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    Quantum coherent transport in

    Meso- and Nanoscopic Systems

    Philippe [email protected]

    U of Arizona

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    General Literature:Electronic Transport in Mesoscopic Systems

    S. Datta, Cambridge Unversity Press, 1995(good, simple introduction)

    Introduction to Mesoscopic PhysicsY. Imry, Oxford University Press, 1997

    Mesoscopic Physics of Electrons and Photons

    E. Akkermans and G. Montambaux, Cambridge UniversityPress, 2007

    (a must if you want to enter the field and plan to stay)

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    Mesoscopic vs. nanoscopic physics

    Nanometer = length scale = 10-9mNanophysics = physics at the sub-micron length scale

    Mesoscopic physics = physics intermediate betweenmacroand micro

    That the humaneye can see

    Atomic level

    In what sense ?-> Phase-coherent nature of the electron matters!

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    Nanoscopic is entirely defined by length scales

    Mesoscopic is a regime (in a sense to be defined)

    Nanometer = length scale = 10-9mNanophysics = physics at the sub-micronic length scale

    Mesoscopic physics = physics intermediate betweenmacroand micro

    Corollary:

    The smallest, cleanest mesoscopic systems fall intothe class of nanoscopic systems

    Mesoscopic vs. nanoscopic systems

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    What is

    Mesoscopic Physics ?

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    system is INCOHERENT (no phase) use CLASSICAL MECHANICS

    V

    Conductivity : !=n e "/mConductance : G=!W/L

    2

    Solid-State Physics 101:Drude-Boltzmann Theory of Transport

    Electrons = point particles ; (charge,mass)=(-e,m)

    Metal is disordered uncorrelated collisions at impurities DIFFUSION

    ~Ohmic conductor with intensive conductivity

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    system is INCOHERENT (no phase) use CLASSICAL MECHANICS

    V

    Conductivity : !=n e "/mConductance : G=!W/L

    2

    Is this all ? Are there quantum corrections ?

    What happens once # is taken into account ?F

    Solid-State Physics 101:Drude-Boltzmann Theory of Transport

    Electrons = point particles ; (charge,mass)=(-e,m)

    Metal is disordered uncorrelated collisions at impurities DIFFUSION

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    Mesoscopic Physics - Length Scales

    # l L L$0L >> L %system is coherent !T-dependent!

    %use Quantum Mechanics !

    L >># %system is semiclassical

    %use small parameter # /L

    $

    F

    F

    F

    FermiWavelength

    Elastic MeanFree Path System Size

    CoherenceLength

    Between microscopic and macroscopic ; N. van Kampen 81

    Diffusive systems ~ lL

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    Some Mesoscopic Systems

    Webb 84 Heiblum 97

    Kouwenhoven 10

    van Wees 08

    Marcus 03

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    What is new in

    Mesoscopic Transport ?

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    Mesoscopic Physics : Novel Anomalous Properties I

    Nonlocality:

    Details of sample out of direct current path matter!!

    See: Washburn and Webb,

    Phys. Today 88

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    Sample-Specificity:

    Nonlocality + Sample Specificity:

    %Breakdown of Ohms Law

    G = !W/L%Look at conductance, not conductivity

    Samesamples, i.e. with same material

    & same fabrication, exhibit discrepancies

    in transport properties

    Mesoscopic Physics : Novel Anomalous Properties II

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    Dependence onsample geometry

    From: Ford et al., PRL 89

    Anomalous Hall Effect

    due to underlying

    classical dynamics

    Mesoscopic Physics : Novel Anomalous Properties III

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    Violationof macroscopic/classical symmetries

    E.g. Onsager 31:

    G(H)=G(-H)

    Dependence on measurement set-up

    From: Benoit et al., PRL 86

    Mesoscopic Physics : Novel Anomalous Properties IV

    Kobayashi et al., J. Phys. Soc. Jpn !02

    II I

    IVV V

    V=

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    Main Novel Fundamental Effects

    inQuantum Coherent Transport

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    Quantum Corrections to Transport I:Weak localization

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    Coherent Mesoscopic Corrections to Transport I:

    Weak Localization

    Th. : Gorkov, Larkin, Khmelnitskii, JETP Lett. 79

    Abrahams, Anderson, Ramakrishnan, PRL 79

    Rev.: Bergmann, Phys. Rep. 83; Lee and Ramakrishnan, RMP 85

    QM destructive interferences induce negative corrections

    to Drude conductivity

    Expansion in # /lIn 2D :

    F

    Fig. From : van den Dries et al., PRL 81

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    Coherent Mesoscopic Corrections to Transport I:

    Weak Localization - Quasiclassical Picture

    A B

    C

    !Break TRS - magnetic field

    !Probability to be at C:

    P(C) ~ |P+P| =2 |P| (1+cos[2&$/$0])22

    QM interferences disappear = positive magnetoconductance

    $

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    Weak Localization - Quasiclassical Picture

    A B

    C

    !Break TRS - magnetic field

    !Probability to be at C:

    P(C) ~ |P+P| =2 |P| (1+cos[2&$/$0])

    !Averaging over loop length/flux distribution

    22

    $

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    (Chang et al., PRL 94) (Chan et al., PRL 95)

    Trademark of Weak Localization - Magnetoresistance

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    Quantum Corrections to Transport II:Universal Conductance Fluctuations

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    Searching for Aharonov-Bohmoscillations in ring with L

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    Quantum Corrections to Transport III:Aharonov-Bohm effects

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    Sharvin and Sharvin 81

    ~Aharonov-Bohm oscillations

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    Magnetoresistance

    ~Aharonov-Bohm oscillations

    Measurement sample

    diam ~1m, width ~0.04m

    Amplitude of oscillations decreases

    with increasing temperature

    ~decoherence/dephasing

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    Quantum Corrections to Transport III:Conductance Quantization

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    [001][100]

    [010]

    two-dimensional

    electron gas

    (2DEG)

    quantum point contact

    (QPC)

    Quantization plateaux at

    multiples of G0=2e2/h

    Gate voltage ~ tunes width of QPvan Wees et al./Wharam et al. 88

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    Quantum Corrections to Transport IV:Coulomb Blockade

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    Electrons are verticallyConfined to 2DEG

    Electrons are laterallyConfined by gates

    Average conductance controlledby tuning opening of contacts

    [001][100]

    [010]

    two-dimensional

    electron gas

    (2DEG)

    What is a quantum dot ?

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    (Marcus lab.,

    Harvard)

    (Alhassid, RMP 01)

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    The two-slit experiment (textbook version)

    |'|2=|'1+'2|2

    1

    2

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    The two-slit experiment (non-textbook version)

    ?

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    The two-slit experiment (non-textbook version)

    Regular cavityChaotic cavity

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    "IS THIS DECOHERENCE ?

    "DO CHAOTIC / COMPLEX SYSTEMS DECOHERE

    WHEREAS REGULAR / INTEGRABLE SYSTEMS

    DO NOT ?

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    NO!It is multiple random scattering

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    The two-slit experiment (non-textbook version)

    Regular cavityChaotic cavity

    Despite multiple chaotic scattering

    the Gaussian envelope still exhibits

    (small) modulations !

    A.k.a. weak localization