These sections are of Pliocene and Early
Pleistocene age. From the studied areas we present
here a sequence (case study) which is similar to the
others.
Atkar site
Atkar (sand pit) lies on the southern remnants of the
Matra pediment. The sand pit deepens 20–25 m into
the surface. The exposure shows the Upper Miocene–
Lower Pliocene sequence where we can easily study
the landscape evolution through geological times
(Fig. 2). It consists of mainly three types of sediments
from upper to the lower: loess–paleosol sequence, a red
clay sequence and sand.
The bottom of the sand bed is made up of 5–10 m
thick grayish-yellow, mica-rich, cross-bedded sand. The
lower part of the sand bed bears different fossils (ani-
mals, plants), sometimes between sandstone benches.
There are particularly numerous brown colored
gastropod internal clasts in this stratum. Many bone
fragments can be found like teeth, jaws, costae from
Hipparion sp., Mastodon sp. and Rhinoceros sp. (Fa-
bian et al. 2004a, b). The cross-bedded sand is overlain
by 2–4 m thick red clay horizon. The red clay (5YR 4/6)
has prismatic structure with slickenside, stress surfaces
and black and yellowish mottles. The lower part of the
red clay strata bears lots of large CaCO3 nodules. It is
covered by a 2–3 m thick loamy loess and recent soil.
The age of the recovered fossils is 6 Ma, but
unfortunately they are only facies indicators and not
persistent stratigraphic markers (Kovacs 2003).
Materials and methods
Red clay samples from the Pannonian Basin were
collected during the field observations. Many expo-
sures and outcrops were investigated in the basin. A
total of 50 samples were taken from the northern part,
from the southwestern and western part of Hungary.
All samples were kept in polythene bags and trans-
ferred to the laboratory for granulometric analyses.
The analyses were carried out at the university’s sedi-
ment lab. The grain-size distribution of all samples was
measured by laser diffraction (Fritsch Analysette 22)
methods according to the approach described by
Konert and Vandenberghe (1997). Laser particle sizers
can identify particle fractions with a higher resolution
than the sieve or pipette method. This instrument has
measurement ranges of 0.3–300 lm, thus giving 63
channels, in that order. After processing the samples
Fig. 1 Schematic mapshowing the sampling sites ofred clay sediments inHungary. Gray areas aremountains and hills. 1 Atkarsite; 2 Hatvan site; 3 Visontasite; 4 Mogyorod site; 5Szuliman site; 6 Cserdi site; 7Pecs-Postavolgy site; 8Beremend site; 9 Csarnotasite; 10 Bataszek and Batasite; 11 Szekszard site; 12 Pakssite; 13 Voros-to site; 14Csipkerek site
172 Int J Earth Sci (Geol Rundsch) (2008) 97:171–178
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with (10 ml, 30%) H2O2 and (10 ml, 10%) HCl to re-
move organic matter and carbonate, respectively,
10 ml of 0.05 N (NaPO3)6 was added to the sample,
which was then ultrasonicated for about 15 min. Next
the sample was transferred to the laser grain-size
analyzer.
Laser diffraction method enables the more accurate
calculation of the moment values of mean, mean
square deviation (MSD), skewness and kurtosis. We
use the sedimentological and statistical methods of Lu
et al. (2001) to present the eolian origin of the red clay.
Results
Grain-size distribution curves
The granulometric results are presented in Table 1.
The grain-size distribution curves demonstrate a pre-
dominantly bimodal character (Fig. 3). The >63 lm
(4F) fraction is almost insignificant in all the sedi-
ments except the fluvial sediments. The fine fraction is
clay-sized or very fine silt, while the coarser fraction is
medium to coarse silt and fine sand in fluvial sedi-
ments. However, the samples from the red clay, loess–
paleosol and fluvial sediments can be distinguished
rather easily from each other: the fine fraction is well
represented in the paleosol, lacustrine sediments and
a bit less in the red clay sediments, but progressively
less evident in the loess and fluvial sediments. The
grain-size distribution of the red clay is very similar to
the loess distribution. The modal size of the coarse
fraction gradually coarsens from the paleosols and
lacustrine sediments (ca. 6–9F) to the red clay
Fig. 2 Simplified geological profile of the Atkar sand pit (idealsection)
Table 1 Statistical parameters of grain-size distribution of thered clay, loess–paleosol, lacustrine and fluvial sediments (in phiunits)
Sample Mean MSD Skewness Kurtosis Y-value Sediment
Rc–RL 5.59 5.08 2.64 9.06 82.22 Red clayRc–Sz 4.84 4.73 2.14 6.07 65.88Rc–Cs 4.64 4.34 2.21 5.28 53.16Rc–S 4.70 4.37 2.71 8.10 61.52Rc–Ba 4.52 4.23 2.30 5.48 51.08Rc–R 5.49 5.35 2.68 10.98 96.85Rc–B 4.72 4.40 2.34 6.18 57.07Rc–H 3.99 3.70 1.46 0.85 27.46Rc–M 3.58 3.19 0.87 1.12 20.26Rc–P 5.51 5.63 1.49 2.89 83.64Rc–L 5.88 5.91 1.76 4.54 96.69Rc–Y 6.67 6.71 1.48 1.90 117.23L1 2.96 4.21 1.60 2.89 49.59 LoessL2 2.92 4.63 1.61 3.26 62.11L3 2.63 4.65 1.25 2.38 61.91P1 7.63 1.54 0.10 2.53 –12.27 PaleosolP2 7.71 1.46 0.15 2.62 –13.11P3 7.52 1.45 0.15 2.70 –12.27F1 5.37 1.85 1.27 4.01 1.21 FluvialF2 5.68 1.95 0.75 3.10 –0.48F3 5.90 1.90 0.80 2.90 –2.59LA1 7.30 16.00 0.10 0.04 760.19 LacustrineLA2 7.75 17.35 0.05 0.03 896.95LA3 6.98 18.86 0.07 0.03 1067.60
Rc–RL to Rc–Cs are the red clay samples from N Hungary; Rc–Sto Rc–M are the red clay samples from SW Hungary; Rc–P toRc–Y are the red clay samples from W Hungary; L1 to L3 are theloess samples; P1 to P3 are the paleosol samples; F1 to F3 are thefluvial sediment samples; LA1 to LA3 are the lacustrine sedi-ment samples from various sites
Int J Earth Sci (Geol Rundsch) (2008) 97:171–178 173
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(5–7F), loess (4–6F) and fluvial sediments (2–3F).
The lacustrine sediment is poorly sorted and has a
wide grain-size distribution range and very small
kurtosis values. Its grain-size distribution is noticeably
bimodal with a fine clay (8–10F) and a medium silt
fraction (5–6F). The red clay, loess, paleosols and
fluvial sediments also show bimodal character. In the
red clay, loess and paleosol, the coarser fraction is
located between 4 and 6F and the finer fraction be-
tween 7 and 9F. In the fluvial sediments it is between
2–3 and 4–6F. The red clay, loess and paleosols are
moderately sorted, while the fluvial sediment is well
sorted.
All the sediment types show positively skewed to
symmetric grain size-distribution, except the paleosol.
The positively skewed distribution indicates that the
finer fraction is included in the grain-size distribu-
tion. This asymmetry is expressed increasingly from
the red clay onward to the loess and to the fluvial
sediments.
According to Pye (1995), the fraction less then
2 lm (9F) may be formed partly by weathering
processes, and/or may be attributed to long distance
dust transport. Most of the particles are in the 2–
50 lm size range, which is typical eolian silt (Lu
et al. 2001). The lacustrine sediments are character-
ized by fine clay, which can be deposited only in
standing water. The bimodality of the fluvial sedi-
ment is explained by a combination of different
transport modes (Visher 1969). The particles of red
Fig. 3 Grain-size distribution curves of randomly selected red clay, loess, paleosol, lacustrine and fluvial sediment samples (for thesamples, see Table 1)
174 Int J Earth Sci (Geol Rundsch) (2008) 97:171–178
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clay finer than 9F are explained mainly as a weath-
ering product, while the particles coarser than 5Fwere transported mainly by dust storm. The particles
between 9 and 5F, the medium and fines silt frac-
tion, were possibly transported by average winds (Lu
et al. 2001).
These analyses demonstrate that the grain-size dis-
tribution of the red clay is similar to that of the loess
and is clearly different from that of the paleosols,
lacustrine and fluvial sediments. Moreover, the red clay
is slightly finer than the loess. This may show that a
weaker wind system transported the dust than that
which formed the red clay, and/or stronger post-
depositional weathering and pedogenesis (Lu et al.
2001; Kovacs 2003).
A–Md plot
A–Md ratios have been plotted in X–Y diagrams
(Fig. 4), in which A is the weight percentage of
particles finer than 4 lm and Md is the median
diameter in micrometres (Passega and Byramjee
1969). In this plot the red clay particle-size distri-
bution is different from the loess–paleosol sediments.
According to Lu et al. (2001) this plot alone cannot
separate samples from the different depositional
environments, and a combination of other grain-size
parameters is needed. The A–Md comparison is very
sensitive indicator of little differences between simi-
lar sediments like red clay and loess–paleosol. This
plot shows that the red clay is finer-grained than the
loess and paleosol sediments. The fine particles are
mainly explained as post-depositional weathering
products (Kovacs 2003).
MSD and skewness
Combined plots of mean, mean square deviation and
skewness are also typical indicators of sedimentary
environments (Folk 1966). These parameters have
been plotted for the red clay, loess, paleosols, fluvial
and lacustrine sediments in Fig. 5. The MSD of the red
clay is positioned close to those of the loesses and
paleosols, which are a little different from the lacus-
trine sediments and are rather different from the fluvial
sediments. The skewness of the red clay lies far to
those of the loesses, paleosols, lacustrine sediments and
the fluvial sediments. The red clay, loess–paleosol and
lacustrine sediments are well sorted, but the fluvial
sediments are poorly sorted. The skewness of the red
clay is very similar to that of the loess–paleosol. The
fine-grained fluvial and lacustrine sediments have
skewness near to zero.
Fig. 4 A–Md plot of the grain-size distribution of the red clay,loess and paleosol sediments
Fig. 5 MSD and skewness of the red clay, loess, paleosol,lacustrine and fluvial sediments as a function of mean grain size
Int J Earth Sci (Geol Rundsch) (2008) 97:171–178 175
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The partly overlapping fields of the red clay and
loess–paleosol populations that are seen in the MSD
and skewness plots may point to a similar origin.
Nevertheless, the overlaps in these plots point to that
the skewness and the MSD alone cannot separate
completely the sediments from different depositional
environments. According to Lu et al. (2001), the sedi-
ment transportation dynamics are not the only aspect
controlling the grain-size distributions of the sedi-
ments, because the material source, depositional
topography and even vegetation cover control the
sediment grain-size distribution. This shows that a
combination of numerous grain-size factors is needed
to study the origin of these deposits.
Empirical judgment equation
The empirical judgment equation (Y = –3.5688 M +
3.0716MSD2 – 2.0766 SK + 3.1175 K) is a statistical
method to differentiate between sediment population
using the grain-size distribution of numerous modern
eolian and other samples of which the depositional
environments are known (Sahu 1964). Y-value is an
index to distinguish the sedimentary environment.
The equation can be used to differentiate between
samples from eolian and other depositional environ-
ments (Sahu 1964). The calculated Y value of the red
clay ranges between 20 and 117, that of the loess 49–
62 and paleosol around –12, fluvial sediments from 1
to –2.59 and the lacustrine sediments from 760 to
1,067 (Fig. 6; Table 1). This illustrates that the Y
values of the red clay are close to those of the loess,
but are differ from those of paleosols, fluvial and
lacustrine sediments. In detail it comes out that the
Y value of the red clay is close to that of loess,
which indicates that the origin of the red clay is
wind-blown origin.
Discussion
The comparison of the grain-size distributions of the
red clay and the lacustrine sediments indicates quite
different sedimentary environments. Visible differ-
ences between the grain-size distributions of the red
clay and the fluvial sediments make obvious that the
red clay is unlikely to have had a fluvial origin. The
particle-size characteristics of the Neogene red clay
sediments are very similar to those of the Pleistocene
loess deposits, suggesting an eolian origin for the red
clay. A small amount of slight differences between the
grain-size distributions of these sediment groups,
however, indicate some differences in transport modes
and depositional environment. It appears from the
sedimentological data that the main part of the red clay
is of a wind-blown origin. The red clay was transported
by weak westerly winds and has been modified by post-
depositional alteration. What was the source of the red
clay? Local source was proposed by Smith et al. (1991)
for the loess and paleosols. The Late Miocene sedi-
ments within the Pannonian Basin are loosely consol-
idated sediments, which underlie the Great Hungarian
Plain. The Late Miocene sediments consist of marine
and shallow lacustrine deposits of conglomerates,
marls, sandstones, clays and sands (Ronai, 1985;
Schweitzer 1997; Magyar et al. 1999). Under suitably
arid–semiarid conditions and/or limited vegetation
cover, these sediments would provide a source of loose
granular material, which could be entrained by eolian
processes (Smith et al. 1991; Wright 2001). Recently it
has been held that the desertification of Pannonian
Basin corresponds to the Messinian Salinity Crisis
(Schweitzer 1997; Fabian et al. 2004a, b). The Late
Miocene or Messinian was a semiarid or semidesert
climatic period (Kretzoi 1987; Schweitzer 1997; Kovacs
2003; Fabian et al. 2004a, b). The climate of the Early
Pliocene was a transition between semidesert and
savannah. In that period Hipparion and Rhinoceros
lived in the Pannonian Basin (Fabian et al. 2004a, b).
The desert climate conditions are reconstructed from
the fossils (Meriones, etc.) and the pebbles covered by
desert varnish, which can be found in W. Hungary and
Pest Plain (Schweitzer 1997; Fabian et al. 2004a, b).
Laboratory experiments have demonstrated the possi-
bility that eolian reworking of the Messinian sands and
other similar deposits could theoretically contribute
material to the red clay, loess and loess-like deposits of
the Pannonian Basin (Smith et al. 1991; Kovacs 2003).
Fig. 6 Y-value of grain-size distribution of the red clay, loess,paleosols, fluvial and lacustrine sediments according to the‘empirical judgment equation’ of Sahu (1964). The Y-values ofthe lacustrine sediments are between 760 and 1,170
176 Int J Earth Sci (Geol Rundsch) (2008) 97:171–178
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Conclusions
We investigated red clay in order to better understand
their mode of formation. Field observations and labo-
ratory analyses of the red clay and the overlying
Pleistocene loess sequence demonstrate great similar-
ities in grain size, suggesting a wind-blown origin for
the Neogene red clay in the Pannonian Basin. The red
clay is mainly composed of two components: (1) a silt
fraction that is very similar to the silt fraction in the
Pleistocene loess, and (2) a rather abundant clay and
very fine silt fraction. The Neogene red clay accumu-
lated under persistent weak winds and a rather steady
warm-arid climate. Therefore, we infer that the clay
transporting wind came from the west, maybe from
central Europe, and we interpret these winds as driven
by the westerlies. The red clay has been modified by
post-depositional weathering under warm–humid cli-
mate. These environmental characteristics accompa-
nying the deposition and weathering of the red clay are
responsible particularly for the finer grain-size distri-
butions and lower dustfall rate than the overlying loess.
We conclude that the red clay in the Pannonian
Basin is of a wind-blown origin, and that it was con-
sequently affected by weathering processes in the Pli-
ocene. To date, the most important evidence for a
wind-blown origin comes from comparison of grain-
size data of the red clay and the overlying loess, al-
though several aspects of these data require further
analysis.
Acknowledgement The author would like to thank Professor F.Schweitzer, G. Szo}or and Thomas Voigt for their most helpfulcomments and reviews. I also thank my colleagues S.A. Fabianand G. Varga for the discussions and contribution during thefield work. I am grateful to J. Dezs}o (Sediment Lab) for helpingin grain-size analyses.
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