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Research Article Radiation Transfer Calculations and Assessment of Global Warming by CO 2 Hermann Harde Experimental Physics and Materials Science, Helmut-Schmidt-University, Holstenhofweg 85, 22043 Hamburg, Germany Correspondence should be addressed to Hermann Harde; [email protected] Received 29 June 2016; Revised 3 October 2016; Accepted 1 November 2016; Published 20 March 2017 Academic Editor: Bin Yu Copyright ยฉ 2017 Hermann Harde. is is an open access article distributed under the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. We present detailed line-by-line radiation transfer calculations, which were performed under di๏ฌ€erent atmospheric conditions for the most important greenhouse gases water vapor, carbon dioxide, methane, and ozone. Particularly cloud e๏ฌ€ects, surface temperature variations, and humidity changes as well as molecular lineshape e๏ฌ€ects are investigated to examine their speci๏ฌc in๏ฌ‚uence on some basic climatologic parameters like the radiative forcing, the long wave absorptivity, and back-radiation as a function of an increasing CO 2 concentration in the atmosphere. ese calculations are used to assess the CO 2 global warming by means of an advanced two-layer climate model and to disclose some larger discrepancies in calculating the climate sensitivity. Including solar and cloud e๏ฌ€ects as well as all relevant feedback processes our simulations give an equilibrium climate sensitivity of = 0.7 โˆ˜ C (temperature increase at doubled CO 2 ) and a solar sensitivity of = 0.17 โˆ˜ C (at 0.1% increase of the total solar irradiance). en CO 2 contributes 40% and the Sun 60% to global warming over the last century. 1. Introduction e Fi๏ฌ…h Assessment Report (AR5) [1] of the Intergov- ernmental Panel on Climate Change (IPCC), a list of all abbreviations is found in the annex, announces new evidence of an anthropogenic climate change based on many inde- pendent scienti๏ฌc analyses from observations of the climate system, paleoclimate archives, theoretical studies of climate processes, and simulations using climate models. So, the IPCC classi๏ฌes the human in๏ฌ‚uence as extremely likely to be the dominant cause of the observed warming since the mid- 20th century (AR5-WG1-SPM-D3). Increasing emissions of carbon dioxide (CO 2 ) over the last century especially are made responsible for this change, and the equilibrium cli- mate sensitivity (ECS or ) as a measure for the Earthโ€™s temperature increase at doubled CO 2 concentration in the atmosphere is speci๏ฌed to be likely in the range 1.5 โˆ˜ C to 4.5 โˆ˜ C (high con๏ฌdence) (AR5-WG1-SPM, p16). Although in all these ๏ฌelds of climate sciences great progress has been achieved over the last decades and our knowledge about the Earth-atmosphere system (EASy) could signi๏ฌcantly be improved, explanations of the observed global warming over the last century in particular the anth- ropogenic contributions to this warming are still quite con- tradictorily discussed. All the more it is surprising (i) that many of the consulted analyses and also the AR5 itself do not better and clearly distinguish between an anthropogenic emission of CO 2 and a naturally generated part, where the latter even contributes more than 95% to the overall emission, and its generation rate and the respective absorption rate sensitively respond on global temperature variations; (ii) that the IPCC claims it would be extremely likely that more than half of the observed increase in global average surface temperature from 1951 to 2010 was caused by the anthropogenic increase in greenhouse gas concentrations and other anthropogenic forcings, while contributions from natural forcing and an internal variability both would only likely be in the range of โˆ’0.1 โˆ˜ C to 0.1 โˆ˜ C; (iii) that the meanwhile well known delayed response of CO 2 and methane (CH 4 ) to sea and air temperature changes (see, e.g., Petit et al. [2]; Monnin et al. [3]; Hindawi International Journal of Atmospheric Sciences Volume 2017, Article ID 9251034, 30 pages https://doi.org/10.1155/2017/9251034

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  • Research ArticleRadiation Transfer Calculations and Assessment ofGlobal Warming by CO2

    Hermann Harde

    Experimental Physics and Materials Science, Helmut-Schmidt-University, Holstenhofweg 85, 22043 Hamburg, Germany

    Correspondence should be addressed to Hermann Harde; [email protected]

    Received 29 June 2016; Revised 3 October 2016; Accepted 1 November 2016; Published 20 March 2017

    Academic Editor: Bin Yu

    Copyright ยฉ 2017 Hermann Harde. This is an open access article distributed under the Creative Commons Attribution License,which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.

    We present detailed line-by-line radiation transfer calculations, which were performed under different atmospheric conditionsfor the most important greenhouse gases water vapor, carbon dioxide, methane, and ozone. Particularly cloud effects, surfacetemperature variations, and humidity changes as well as molecular lineshape effects are investigated to examine their specificinfluence on some basic climatologic parameters like the radiative forcing, the long wave absorptivity, and back-radiation as afunction of an increasing CO2 concentration in the atmosphere. These calculations are used to assess the CO2 global warmingby means of an advanced two-layer climate model and to disclose some larger discrepancies in calculating the climate sensitivity.Including solar and cloud effects as well as all relevant feedback processes our simulations give an equilibrium climate sensitivity of๐ถ๐‘† = 0.7โˆ˜C (temperature increase at doubled CO2) and a solar sensitivity of ๐‘†๐‘† = 0.17โˆ˜C (at 0.1% increase of the total solar irradiance).Then CO2 contributes 40% and the Sun 60% to global warming over the last century.

    1. Introduction

    The Fifth Assessment Report (AR5) [1] of the Intergov-ernmental Panel on Climate Change (IPCC), a list of allabbreviations is found in the annex, announces new evidenceof an anthropogenic climate change based on many inde-pendent scientific analyses from observations of the climatesystem, paleoclimate archives, theoretical studies of climateprocesses, and simulations using climate models. So, theIPCC classifies the human influence as extremely likely to bethe dominant cause of the observed warming since the mid-20th century (AR5-WG1-SPM-D3). Increasing emissions ofcarbon dioxide (CO2) over the last century especially aremade responsible for this change, and the equilibrium cli-mate sensitivity (ECS or ๐ถ๐‘†) as a measure for the Earthโ€™stemperature increase at doubled CO2 concentration in theatmosphere is specified to be likely in the range 1.5โˆ˜C to 4.5โˆ˜C(high confidence) (AR5-WG1-SPM, p16).

    Although in all these fields of climate sciences greatprogress has been achieved over the last decades and ourknowledge about the Earth-atmosphere system (EASy) couldsignificantly be improved, explanations of the observedglobal warming over the last century in particular the anth-

    ropogenic contributions to this warming are still quite con-tradictorily discussed.

    All the more it is surprising

    (i) that many of the consulted analyses and also the AR5itself do not better and clearly distinguish betweenan anthropogenic emission of CO2 and a naturallygenerated part, where the latter even contributesmorethan 95% to the overall emission, and its generationrate and the respective absorption rate sensitivelyrespond on global temperature variations;

    (ii) that the IPCC claims it would be extremely likelythat more than half of the observed increase in globalaverage surface temperature from 1951 to 2010 wascaused by the anthropogenic increase in greenhousegas concentrations and other anthropogenic forcings,while contributions from natural forcing and aninternal variability both would only likely be in therange of โˆ’0.1โˆ˜C to 0.1โˆ˜C;

    (iii) that the meanwhile well known delayed response ofCO2 and methane (CH4) to sea and air temperaturechanges (see, e.g., Petit et al. [2]; Monnin et al. [3];

    HindawiInternational Journal of Atmospheric SciencesVolume 2017, Article ID 9251034, 30 pageshttps://doi.org/10.1155/2017/9251034

    https://doi.org/10.1155/2017/9251034

  • 2 International Journal of Atmospheric Sciences

    Caillon et al. [4]; Torn and Harte [5]; Humlum etal. [6]; Salby [7]) are not considered in AR5, andrespective consequences for an anthropogenic globalwarming are not discussed;

    (iv) that quite uncertain data about cloud feedbacks andstudies of the radiative forcing (RF) of greenhouse(GH) gases are referred, which are mostly valid forclear sky conditions, while the introduction of cloudsis usually omitted (AR5-WG1- Chap.8.3.1);

    (v) that the IPCC denies any noticeable solar influenceon the actual climate, although strong evidence of anincreasing solar activity over the last century exists(see, e.g., Hoyt & Schatten [8]; Willson & Mordvinov[9]; Shapiro et al. [10]; Ziskin & Shaviv [11]; Scafetta& Willson [12]; Usoskin et al. [13]; Zhao & Feng [14];Soon et al. [15]);

    (vi) that obviously important effects like convection andevaporation feedback, which can contribute to sig-nificant negative feedback (Harde-2014 [16]), are notconsidered in many analyses.

    Nevertheless, despite these deficits and simplifications themean equilibrium climate sensitivity is specified with highconfidence, and the GH gases are even assigned with veryhigh confidence (95%) to be responsible for the actual climatechanges.

    Here we will focus on the assessment of one of the mostimportant quantities in climate sciences and its validation,the ECS, which has to be scrutinized in more detail. Due toits far reaching consequences for future climate predictions itis particularly important to understand and to discover thelarge discrepancies between different accounting methodsapplied for this quantity. Also the weighting of some quitedifferent and even counteracting processes which controlour climate, but which are not always well understood,has carefully to be investigated with its implications on theclimate sensitivity. A quite critical report of actually publishedECS values and accounting methods expanded in AR5 hasbeen published by Lewis and Crok [17].

    In this contribution we will also retrace the main stepsof the IPCCโ€™s preferred accounting system and compare thiswith our own advanced two-layer climate model (2LCM),which is especially appropriate to calculate the influence ofincreasing CO2 concentrations on global warming as wellas the impact of solar variations on the climate (Harde-2014 [16]). This model describes the atmosphere and theground as two layers acting simultaneously as absorbers andPlanck radiators, and it includes additional heat transferbetween these layers due to convection and evaporation. Italso considers short wave (sw) and long wave (lw) scatteringprocesses at the atmosphere and at clouds; it includes allcommon feedback processes like water vapor, lapse rate,and albedo feedback but additionally takes into accounttemperature dependent sensible and latent heat fluxes aswell as temperature induced and solar induced cloud coverfeedback.

    The objective of our studies is not to present a new onlyโ€œtrue ECSโ€ but to identify some of the different assumptions

    and approximations with their far reaching consequencesin climate politics. It is without any doubt that the ECSis the most important measure for the CO2 influence onour climate, but it is also clear that this quantity does notdistinguish between anthropogenic and natural CO2 emis-sions. Therefore, as long as any natural variations in the CO2concentrations are not accurately known, the ECS cannot beused as a reliable indicator only for an anthropogenic globalwarming. All this in mind the reader may have his ownreservations about the published data for this measure andits significance for a man-made climate change.

    For the assessment of the ECS the IPCC favors theconcept of radiative forcing (RF), which is supposed tobe appropriate to describe the transition of the surface-troposphere system from one equilibrium state to anotherin response to an externally imposed perturbation. There-fore, in Section 2 we briefly outline some basic relationscharacterizing this concept, before we present in Section 3detailed line-by-line radiation transfer (LBL-RT) calculationsfor the lw up- and downwelling fluxes in the atmosphere (fordetails see Harde [16, 18, 19]), this for clear sky, global meancloud cover, full cloudiness, different surface temperatures,humidity, and even different lineshapes. These calculationswere performed for themost importantGHgaseswater vapor(WV), carbon dioxide, methane, and ozone and are basedon the HITRAN08 database [20]. Since the concentrationof the GH gases and the atmospheric pressure are changingwith temperature and altitude, the atmosphere has to besegmented into up to 228 sublayers from ground to 86 kmheight and in some cases additionally into three climatezones. When these computations are repeated for differentCO2 concentrations at otherwise same conditions, from thechanging fluxes on the one hand the CO2 initiated RF asthe main parameter for the IPCC accounting scheme and onthe other hand the sw and lw absorptivities as well as theback-radiated fraction of the atmospheric emission as the keyparameters in our 2LCM can be derived.

    Section 4 summarizes the main features of the 2LCM andits calibration to satellite data, for the radiation and heatfluxes using the well known radiation and energy budgetscheme of Trenberth et al. [21], for temperature changes dueto cloud cover variations applying the observationswithin theInternational Satellite Cloud Climatology Project (ISCCP)[22]. With the respective key parameters of Section 3 inte-grated in the climate model we simulate the Earthโ€™s surfacetemperature and the lower tropospheric temperature as afunction of the CO2 concentration.The temperature increaseat doubled CO2 concentration then directly gives the CO2climate sensitivity. Such simulations reproduce the direct orbasic ECS value (without feedback processes), as specifiedby the IPCC, within better than 10%. Significant differences,however, can be observed with the different feedback effectsincluded. Our investigations show the largest discrepanciesfor the WV and cloud feedback, but they also disclose theimportance of one of the primary stabilizers of the wholeclimate system, the evaporation feedback. Therefore, theseprocesses and their contributions are extensively analyzedunder different humidity, surface temperature, lapse rate, andcloud cover conditions.

  • International Journal of Atmospheric Sciences 3

    In particular, these studies show that the observed cloudchanges within the ISCCP cannot exclusively be explained bypure thermally induced cloud cover changes but obviously areadditionally controlled by a further cloud forcingmechanism.Since there exists strong evidence that the solar activityalso has a powerful influence on the cloud cover, it isreasonable to postulate such a solar induced cloud feedback(see, e.g., Svensmark [23]; Haigh [24]). This is investigatedin detail in Section 5, differentiating between a pure thermalimpact of an increasing solar activity and a nonthermallyinduced solar cloud feedback. An important criterion fora validation, which mechanism might control such cloudchanges, can be derived from model simulations, whichinclude the solar anomaly over the last century and comparethis directly with the observed global warming over thisperiod. These investigations indicate that due to the strongcloud feedback the observed warming over the last centurycan only satisfactorily be explained, attributing a significantfraction to the increased solar activity over this period (seealso Ziskin & Shaviv [11]; Vahrenholt & Luฬˆning [25]).

    Our simulations predict a solar contribution of about 60%and a CO2 induced contribution of 40% to global warmingover the last centurywith an equilibrium climate sensitivity of0.7โˆ˜C, which is almost a factor of five smaller than publishedin AR5.

    2. Radiative Forcing

    The concept of RF is well established in climate sciences andused to assess the global warming as a result of an externalperturbation of EASy (AR5-WG1-Chap.8). This perturbationcan result from solar anomalies, from increased GH gasconcentrations or volcanic activities. In all cases a directproportionality of the Earthโ€™s temperature increase ฮ”๐‘‡๐ธ asresponse to an external forcing ฮ”๐น is assumed in the form

    ฮ”๐‘‡๐ธ = ๐œ†๐‘† โ‹… ฮ”๐น, (1)with ๐œ†๐‘† as the climate sensitivity parameter, also known asPlanck sensitivity. The negative reciprocal of ๐œ†๐‘† is called thePlanck feedback (see AR5-WG1-Chap.9), although this is nota feedback process in the common sense like the water vapor,the albedo, or lapse rate feedback, which all describe aninternal amplification or attenuation of an external pertur-bation. The Planck feedback rather represents the change ofthe outgoing long wave radiation (OLR), or more preciselythe change of the total upwelling lw intensity ๐ผuptotal with theground temperature. Since an increasing amount ofOLRwiththe temperature causes a negative feedback for EASy, it can bedefined as the negative partial derivative as follows:

    โˆ’๐œ•OLR๐œ•๐‘‡๐ธ = โˆ’๐œ•๐ผuptotal๐œ•๐‘‡๐ธ =

    1๐œ†๐‘† . (2a)

    Its value, deduced as an average from different climatemodels, is given in AR5-WG1-Tab.9.5 as โˆ’3.2W/m2/โˆ˜C, and,thus, the Planck sensitivity becomes ๐œ†๐‘† = 0.31Wโˆ’1m2 โˆ˜C. Asomewhat simplified method to assess the Planck feedbackand sensitivity, which agrees within 15% with these values, is

    to use the slope of the Stefan-Boltzmann law at an effectiveEarth temperature ๐‘‡eff = 255K and emissivity ๐œ€eff = 1 with

    โˆ’๐œ•๐ผuptotal๐œ•๐‘‡๐ด

    ๐‘‡eff=255K= โˆ’4๐œ€eff๐œŽ๐‘‡3eff = โˆ’4๐ผ

    uptotal๐‘‡eff โ‡’

    1๐œ†๐‘† (2b)

    and to assume the same temperature response for the surfaceas for the atmosphere. This results in a Planck feedbackof โˆ’3.76W/m2/โˆ˜C and a climate sensitivity parameter ๐œ†๐‘†= 0.27Wโˆ’1m2 โˆ˜C. ๐œŽ is the Stefan-Boltzmann constant with5.67โ‹…10โˆ’8W/m2/โˆ˜C4 and ๐ผuptotal the OLR with 239.4W/m2.

    Eq. (1) is the basis for many climate models (see AR4[26] and AR5 [1]) and even for more complex mod-els like the Atmosphere-Ocean-General-Circulation Models(AOGCMs) this fundamental relation is used to expressthe influence of the growing GH gas concentrations on thesurface temperature. So, for these models and also for theobservationally based energy budget ECS estimates (see,e.g., Forster & Gregory [27]; Lindzen & Choi [28]) ฮ”๐นis a quite fundamental quantity, which cannot directly bemeasured but has to be deduced from extensive spectroscopiccalculations or solar data, which on their part rely on manyindividual observations and measurements. For quite actualinvestigations of ฮ”๐น see also Feldman et al. [29].

    In this context it should be noticed that alternativedefinitions of RF have been developed, each with its ownadvantages and limitations (see AR5-WG1-Chap.8). Herewe only consider the instantaneous RF, which refers to aninstantaneous change in the net (down minus up) radiativeflux (sw plus lw) due to an imposed change. This forcing isusually defined in terms of flux changes at the top of theatmosphere (TOA) or at the tropopause.

    In this contribution, particularly the influence of CO2on global warming is of interest. Therefore, in the nextsubsection we present some actual radiation transfer (RT)calculations, fromwhich the instantaneous RF due to increas-ing CO2 in the atmosphere and also some related quantities,which are of relevance for our two-layer climate model,can be derived. Since for these model calculations it is notsufficient only to consider the net radiative fluxes at thetropopause, neglecting the downwelling absorption changesin the troposphere and the upwelling absorption changes overthe stratosphere, we apply the RT concept from the surface toTOA and vice versa. The sw absorption changes over the fullatmosphere and this as a function of the CO2 concentrationcan be captured from our previous investigations (Harde-2014 [16]).

    As already outlined, an important reference for theinfluence of CO2 is the temperature increase at doubled CO2concentration under steady state conditions, which is knownas the equilibrium climate sensitivity ECS or ๐ถ๐‘†, and therespective lw forcing may be designated as ฮ”๐น2ร—CO2 . Since atTOA a lw downwelling flux is zero, the forcing at TOA can bedefined as difference of the total outgoing intensities ๐ผuptotal atsingle and doubled CO2 concentration ๐ถ:

    ฮ”๐น2ร—CO2 = ๐ผuptotal (๐ถ) โˆ’ ๐ผuptotal (2๐ถ) , (3)

  • 4 International Journal of Atmospheric Sciences

    where here we primarily consider the lw radiative forcing.๐ผuptotal can be explained to consist of the nonabsorbed terrestrialintensity (๐ผ๐ธ โˆ’ ๐ผabs) plus the emitted intensity of the atmo-sphere in upward direction ๐ผup๐ด ; thus, it holds the following:

    ฮ”๐น2ร—CO2 = ๐ผ๐ธ โˆ’ ๐ผabs (๐ถ) + ๐ผup๐ด (๐ถ) โˆ’ ๐ผ๐ธ + ๐ผabs (2๐ถ)โˆ’ ๐ผup๐ด (2๐ถ)

    = ฮ”๐ผup๐ด โˆ’ ฮ”๐ผabs(4)

    with

    ฮ”๐ผup๐ด = ๐ผup๐ด (๐ถ) โˆ’ ๐ผup๐ด (2๐ถ) ,ฮ”๐ผabs = ๐ผabs (๐ถ) โˆ’ ๐ผabs (2๐ถ) .

    (5)

    ๐ผ๐ธ is the intensity of the incident terrestrial radiation and ๐ผabsthe absorbed flux in the atmosphere.

    So, due to (4) this forcing generally consists of two con-tributions, the change in the upward atmospheric emissionand the change in the atmospheric absorption of terrestrialradiation, both as response to a doubling of the CO2 concen-tration.

    Expressing the downwelling atmospheric intensity ๐ผdown๐ดvia the total emitted intensity ๐ผtotal๐ด and the fraction๐‘“๐ด, whichis directed downward (also called asymmetry factor of theemitted atmospheric radiation) and which is generally foundfrom integrating the respective spectral intensities ๐ผup,down

    ๐ด,]ฬƒat TOA and the surface over the frequency or reciprocalwavelength (wavenumber) ]ฬƒ with

    ๐‘“๐ด = ๐ผdown๐ด

    ๐ผtotal๐ด =โˆซโˆž0๐ผdown๐ด,]ฬƒ ๐‘‘]ฬƒ

    โˆซโˆž0๐ผdown๐ด,]ฬƒ ๐‘‘]ฬƒ + โˆซโˆž0 ๐ผup๐ด,]ฬƒ๐‘‘]ฬƒ

    , (6)

    the difference ฮ”๐ผdown๐ด between single and doubled concentra-tion gives

    ฮ”๐ผdown๐ด = ๐ผdown๐ด (๐ถ) โˆ’ ๐ผdown๐ด (2๐ถ)= ๐ผtotal๐ด (๐ถ) โ‹… ๐‘“๐ด (๐ถ) โˆ’ ๐ผtotal๐ด (2๐ถ) โ‹… ๐‘“๐ด (2๐ถ)= ๐ผtotal๐ด (๐ถ) โ‹… ๐‘“๐ด (๐ถ) โˆ’ (๐ผtotal๐ด (๐ถ) โˆ’ ฮ”๐ผtotal๐ด )โ‹… (๐‘“๐ด (๐ถ) โˆ’ ฮ”๐‘“๐ด)

    = ๐ผtotal๐ด (๐ถ) โ‹… ฮ”๐‘“๐ด + ฮ”๐ผtotal๐ด โ‹… ๐‘“๐ด (๐ถ) โˆ’ ฮ”๐ผtotal๐ดโ‹… ฮ”๐‘“๐ด,

    (7)

    with ฮ”๐ผtotal๐ด and ฮ”๐‘“๐ด as the respective differences of ๐ผtotal๐ด and๐‘“๐ด at single and doubled CO2 concentration.

    Then, with (7), for the difference of the upwelling atmo-spheric intensities we can write

    ฮ”๐ผup๐ด = ๐ผtotal๐ด (๐ถ) โ‹… (1 โˆ’ ๐‘“๐ด (๐ถ)) โˆ’ ๐ผtotal๐ด (2๐ถ)โ‹… (1 โˆ’ ๐‘“๐ด (2๐ถ))

    = ๐ผtotal๐ด (๐ถ) โˆ’ ๐ผtotal๐ด (2๐ถ) โˆ’ ๐ผtotal๐ด (๐ถ) โ‹… ๐‘“๐ด (๐ถ)+ ๐ผtotal๐ด (2๐ถ) โ‹… ๐‘“๐ด (2๐ถ)

    = ฮ”๐ผtotal๐ด โˆ’ ๐ผtotal๐ด (๐ถ) โ‹… ฮ”๐‘“๐ด โˆ’ ฮ”๐ผtotal๐ด โ‹… ๐‘“๐ด (๐ถ)+ ฮ”๐ผtotal๐ด โ‹… ฮ”๐‘“๐ด

    = ฮ”๐ผtotal๐ด โ‹… (1 โˆ’ ๐‘“๐ด (๐ถ) + ฮ”๐‘“๐ด) โˆ’ ๐ผtotal๐ด (๐ถ) โ‹… ฮ”๐‘“๐ด,

    (8)

    and the radiative forcing at doubled CO2 concentration canfinally be expressed as follows:

    ฮ”๐น2ร—CO2 = ฮ”๐ผtotal๐ด โ‹… (1 โˆ’ ๐‘“๐ด (๐ถ) + ฮ”๐‘“๐ด) โˆ’ ๐ผtotal๐ด (๐ถ)โ‹… ฮ”๐‘“๐ด โˆ’ ฮ”๐ผabs.

    (9)

    This CO2 forcing can directly be derived from radiationtransfer calculations (Schwarzschild [30, 31]; Goody andYung [32]; Salby-2012 [33]; Harde-2013 [18]; Harde-2014 [16]),by which the up- and downwelling fluxes as well as theabsorption and emission in the atmosphere are computed.

    3. Radiation Transfer Calculations

    Since it is obvious that the cloud cover has a strong influenceon the up- and downwelling fluxes in the atmosphere and alsoon the strength of the GH effect, we have performed line-by-line radiation transfer (LBL-RT) calculations under differentcloudiness conditions, ground temperatures, and humidity toevaluate the influence of CO2 on global warming. We alsobriefly investigate the influence of lineshape effects on RTcalculations and their consequences for the ECS.

    Here we only present global RT calculation with averagedvalues for the temperature, water vapor concentration, andan average lapse rate, since separate computations for thetropics mid- and high-latitudes with individual profiles andaveraging over the climate zoneswith an areaweighting factorgave almost the same results (see also Harde [16]).

    3.1. Clear Sky at Global Mean Temperature. Table 1 shows theresults of our LBL calculations under clear sky conditionsas a function of the CO2 concentration, using a groundtemperature of๐‘‡๐ธ = 289.15 K = 16โˆ˜C and a terrestrial intensityof ๐ผ๐ธ = 396W/m2.These values are consistent with those usedby Trenberth et al. [21].

    As an average over the three climate zones thewater vaporconcentration at ground was assumed to be 14,615.3 ppmand decreasing with altitude due to the Clausius-Clapeyronequation (for details see Harde-2014 [16]). These data havebeen derived from satellite measurements (Vey [34]) andare almost a factor of two larger than those given by the

  • International Journal of Atmospheric Sciences 5

    Table 1: RT-calculations for different CO2 concentrations at clear sky (๐ผ๐ธ = 395.78W/m2, ๐‘‡๐ธ = 289.15 K, water vapor at ground: 14615.3 ppm,CH4: 1.8 ppm, and O3 varying over the stratosphere with a maximum concentration of 7 ppm).

    CO2ppm

    ๐ผuptotalW/m2

    ๐ผup๐ดW/m2

    ๐ผdown๐ดW/m2

    ๐ผtotal๐ดW/m2

    ๐ผabsW/m2

    aLW%

    ๐‘“๐ด%

    0 290.72 201.03 283.40 484.43 303.09 77.06 58.5035 272.70 194.92 295.40 490.32 315.00 80.08 60.2570 269.62 193.96 297.54 491.50 317.13 80.62 60.54140 266.26 193.22 300.08 493.30 319.75 81.29 60.83210 264.08 192.86 301.08 493.94 321.57 81.75 60.95280 262.40 192.64 303.16 495.80 323.02 82.12 61.15350 261.01 192.50 304.31 496.81 324.27 82.44 61.25380 260.48 192.45 304.75 497.20 324.76 82.57 61.29420 259.81 192.41 305.32 497.73 325.38 82.72 61.34490 258.75 192.36 306.23 498.59 326.40 82.98 61.42560 257.78 192.34 307.08 499.42 327.34 83.22 61.49630 256.90 192.35 307.86 500.21 328.23 83.45 61.55700 256.08 192.37 308.60 500.97 329.07 83.66 61.60760 255.42 192.40 309.21 501.61 329.76 83.84 61.64380โ€“760 5.06 0.05 โˆ’4.46 โˆ’4.41 โˆ’5.00 โˆ’1.27 โˆ’0.35ฮ”๐ผup๐ด โˆ’ ฮ”๐ผabs 5.05

    US Standard Atmosphere [35]. But they are in quite goodagreement with the Average Global Atmosphere (Ollila [36]),which even specifies values 12% larger than ours. The CH4concentration was set to 1.8 ppm and O3 to vary over thestratosphere with a maximum concentration of 7 ppm at38 km altitude. The lapse rate and pressure variation withaltitude agree with the US Standard Atmosphere.

    Our calculations cover a spectral interval from 10 to2500 cmโˆ’1, corresponding to 99.86% of a Planck radiator at๐‘‡๐ธ, and they include more than 78,000 lines with spectralintensities larger 10โˆ’24 cmโˆ’1/(moleculesโ‹…cmโˆ’2). The spectralresolution for calculations at CO2 concentrations of 380and 760 ppm, which are used as reference data, was chosenas 0.07 cmโˆ’1 (2.2 GHz), and for the vertical direction 228sublayers were distinguished, whereas the calculations at theother concentrations were performed with half the spectraland vertical resolution.

    Comparison of the two last values in column 2 of Table 1shows that within rounding errors (9) is well confirmed.Looking at the upwelling intensity ๐ผup๐ด of the atmosphere (col-umn 3) we see that this is almost identical at single and dou-bled CO2 concentration, while the downwelling part ๐ผdown๐ด(column 4) and the total atmospheric radiation ๐ผtotal๐ด (column5) both are increasing by more than 4.4W/m2. This meansthat at clear sky conditions most of the additionally absorbedterrestrial radiation at doubled CO2 (see column 6) is instan-taneously directed back to the surface, and only a relativelysmall contribution of 0.6W/m2 is trapped in the atmosphere.

    Since in this case the first two terms in (9) almost exactlycompensate each other, the forcing under clear sky conditionsis in good approximation only determined by the absorptiondifference. Thus, from the simple radiative forcing model (1)it follows that also the ground temperature variations arealmost only determined by this additionally absorbed power.

    In general, however, it should be clear that the surfacetemperature also depends on the emission characteristic ofthe atmosphere, which changes with the GH gas concentra-

    fA clear skylog ๏ฟฝt fA

    aLW clear skylog ๏ฟฝt aLW

    84

    82

    80

    78

    76

    74

    72

    64

    63

    62

    61

    60

    59

    58

    CO2-concentration (ppm)

    fA

    (%)

    8007006005004003002001000

    a LW

    (%)

    Figure 1: Lw absorptivity aLW (black diamonds) and downwellingfraction๐‘“๐ด of emitted atmospheric radiation (blue triangles) at clearsky with respective logarithmic approximations.

    tion as well as with the cloud cover and is determined by thefirst two terms in (9). Only under clear sky they just feedmostof the additionally absorbed power back to the surface.

    In a more advanced model, as this will be discussed laterwith a radiation and energy balance at TOAand at the surface,including heat fluxes of sensible and latent heat or fromneighbouring climate zones, as well as sw and lw absorptionlosses, even at clear sky conditions the atmospheric emissioncharacteristic is of relevance, which can well be representedby the fraction ๐‘“๐ด of the downward emitted radiation.

    The relative absorption of terrestrial radiation by the GHgases and its variation with increasing CO2 concentration arelisted in column 7. It is normalized to the incident terrestrialflux and in this way represents the lw absorptivity aLW asdefined in Harde-2014 [16] (4). This absorptivity is repre-sented in Figure 1 (black diamonds) together with the back-radiated fraction ๐‘“๐ด of the atmosphere (blue triangles). Athigher concentrations both quantities canwell be represented

  • 6 International Journal of Atmospheric Sciences

    Table 2: RT-calculations for CO2 concentrations of 380 and 760 ppm at a surface temperature of 20.3โˆ˜C (293.45 K) and clear sky (๐ผ๐ธ =

    420W/m2, water vapor at ground: 18,353.2 ppm, CH4 of 1.8 ppm and O3 varying over the stratosphere with a maximum concentration of7 ppm).

    CO2ppm

    ๐ผuptotalW/m2

    ๐ผup๐ดW/m2

    ๐ผdown๐ดW/m2

    ๐ผtotal๐ดW/m2

    ๐ผabsW/m2

    aLW%

    ๐‘“๐ด%

    380 270.22 203.99 334.02 538.01 353.52 84.08 62.08760 264.76 203.31 338.34 541.65 358.30 85.22 62.46ฮ” 5.46 0.68 โˆ’4.32 โˆ’3.64 โˆ’4.78 โˆ’1.14 โˆ’0.38

    by logarithmic graphs (magenta line for aLW, green line for๐‘“๐ด), indicating that due to saturation effects then only the farwings will further contribute to an increasing absorption oremission.

    3.2. RT Calculations at Clear Sky and Increased Surface Tem-perature. Whereas the above calculations reflect a somewhatartificial situation, assuming clear sky and a global meantemperature of 16โˆ˜C, we know that with declining cloud coverthe average surface temperature is significantly climbing up.So, fromobservationswithin the International Satellite CloudClimatology Project (ISCCP) [22] it is found that aroundthe global mean cloud cover of 66% a reducing cloudinessof 1% causes a temperature increase of about 0.06โ€“0.07โˆ˜C, atendency which is also confirmed by data of Hartmann [37].

    Therefore, to get a better understanding of how suchhigher temperature modifies the respective fluxes in theatmosphere and especially this affects the CO2 radiativeforcing, we have performed additional calculations for asurface temperature of 20.3โˆ˜C. At this temperature and asurface emissivity of 100% the terrestrial radiation climbsup to 420W/m2. But with the higher temperature also thehumidity increases and therefore affects the absorptivity oftheGHgases. From themeasuredwater vapor concentrationsas well as the temperatures atmid-latitudes and the tropics wededuce at the higher temperature a growth of the vapor con-centration of 3,738 ppm with a new total mean concentrationnear the surface of 18,353 ppm.

    Calculations for this higher ground temperature andwater vapor concentration are shown in Table 2.

    Since for an evaluation of CO2 with its influence on theradiation budget it is sufficient to concentrate on the fluxes atsingle and doubled CO2 concentration, here we only presentthis reduced data set. Compared to the lower temperaturecalculations the radiative forcing increases by 0.4W/m2,which is mainly due to changes in the upward atmosphericemissionwithฮ”๐ผup๐ด = 0.7W/m2, while the absorption changeswithฮ”๐ผabs = โˆ’4.8W/m2 are even getting slightly smaller. Alsothe downward directed flux change withฮ”๐ผdown๐ด = โˆ’4.3W/m2and the total atmospheric emission change with ฮ”๐ผtotal๐ด =โˆ’3.6W/m2 are reducing, although the absolute fluxes andthe absorption are considerably larger, caused by the highertemperature and water vapor.

    The absorptivity as calculated under these modifiedconditions is shown in Figure 2 (black diamonds) togetherwith the back-radiated fraction ๐‘“๐ด of the atmosphere (bluetriangles). At higher CO2 concentrations both graphs can

    fA clear skylog ๏ฟฝt fA

    aLW clear skylog ๏ฟฝt aLW

    84

    86

    82

    80

    78

    76

    74

    72

    64

    63

    62

    61

    60

    59

    58

    CO2-concentration (ppm)

    fA

    (%)

    8007006005004003002001000a L

    W(%

    )

    Figure 2: Lw absorptivity aLW (black diamonds) and downwellingfraction ๐‘“๐ด of atmospheric radiation at ๐‘‡๐ธ = 20.3โˆ˜C and clear skywith respective logarithmic approximations.

    again well be approximated by logarithmic functions, similarto Figure 1 (magenta line for aLW, green line for ๐‘“๐ด), only onslightly shifted scales.

    3.3. LBL-RTCalculations at GlobalMeanCloudCover. Underregular cloud cover significant changes from clear sky condi-tions have to be expected for the up- and downwelling fluxesdue to the strong shielding effect of clouds not only for sw butalso for lw radiation. In our radiation transfer calculationsthe clouds are considered as a single thinner layer, whichabsorbs the incident lw radiation from up or down directionwith a cloud absorptivity aLC and which has a transmissivityof 1 โˆ’ aLC, while lw scattering processes at the clouds arehere neglected. For the RT calculation only the resultingattenuation of radiation, which passes the layer, is of rele-vance, and for these calculations it is sufficient to express thetotal attenuation uniformly only by one parameter, the cloudabsorptivity. In addition to the transmitted radiation theclouds are also emitting as a Planckian radiator with an emis-sivity ๐œ€LC and a temperature determined by the cloud altitude.

    The Global Energy and Water Cycle Experiment(GEWEX) Radiation Panel, which compares the availableglobal long-term cloud data products with the ISCCPand consists of 12 satellite measurement teams, specifiesthe global total cloud amount between 56% and 74%(Stubenrauch et al. [38]), where this relatively wide rangeis mainly explained by different instrument sensitivity andby retrieval methodology. For our further calculations weassume a global mean cloud cover of ๐ถ๐ถ = 66% in agreement

  • International Journal of Atmospheric Sciences 7

    Table 3: RT-calculations for different CO2 concentrations at mean cloud cover of 66%, a cloud altitude of 5.1 km, and cloud emissivity of 63%(๐ผ๐ธ = 396W/m2, ๐‘‡๐ธ = 289.15 K = 16.0โˆ˜C, water vapor at ground of 14,615.3 ppm, CH4 of 1.8 ppm, and O3 varying over the stratosphere with amaximum concentration of 7 ppm).

    CO2ppm

    ๐ผuptotalW/m2

    ๐ผup๐ดW/m2

    ๐ผdown๐ดW/m2

    ๐ผtotal๐ดW/m2

    ๐ผabsW/m2

    aLW%

    ๐‘“๐ด%

    0 262.82 210.01 308.62 518.63 342.97 79.34 59.5135 248.31 202.49 317.89 520.38 349.96 81.09 61.0970 245.88 201.31 319.57 520.88 351.21 81.40 61.35140 243.24 200.22 321.55 521.77 352.76 81.78 61.63210 241.49 199.49 322.83 522.32 353.78 82.05 61.81280 240.21 199.08 323.89 522.97 354.64 82.29 61.93350 239.62 199.26 326.14 525.40 355.41 82.49 62.07380 239.22 199.22 326.49 525.71 355.77 82.57 62.10420 238.72 199.01 326.93 525.94 356.06 82.67 62.16490 237.92 198.80 327.64 526.44 356.66 82.83 62.24560 237.20 198.64 328.29 526.93 357.21 82.97 62.30630 236.54 198.50 328.90 527.40 357.74 83.10 62.36700 235.93 198.38 329.47 527.85 358.23 83.21 62.42760 235.45 198.38 329.94 528.32 358.70 83.31 62.45ฮ” 3.77 0.84 โˆ’3.45 โˆ’2.61 โˆ’2.93 โˆ’0.74 โˆ’0.35ฮ”๐ผup๐ด โˆ’ฮ”๐ผabs 3.77

    with the ISCCP [22]. The cloud altitude with โ„Ž๐ถ = 5.1 kmand the emissivity with ๐œ€LC = 63% were chosen to almostexactly reproduce the widely accepted radiation and energybudget scheme of Trenberth et al. [21] (hereafter calledTFK-scheme) with a total upward flux of ๐ผuptotal = 239.2W/m2and a nonabsorbed outgoing radiation from the surface with๐ผuptotal โˆ’ ๐ผup๐ด = 40W/m2.

    Our RT calculations under otherwise identical conditionsas described in Section 3.1 and at a surface temperature ๐‘‡๐ธ =16โˆ˜C are listed in Table 3. They show significant changes tothe radiation fluxes under clear sky, for example, for ๐ผdown๐ด ,more than 20W/m2 or for ๐ผtotal๐ด even 28W/m2. Also thetotal absorption, now additionally increased by the clouds, is31W/m2 larger than at clear sky.

    But respective differences between single and doubledCO2 concentrations, which are here of main interest, ingeneral are getting smaller. So, the radiative forcing reducesto ฮ”๐น2ร—CO2 = 3.77W/m2 and is almost identical with thefigure used by the IPCC (Myhre et al. [39]), although here weconsider only the instantaneous lw RF at TOA. This forcingis the result of the upwelling atmospheric contribution ofฮ”๐ผup๐ด = 0.84W/m2 and on the other hand a reducedabsorption difference of ฮ”๐ผabs = โˆ’2.93W/m2 compared toโˆ’5W/m2 at clear sky. Also changes in the back-radiationdiminish from โˆ’4.5W/m2 to ฮ”๐ผdown๐ด = โˆ’3.5W/m2 and thetotal emission even from โˆ’4.4W/m2 to ฮ”๐ผtotal๐ด = โˆ’2.6W/m2.

    Because of this smaller alteration in the atmosphericemission the 1st term in (9) with ฮ”๐ผtotal๐ด โ‹… (1 โˆ’ ๐‘“๐ด(๐ถ) + ฮ”๐‘“๐ด)now reduces to โˆ’0.99W/m2, whereas the 2nd term withโˆ’๐ผtotal๐ด (๐ถ)โ‹…ฮ”๐‘“๐ด = 1.83W/m2 dominates. From the total forcingof 3.77W/m2 in this case 3.45W/m2 goes back to the surface,while 0.32W/m2 remains in the atmosphere.

    To deduce the lw absorptivity at cloudiness from the radi-ation transfer calculations, the absorbed intensity listed in

    fA 66% cloudslog ๏ฟฝt fA

    aLW 66% cloudslog ๏ฟฝt aLW

    83

    81

    79

    77

    75

    63

    62

    61

    60

    59

    CO2-concentration (ppm)

    fA

    (%)

    8007006005004003002001000

    a LW

    (%)

    Figure 3: Lw absorptivity aLW (black diamonds) and downwellingfraction ๐‘“๐ด of emitted atmospheric radiation at 66% cloud coverwith respective logarithmic approximations.

    column 6 of Table 3, which now reflects the total absorptioncaused by the GH gases and the clouds, has to be reducedby the cloud fraction. Such correction seems appropriate fora direct comparison of the absorptivity changes caused bythe GH gases at clear sky and clouds, and it is necessary forour two-layer climate model, where the cloud absorption isalready integrated in themodel and represented by respectiveparameters. Such a correction is done by comparing theabsorption, for example, at 380 ppm with and without cloudsat the same ground temperature, and reducing column 6 bythis difference. Normalizing the corrected absorption to theincident radiation then gives in good approximation the lwabsorptivity aLW of the GH gases in the presence of clouds.

    Figure 3 shows the respective absorptivity aLW (blackdiamonds) and the back-radiated fraction ๐‘“๐ด (blue triangles)at a cloud cover of 66%. Again both quantities can well be

  • 8 International Journal of Atmospheric Sciences

    Table 4: RT-calculations with MRT lineshape for CO2 concentrations of 380 and 760 ppm at mean cloud cover of 66%, a cloud altitude of6.0 km, and cloud emissivity of 47.8% (๐ผ๐ธ = 396W/m2, ๐‘‡๐ธ = 289.15 K = 16.0โˆ˜C, water vapor at ground of 14,615.3 ppm, CH4 of 1.8 ppm, and O3varying over the stratosphere with a maximum concentration of 7 ppm).

    CO2ppm

    ๐ผuptotalW/m2

    ๐ผup๐ดW/m2

    ๐ผdown๐ดW/m2

    ๐ผtotal๐ดW/m2

    ๐ผabsW/m2

    aLW%

    ๐‘“๐ด%

    380 239.47 199.48 329.41 528.89 355.78 89.77 62.28760 235.68 198.50 332.59 531.09 358.60 90.48 62.62ฮ” 3.79 0.98 โˆ’3.18 โˆ’2.20 โˆ’2.82 โˆ’0.71 โˆ’0.34

    represented by logarithmic graphs (magenta line for aLW,green line for ๐‘“๐ด). While ๐‘“๐ด slightly increases by 0.8%,ฮ”๐‘“๐ด remains constant. However, the absorptivity changesalmost decline by a factor of two to โˆ’0.74% at doubled CO2concentration.

    Simulations at higher cloud altitudes under otherwisesame constrains give a reduced upwelling flux ๐ผuptotal and afurther diminishing radiative forcing ฮ”๐น2ร—CO2 .3.4. RT Calculations with MRT Lineshape. While the pre-ceding calculations are based on the standard molecularcollision theory, considering collisional broadening of spec-tral transitions, which are characterized by a Lorentzianlineshape or at higher altitudes also by a Voigt profile, wehave also performed extensive calculations using a moresophisticated lineshape as given by the molecular responsetheory (MRT) (Harde et al. [40โ€“44]). This theory representsa generalization and unification of the classical collisiontheories of Lorentz and on the other hand of van Vleck andWeisskopf, considering thermalization of molecules during acollision, which in its limit is determined by the reciprocal ofthemolecular transition frequency and controlled byHeisen-bergโ€™s uncertainty principle (Harde & Grischkowsky [44]).The specialty applying MRT is that it not only describes thenear resonance absorption and emission behavior as alreadyadequately characterized by a Lorentzian, but also reflects thefar wing response, which is mainly caused by the ultrafasttime response ofmolecules to an external electric field duringcollisions. So, the MRT lineshapes already represent verywell the continuum water vapor absorption extending upto 1200 cmโˆ’1 and caused by the low frequency water vaporabsorption band around 200 cmโˆ’1 (see Burch & Gryvnak[45]; Roberts et al. [46]).

    This continuum water vapor background together withthe far wing contributions of the othermolecules significantlymodifies the absolute up- and downwelling fluxes. Therefore,to further satisfy the radiation and energy balance of theTFK-scheme, in the radiation transfer calculations the cloud alti-tude has to be increased to 6 km and the cloud absorptivity =emissivity reduced to 47.8%.

    The results of such a calculation at a mean cloud coverof 66% and at otherwise same conditions as described inSection 3.3 is shown in Table 4. To compare the alterationscaused by doubling the CO2 concentration it is again suffi-cient only to display the calculations for 380 and 760 ppmCO2. It is interesting to see that the more sophisticatedlineshape and the continuum background absorption almost

    have no influence on ฮ”๐น2ร—CO2 , the RF at doubled CO2, whichagrees within better than 1% with the simpler calculationsshown in Table 3, neglecting the continuum absorption andusing a Lorentzian lineshape. Also changes in the otherfluxes at doubled CO2 concentration are consistent within0.1W/m2; only the back-radiation changes to ฮ”๐ผdown๐ด =โˆ’3.18W/m2 and is about 0.3W/m2 smaller; thus, the powerleft in the atmosphere increases by this amount.

    For this insensitivity to a different collision and line-shape theory we see three main reasons: first, because ofthe larger absolute flux variations, caused by the differentwing absorption and WV continuum, the outgoing fluxeswere recalibrated to the TFK-scheme via cloud altitudeand absorptivity to ensure comparable absolute fluxes inagreement with the observations. Second, we only considerflux differences at single and doubled CO2 concentration forthe same shape, so that discrepancies to another shape arenot directly observed and smaller absolute variations with theCO2 concentration are to some extent cancel out. Third, theinterference of the CO2 spectrum with strong water vaporlines and the underlying WV continuum further attenuatesany CO2 lineshape effects.

    So, calculations based on the classical collision theoryobviously reproduce quite reliable data of any radiationchanges in the atmosphere. Since the far wings of the CO2lines are found to decay more rapidly than a Lorentzian andthus should contribute less to the total absorption (see, e.g.,Edwards and Strow [47]), such calculations even simulateslightly worse conditions and result in a more conservativeassessment of global warming by CO2. For actual CO2 line-shape studies see also Happer [48], and for RT calculationsincluding CO2 linemixing seeMlynczak et al. [49], andOzaket al. [50].

    3.5. RT Calculations for Total Cloud Cover. With a furtherincreasing cloud cover and thus a stronger shielding of thesw radiation also the surface temperature further drops, andowing to the ISCCP observations at 100% cloudiness thena reduced temperature of approximately 2.2โˆ˜C compared tomean cloudiness is expected.

    Respective radiation transfer calculations at 100% cloudcover, a surface temperature of 13.8โˆ˜C with a terrestrialintensity of 384W/m2, and a further reduced water vaporconcentration at ground of 12,703 ppm, otherwise using thesame conditions as in Section 3.3, are shown in Table 5.The total outgoing radiation ๐ผuptotal drops by 15.4W/m2 andthe total atmospheric emission ๐ผtotal๐ด by 6.6W/m2 compared

  • International Journal of Atmospheric Sciences 9

    Table 5: RT-calculations for different CO2 concentrations at 100% cloudiness, a cloud altitude of 5.1 km, and cloud emissivity of 63%(๐ผ๐ธ = 384W/m2, ๐‘‡๐ธ = 286.95 K = 13.8โˆ˜C, water vapor: 12,702.9 ppm, CH4: 1.8 ppm, and O3 varying over the stratosphere with a maximumconcentration of 7 ppm).

    CO2ppm

    ๐ผuptotalW/m2

    ๐ผup๐ดW/m2

    ๐ผdown๐ดW/m2

    ๐ผtotal๐ดW/m2

    ๐ผabsW/m2

    aLW%

    ๐‘“๐ด%

    380 223.80 197.75 321.34 519.09 357.86 81.55 61.90760 220.84 196.72 324.27 520.99 359.79 82.05 62.24ฮ” 2.96 1.03 โˆ’2.93 โˆ’1.90 โˆ’1.93 โˆ’0.50 โˆ’0.34

    fA 100% cloudslog ๏ฟฝt fA

    aLW 100% cloudslog ๏ฟฝt aLW

    82

    81

    80

    79

    77

    78

    63

    64

    62

    61

    60

    59

    CO2-concentration (ppm)

    fA

    (%)

    8007006005004003002001000

    a LW

    (%)

    Figure 4: Lw absorptivity aLW (black diamonds) and downwellingfraction ๐‘“๐ด (blue triangles) of emitted atmospheric radiation at100% cloudiness and a ground temperature of 13.8โˆ˜Cwith respectivelogarithmic approximations.

    to a cloud cover of 66%. Nevertheless, the forcing due todoubled CO2 reduces to ฮ”๐น2ร—CO2 = 3.0W/m2, consisting ofa slightly increasing contribution ฮ”๐ผup๐ด = 1.0W/m2 and adecreasing absorption ฮ”๐ผabs = โˆ’1.9W/m2. Also the absolutedownwelling radiation ๐ผdown๐ด further decreases by 5.2W/m2,and its alteration at doubled CO2 concentration reduces toโˆ’2.9W/m2, so almost nothing remains in the atmosphere.

    The absorptivity aLW as listed in column 7 is againfound by comparing the absorption at 380 ppm with clouds(357.86W/m2) and without clouds (313.57W/m2), reducingcolumn 6 by this difference and then normalizing the cor-rected absorption to the incident radiation. aLW is showntogether with the parameter ๐‘“๐ด in Figure 4. Both graphs canagain well be represented by logarithmic plots.

    The changes in absorptivity from single to doubledCO2 with ฮ”aLW = โˆ’0.5% further decline compared to 66%cloudiness or clear sky, and also ฮ”๐‘“๐ด is slightly reducing toโˆ’0.34%.

    So, from these calculations it is clear that the up- anddownwelling fluxes and also the absorption in the atmosphereare significantly varying with the cloud clover and, therefore,they will also significantly influence the global mean surfacetemperature. But it can also well be recognized, that changeswith theCO2 concentration by trend get smaller with increas-ing cloudiness.

    4. Assessment of CO2 Global Warming

    Different to general circulation models, which try to predictlocal climate variations over some time period and, there-fore, have to solve complex coupled nonlinear differentialequations with a large number of parameters, making thesecalculations extremely time consuming and even unstable,for computing the equilibrium climate sensitivity ๐ถ๐‘† it issufficient to rely on a much simpler model, which calculatesan equilibrium energy and radiation balance and averagesover larger local variations.

    But independent of the modelโ€™s complexity, almost allknown models are based on the simple relation given by (1)that the ground temperature is scaling proportional with theradiative forcing of an external perturbation. Any feedbackprocesses, for example, by water vapor, albedo, the lapserate, or clouds, are generally included in this equation as anadditional prefactor (1 โˆ’ f โ‹… ๐œ†๐‘†)โˆ’1 in the following form:

    ฮ”๐‘‡๐ธ = ๐œ†๐‘†1 โˆ’ f โ‹… ๐œ†๐‘† โ‹… ฮ”๐น, (10)

    where f is the feedback parameter, by which all linearand nonlinear responses of EASy to a changing surfacetemperature are represented (see also Lindzen & Choi [28],only using different symbols).

    Thus, the simplest way to assess ๐ถ๐‘† is to directly apply(10) with the known feedback and radiative forcing. Often,however, this calculus method suffers from the fact

    (i) that the Planck sensitivity ๐œ†๐‘† has to be adapted fromother models;

    (ii) that it is difficult to distinguish between differentforcings with different feedbacks;

    (iii) that this method only considers a radiation balanceat the tropopause or TOA, but not an additionalradiation and energy balance at the surface;

    (iv) that it does not consider the feedback of the atmo-sphere to the surface and vice versa, caused byradiation changes as well as changes of sensible andlatent heat;

    (v) that some feedback processes and their evaluation arenot really retraceable from other sources;

    (vi) and that for simplicity reasons often sw feedbackeffects are completely neglected.

  • 10 International Journal of Atmospheric Sciences

    rSM + rSC

    rSM rSC

    rSErSE

    rLE

    rLE

    rLC

    atmosphere

    I0

    aSC

    aSW

    aLC

    aLW

    (1 โˆ’ fA) ยท IA

    fA ยท IA

    IC IL IEEarth

    aO3

    Figure 5: Two-layer climate model for the Earth-atmosphere system with the main parameters.

    Therefore, here we use our own advanced two-layer climatemodel, which is free from these deficits and which then canbe compared with the IPCC accounting scheme or othermethods. In addition, we investigate the effect and the sizeof the slightly changing reradiation of the atmosphere withincreasing CO2 concentration as represented by the back-radiated fraction ๐‘“๐ด.4.1. Model Adaptation to Satellite Measurements. Our two-layer climate model is especially appropriate to calculate theinfluence of the increasing CO2 concentrations on globalwarming as well as the impact of solar variations on theclimate.Themodel describes the atmosphere and the groundas two layers acting simultaneously as absorbers and Planckradiators. It includes additional heat transfer between theselayers due to convection and evaporation, and it considerscloud effects for the sw and lw radiation as well as all relevantfeedback effects like water vapor, lapse rate, albedo, cloudcover, convection, and evaporation. At equilibrium both theatmosphere and the ground release as much power as theyabsorb from the Sun and the neighbouring layer. An externalperturbation, caused by variations of the solar activity orthe GH gases, then forces the system to come to a newequilibrium with new temperature distributions of EASy.Figure 5 shows the main features of the two-layer climatemodel with its relevant parameters.

    Different to other schemes, in our model the key param-eters are not the radiative forcing, but the sw and lw absorp-tivities aSW and aLW as well as the back-radiated fraction ofthe atmosphere ๐‘“๐ด, all of which are varying with the CO2concentration (see Figures 1โ€“4). Whereas the sw absorptivitycan well be adopted from our previous calculations (Harde-2014 [16]), for the actual simulations we use the new andmore advanced radiation transfer calculations, presented inSection 3, which clearly distinguish between clear sky andcloudy conditions. All other parameters like the cloud and swozone absorptivities, the scattering coefficients at clouds andthe atmosphere, and the Earthโ€™s reflectivities were adapted in

    such a way that all radiation and heat fluxes almost exactlyreproduce the widely accepted TFK-scheme (see also Harde-2014 [16], Fig. 10), which essentially relies on data fromsatellitemeasurements within the ERBE andCERES program[51โ€“55]. This adaptation yields a calibration of our modelto the observed up- and downwelling fluxes under standardconditions in the atmosphere and for constant heat fluxesbetween the surface and atmosphere. All relevant parametersare listed in Table 6.

    Compared to our previous simulations (Harde-2014 [16])some of these parameters had slightly to be modified tofurther reproduce the TFK-scheme, this as a consequence ofthe changing fluxes and absorptivities with the ground tem-perature at clear sky or cloudiness. Particularly to reproducethe measured temperature variations with the cloud cover,the parameters ๐‘ŸSM and ๐‘ŸSC had to be adjusted to satisfy theTFK, as well as the ISCCP observations. In this sense ourmodel is similar to the energy budget ESC estimates, whichprovide an independent observationally based constraint ofthis important parameter (see Lewis & Crok [17], Forster &Gregory [27], and Lindzen & Choi [28]).

    For the temperature response of EASy and, thus, thecalibration of themodel we relate to the temperature anomalydata of the Hadley Centre and Climate Research Unit(HadCRUT3) as a function of the monthly global cloudcover data of the ISCCP (scatter diagram of O. Hum-lum, http://www.climate4you.com/ [22]) with a responseof โˆ’0.065โˆ˜C/%, while a reverse scatter plot for the sameISCCP data over the Berkley Earth Surface Temperature(BEST) leads to a much stronger temperature variationwith cloud cover of about โˆ’0.3โˆ˜C/%. Consequences for athermally induced cloud cover feedback will be discussed inSection 4.3.6.

    Our climate model also contains a parameter for thelw scattering at clouds (๐‘ŸLC) with the ability of multiplereflections between clouds and the surface. Since this quantityhas no meaning in an RT calculation, considering only a oneway propagation of radiation, the respective adaptation of the

    http://www.climate4you.com/

  • International Journal of Atmospheric Sciences 11

    Table 6: Parameter set at mean global cloud cover and meantemperature to reproduce the TFK data.

    Parameter Symbol Unit Valueaveraged solar flux ๐ผ0 W/m2 341.3cloud cover ๐ถ๐ถ % 66.0sw molec. scatteringcoef. ๐‘ŸSM % 13.2sw cloud scatteringcoef. ๐‘ŸSC % 18.14sw Earth reflectivity ๐‘ŸSE % 17.0sw ozone absorptivity aO3 % 8.0sw cloud absorptivity aSC % 12.15sw H2O-CO2-CH4absorptivity aSW % 14.51

    lw Earth's reflectivity ๐‘ŸLE % 0.0lw cloud scatteringcoef. ๐‘ŸLC % 20.9lw cloud absorptivity aLC % 54.1lw H2O-CO2-CH4-O3absorptivity aLW % 82.58

    Earthโ€™s emissivity ๐œ€๐ธ % 100.0atmospheric emissivity ๐œ€๐ด % 87.5back-radiated fraction ๐‘“๐ด % 61.8sensible heat flux ๐ผ๐ถ W/m2 17.0latent heat flux ๐ผ๐ฟ W/m2 80.0

    total upward flux and direct flux from the surface had to befitted in the RT calculations via the cloud absorptivity aLC,which, therefore, differs from the absorptivity used in the2LCM.

    The up- and downward fluxes as calculated by the two-layer climate model are compiled in Table 7 and show theexcellent agreement with the TFK data. The smaller devia-tions mainly result from the fact that the fluxes in the TFK-scheme are not completely balancing in up- and downwarddirection but contribute to a net surface absorption of0.9W/m2, while our calculations are valid for steady stateconditions with an exact balance between the absorbed solarradiation and the OLR.

    It should also be noticed that the direct flux from thesurface to TOA with 40W/m2 can only be realized witha relatively high lw cloud scattering and medium cloudabsorption.These parametersmainly determine the referencetemperature๐‘‡๐‘… and lw fluxes but have negligible influence oncalculations of the ECS. So, for example, for ๐‘ŸLC = 0 and aLC= 77%, for which the direct flux declines by 6W/m2, whilethe indirect flux increases by the same amount, the climatesensitivity stays the same.

    Since the objective of our investigations here is to evaluatethe influence of CO2 on global warming, the parameters inTable 6 and the fluxes in Table 7 primarily define a workingpoint for further considerations; in particular they determinethe reference temperature ๐‘‡๐‘… = 16โˆ˜C of the Earthโ€™s surface ata CO2 concentration of 380 ppm. Only deviations from thisreference, caused by a changing CO2 concentration and the

    Table 7:Comparison of calculated fluxes under regular atmosphericconditions with the TFK data.

    Flux (W/m2) ThismodelTFKdata

    sw: incoming solar radiation 341.3 341.3backscattered from molecules 14.1backscattered from clouds 65.0together backscattered 79.0 79reflected at Earthโ€™s surface 22.9 23total reflected solar radiation 101.9 101.9absorbed by O3, 27.3

    clouds, 19.1water vapor, CO2, CH4 31.6

    total absorption of atmosphere 78.0 78.0absorption in surface 161.3 161

    lw: surface radiation 396.3 396absorbed by GH-gases 327.3absorbed by clouds 19.5backscattered by clouds 9.5absorb. & scat. surface radiation 356.3 356sensible heat 17.0 17latent heat 80.0 80total absorption in atmosph. 521.8outgoing radiation fr. atmosph. 199.3 199outgoing directly from surface 40.0 40total outgoing radiation 239.4 238.5back-radiation 331.9 333net emission of surface 64.4

    total outgoing radiation at TOA 341.3 340.4

    different feedback processes, are of further interest, not somuch absolute temperature levels.

    4.2. Direct Influence of CO2. First we consider the simplestcase, neglecting any feedback processes and looking onlyto the direct influence of CO2 on global warming. Withthe sw and lw absorptivities as well as the back-radiatedfraction integrated in the climate model, the Earthโ€™s surfacetemperature and the lower tropospheric temperature aresimulated as a function of the CO2concentration. For details,how these temperatures are calculated by the 2LCM and howthey are defined, see Harde-2014 [16], Subsection 4.4.

    For the case of clear sky (๐ถ๐ถ = 0) this is shown inFigure 6(a), where the red graph indicates Earthโ€™s tem-perature ๐‘‡๐ธ at the surface and the blue graph the lowertropospheric temperature ๐‘‡๐ด as derived from the Stefan-Boltzmann relation when inserting the back-radiated power.The increase of๐‘‡๐ธ at doubledCO2 concentration (from380 to760 ppm) defines the CO2 climate sensitivity as a measure forthe response of EASy on a changing CO2 concentration. Atclear sky conditions and without feedback effects this climatesensitivity is found as ๐ถ๐‘† = 1.79โˆ˜C, which is significantly

  • 12 International Journal of Atmospheric Sciences

    24

    20

    16

    12

    8

    4

    Tem

    pera

    ture

    T(โˆ˜

    C) CS = 1.79โˆ˜C

    Tem

    pera

    ture

    T(โˆ˜

    C)

    18

    14

    10

    6

    2

    CS = 1.09โˆ˜C

    16

    12

    8

    4Tem

    pera

    ture

    T(โˆ˜

    C)

    CO2-concentration (ppm)0

    077070063056049042035028021014070

    CS = 0.89โˆ˜C

    TE TA logarithmic

    (a)

    (b)

    (c)

    Figure 6: Calculated Earth temperature ๐‘‡๐ธ (red) and lower tropo-spheric temperature ๐‘‡๐ด (blue) as a function of the CO2 concentra-tion under (a) clear sky, (b) 66% cloud cover, and (c) total cloudiness.Logarithmic approximations are plotted as green lines.

    larger than our previously published value of 1.1โˆ˜C (Harde-2014 [16]).

    The reason for this discrepancy is twofold. So, the new RTcalculations (see Section 3.2) were performed for a groundtemperature at clear sky of 20.3โˆ˜C, which increases the lwabsorptivity due to water vapor and, thus, lifts the climatesensitivity by about 0.4โˆ˜C. Another contribution of 0.3โˆ˜C isinitiated by the back-radiation, which slightly changes via๐‘“๐ด with the CO2 concentration (Figure 2). Although at clearsky the radiative forcing ฮ”๐น2ร—CO2 is almost only determinedby the absorption losses in the atmosphere (see Table 2), thesmall variationฮ”๐‘“๐ด of less than 0.4%,multipliedwith the totalatmospheric emission ๐ผtotal๐ด , causes this additional increase inour model (see second term in (9)).

    A higher cloudiness not only reduces the average surfacetemperature but also diminishes the climate sensitivity. Thiscan be seen from Figures 6(b) and 6(c), showing the surfaceand atmospheric temperature at themean cloud cover of 66%and 100% as a function of the CO2 concentration. At 66%cloudiness the climate sensitivity declines to ๐ถ๐‘† = 1.09โˆ˜C,while at 100% it even reduces to 0.89โˆ˜C.

    The green graphs in Figure 6 represent logarithmic fits,indicating that due to saturation effects and only far wingabsorption at higher CO2 concentrations the surface temper-ature can well be approximated by a logarithmic function ofthe following form:

    ๐‘‡๐ธ (๐ถ) = ๐‘‡๐ธ (๐ถ0) + ๐œ†๐‘† โ‹… ๐›ผ โ‹… ln( ๐ถ๐ถ0)

    = ๐‘‡๐ธ (๐ถ0) + ๐œ†๐‘† โ‹… ฮ”๐น2ร—CO2ln (๐ถ/๐ถ0)

    ln 2 ,(11)

    where ๐‘‡๐ธ(๐ถ0) is the temperature at a CO2 concentration๐ถ0 =380 ppm, ๐œ†๐‘† is the Planck sensitivity as it results fromour two-layer climate model, and ๐›ผ is defined as ๐›ผ =ฮ”๐น2ร—CO2/ ln 2 (see also Myhre et al. [39]).

    For the special case ๐ถ = 2 โ‹… ๐ถ0, (11) merges into (1),and we see that either ๐œ†๐‘† can be derived from a logarithmicfit to the temperature data or from the climate sensitivityusing (1). Table 8 summarizes the related quantities, whichcharacterize the influence of CO2 on global warming underdifferent cloud situations, but neglecting feedback processes.From these data we can assert that the Planck sensitivity,as deduced from our two-layer model, agrees within 8%with the model mean of the CoupledModel IntercomparisonProject Phase 5 (CMIP5) AOGCMs (AR5-WG1-Tab.9.5) andis slightly varying with the cloud cover. The same holds forthe reciprocal value, the Planck feedback.

    In this context it should be emphasized that the climatesensitivities from our model were derived with the swabsorptivity changes included, while ฮ”๐น2ร—CO2 in (11) onlyrepresents the lw RF at TOA, different to AR5.

    While the declining temperatures are a direct conse-quence of the dominating shielding effect for solar radiation,the smaller sensitivities are the result of the increasinginfluence of the lw cloud absorption and backscattering, bywhich the importance of the GH-gases is more and morerepelled.

    We also see that in comparison to the surface the loweratmosphere is responding less sensitively to the CO2 changes.This may be explained due to the changing radiation andenergy balance between the surface and atmosphere with anincreasing up- and downward emission of the atmosphere.But the difference between the two curves is more and morereducing at higher cloudiness.

    4.3. Feedback Processes. Many climate models agree withinacceptable limits in their prediction for the CO2 climatesensitivity, as long as feedback effects are excluded. Butbig discrepancies can be observed, when different feedbackprocesses and also climate drivers are included. One reasonmay be the complexity of these effects, from which theirinterrelated actions and their mutual interference are not

  • International Journal of Atmospheric Sciences 13

    Table 8: Compilation of some figures at clear sky, global mean cloud cover, and total cloudiness.

    Quantity/parameter Symbol Unit Valuecloud cover ๐ถ๐ถ % 0 66 100surface temperature ๐‘‡๐ธ โˆ˜C 20.3 16.0 13.8climate sensitivity ๐ถ๐‘† โˆ˜C 1.79 1.09 0.89CO2 radiative forcing ฮ”๐น2ร—CO2 W/m2 5.46 3.77 2.96Planck sensit. this model ๐œ†๐‘† Wโˆ’1m2 โˆ˜C 0.33 0.29 0.30Planck feedb. this model โˆ’1/๐œ†๐‘† W/m2/โˆ˜C โˆ’3.05 โˆ’3.47 โˆ’3.31Planck feedback, AR5 โˆ’1/๐œ†๐‘† W/m2/โˆ˜C โˆ’3.20

    really known. Another reason can also be a wrong orundifferentiated assignment of the feedbacks to a specificclimate driver, or the simple neglect of an effect.

    In this subsection we first consider the influence and sizeof the well known feedback processes caused by water vapor,the lapse rate, or albedo. Further we investigate the additionaleffects of convection, evaporation, and cloud cover feedback,which in this form are not discussed and the first ones areeven not mentioned in AR5.

    4.3.1. Water Vapor Feedback. Water vapor (WV) is by far thelargest contributor to the natural GH effect and, therefore,plays an essential role in Earthโ€™s climate (AR5-WG1-Chap.8.1).Since its amount in the atmosphere is only controlled by theair temperature, rather than by emissions, scientists considerit as a feedback agent, rather than a forcing to climate change.

    In AR5 we read as follows: โ€œthe contribution of watervapor to the natural greenhouse effect relative to that ofCO2 depends on the accounting method, but can be consid-ered to be approximately two to three times greater.โ€ Withrespect to their relative concentrations in the atmosphere thisproportion appears very small, as an amplifier for the basicclimate sensitivity; however, it is quite significant and has tobe investigated in more detail.

    Indeed, different methods can be applied to estimatethis ratio, and their results deviate significantly, dependingon what is made responsible for the GH effect and itsdefinition. So, similar to the procedure used to determinethe RF at doubled CO2, one way is first to calculate the totalupwelling intensity without WV, ๐ผuptotal (no WV), minus theintensity with all GH gases in the atmosphere ๐ผuptotal (all). Atglobal mean cloud cover and with MRT lineshapes (see alsoTable 4) this gives a difference ๐ผuptotal (no WV) โˆ’ ๐ผuptotal (all) =298.5 โˆ’ 239.5 = 59W/m2. Next one has to calculate thedifference between the intensities without CO2 and with allgases yielding ๐ผuptotal (no CO2) โˆ’ ๐ผuptotal (all) = 263.1 โˆ’ 239.5 =23.6W/m2. Comparison of these differences gives a ratio of59/23.6 = 2.5 in good agreement with AR5. However, thismethod essentially characterizes the efficiencies of these gasesto block the OLR to space, and thus primarily reflects theradiation balance at TOA, but not so much at the surface.

    Therefore, another way of accounting is to considerthe differences of the downwelling intensities, which atcloudiness result in ๐ผdown๐ด (all) โˆ’ ๐ผdown๐ด (no WV) = 329.4 โˆ’

    139.3 = 190.1W/m2 and ๐ผdown๐ด (all) โˆ’ ๐ผdown๐ด (no CO2) =329.4 โˆ’ 315.0 = 14.4W/m2 with a ratio 190.1/14.4 = 13.2.This method is particularly sensitive to the contributionsof WV or CO2 at the surface and shows the dominatinginfluence of WV in the lower troposphere, which in thisaccounting scheme contributes about 60% to the GH effect,while CO2 is donating not more than 4% and thus relativizesthe importance of CO2 as a dangerous climate driver in theatmosphere. An even slightly larger ratio of WV to CO2 tothe GH effect of about 14 can be found, when calculating theback-radiation under clear sky conditions. A similar resultis found considering only the absorption of the terrestrialradiation, first for all gases and then without one of thecomponents, yielding a weighting ratio of 15.

    With respect to feedback processes these numbers lookquite dramatic. But the contribution of a gas or vapor to theGH effect does not automatically determine its influence asa feedback agent. Therefore, this has to be considered moreextensively.

    Due to the Clausius-Clapeyron equation theWV contentis rapidly increasing with rising temperatures. So, from GPS-measurements (Vey [34]) of the water content in differentclimate zones we can derive the averageWV concentration ina zone (see Harde-2014 [16], Fig. 1), and with the temperaturedifferences between these zones we then estimate that withevery extra degree of air temperature the atmosphere retains5.9% more water vapor. Therefore, also the WV absorptionis further increasing and generally contributes to a positivefeedback in the total budget. In the literature this feedback isdesignated as the most serious effect with dramatic amplifi-cation values. So in AR5-WG1-Chap.8 we can read โ€œalthoughCO2 is the main anthropogenic control knob on climate, watervapor is a strong and fast feedback that amplifies any initialforcing by a typical factor between two and three.โ€

    Our own investigations, however, show a less dramaticinfluence of water vapor. One aspect is that, similar toCO2, also the water lines are already strongly saturatingover wider spectral regions. Therefore, with increasing vaporconcentration only the far wings of these lines and weakabsorption bands can further contribute to an additionalabsorption, which roughly logarithmically increases with thevapor concentration.

    Another aspect is that always both sw and lw absorptionhave to be considered. Whereas the lw outgoing radiation ismore efficiently blocked and thus contributes to a positive

  • 14 International Journal of Atmospheric Sciences

    Table 9: sw absorptivity aSW, total lw absorptivity a๐‘‡, and back-radiated fraction ๐‘“๐ด as a function of the surface temperature andwater vapor concentration in three climate zones.

    Climatezone

    ๐‘‡๐ธโˆ˜C

    ๐ถWVppm

    aSW%

    a๐‘‡%

    ๐‘“๐ด%

    High-lat. โˆ’7 2,359 12.5 81.5 59.2Mid-lat. 8 7,253 13.4 85.5 61.0Tropics 26 22,900 15.2 90.8 62.9

    feedback, the sw radiation is also more strongly absorbedin the atmosphere, and less of it reaches the surface, whichsupplies a negative feedback contribution.

    Table 9 shows the results of our calculations for thesw absorptivity aSW, the total lw absorptivity a๐‘‡ (includingcloud absorption), and the back-radiated fraction ๐‘“๐ด, which,different to our computations in Section 3, for these feedbackstudies were calculated at a fixed CO2 concentration of380 ppm, but for three climate zones with different surfacetemperatures and, thus, also different WV concentrations๐ถWV. While aSW was taken over from Harde [16], thelw absorptivity and ๐‘“๐ด were derived under conditions asdescribed in Section 3.4, assuming a cloud cover of 66%, acloud altitude of 6 km, and a cloud emissivity of 48% andusing MRT lineshapes, which already include the WV con-tinuum.We have used the same global mean cloud cover andheight over all zones. For typical expected cloud variationsover the zones and comparing this with the case of clear skywe estimate that this simplification results in an error of lessthan 5%. Variations of the cloud cover with temperature andtheir feedback effects are discussed in Section 4.3.6. For theactual feedback analyses it is sufficient and even preferentialonly to consider the total lw absorptivity, which we designateas a๐‘‡ andwhich consists of the absorption byGHgases as wellas by clouds.

    Figure 7 displays the three key parameters aSW, a๐‘‡, and๐‘“๐ดas a function of the surface temperature.The red and the blueline as fits to the calculations directly reflect the temperaturedependence of the absorptivities, which at constant gasconcentrations would have slightly dropped with increasingtemperature but due to the dominating growth of the WVconcentration results in a net increase. The linear incline isthe result of an exponential growth of the WV concentrationwith temperature due toClausius-Clapeyron and on the otherhand a logarithmic growth of the absorptivities with thevapor concentration due to saturation effects.

    The sw and lw absorptivity changes can well be repre-sented by straight lines with the slopes

    ๐‘‘aSW๐‘‘๐‘‡๐ธ = 0.10%/

    โˆ˜C, (12)

    ๐‘‘a๐‘‡๐‘‘๐‘‡๐ธ = 0.28%/

    โˆ˜C. (13)

    For clear sky calculations we further use the value ๐‘‘aLW/๐‘‘๐‘‡๐ธ= 0.38%/โˆ˜C (Harde [16], (80)).

    1009080706050403020100

    0 5

    Surface temperature TE (โˆ˜C)

    3025201510โˆ’5โˆ’10

    aTaSWfAfA(CMIP5)

    ๏ฟฝt aT๏ฟฝt aSW๏ฟฝt fA

    Abso

    rptiv

    ity,f

    A(%

    )

    Figure 7: sw absorptivity (blue squares and fit), total lw absorptivity(red triangles and fit) and back-radiated fraction (green circles andfit) for high-latitudes, mid-latitudes, and the tropics. Additionallyshown is the predicted back-radiated fraction due to CMIP5 asmagenta line.

    The back-radiated fraction ๐‘“๐ด (green circles in Figure 7)as a function of the surface temperature can also well berepresented by a straight line with the slope

    ๐‘‘๐‘“๐ด๐‘‘๐‘‡๐ธ = 0.11%/

    โˆ˜C. (14)While our calculations in Section 3 describe the variationsof ๐‘“๐ด with the CO2 concentration and also with cloudiness(see Figures 1โ€“4), this graph displays the additional responseof ๐‘“๐ด on the temperature and the humidity changes. Thisresponse is a typical feedback process, which modifies theup- and downwelling fluxeswith the surface temperature and,thus, influences the total radiation and energy balance ofEASy. Although the main part of this feedback can be tracedback to the increasing WV concentration with temperature,another contribution can be induced by changes of thevertical temperature distribution over the atmosphere and,thus, by changes in the lapse rate. Since it is not advisable tofurther split these contributions, the temperature dependenceof ๐‘“๐ด as a whole will be considered in more detail in the nextsubsection as lapse rate feedback.

    Now, taking advantage of (12) and (13) the WV feedbackcan directly be integrated in our model. This is realized byan iterative procedure, which has been explained in moredetail elsewhere (Harde-2014 [16], Section 4, pp. 26-27). Ina first step the temperature deviation from the referencetemperature ๐‘‡๐‘…, caused by a deviation of CO2 from thereference concentration (here 380 ppm), is calculated.This๐‘‡-offset is used to compute with (12) and (13) the correctionsin the absorptivities. With the new values again correctedtemperatures are determined, which give new absorptioncorrections. This is repeated, until the temperatures showself-consistency.

    The result of such a calculation with WV feedback isillustrated in Figure 8, showing the temperature increase of

  • International Journal of Atmospheric Sciences 15Te

    mpe

    ratu

    reT

    (โˆ˜C)

    18

    22

    26

    14

    10

    6

    2

    CS = 2.81โˆ˜C

    Tem

    pera

    ture

    T(โˆ˜

    C)

    CO2-concentration (ppm)0 77070063056049042035028021014070

    18

    14

    10

    6

    2

    CS = 1.24โˆ˜C

    TE TA logarithmic

    (a)

    (b)

    Figure 8: Calculated Earth temperature ๐‘‡๐ธ (red) and lower tropo-spheric temperature ๐‘‡๐ด (blue) as a function of the CO2 concentra-tion under (a) clear sky and (b) 66% cloud cover, both with watervapor feedback. Logarithmic approximations are plotted as greenlines.

    ๐‘‡๐ธ and๐‘‡๐ด as a function of theCO2 concentration. At clear sky(Figure 8(a)) the climate sensitivity rises up from ๐ถ๐‘† = 1.79โˆ˜Cto 2.81โˆ˜C, which results in an amplification factor due to theWV feedback of 1.57, or in terms of the feedback parameter(see (9)) gives fWV = 1.10W/m

    2/โˆ˜C. At global mean cloudcover (Figure 8(b)), however, ๐ถ๐‘† only increases from 1.09โˆ˜Cto 1.24โˆ˜C, corresponding to an amplification of 1.14 or to afeedback of fWV = 0.43W/m

    2/โˆ˜C.Compared to AR5-WG1-Tab.9.5, where the WV feedback

    is specified as a model mean of fWV = 1.6 ยฑ 0.3W/m2/โˆ˜C(corresponding to an amplification factor of two), this is asignificant discrepancy, even to our clear sky result.

    The reasons for this discrepancy are manifold. So, asalready mentioned, our calculations also consider the swabsorptivity, which causes a negative feedback, while thisis not clear for the feedbacks specified in AR5. The maindifferences, however, go back to the procedures appliedto determine the changes of aLW or a๐‘‡ with temperature,independent of any variations in๐‘“๐ด.This can best be retracedconsidering the most important contributions, which areresponsible for these changes.

    Quite generally we can distinguish two effects and write

    ๐‘‘aLW,๐‘‡ = ๐œ•aLW,๐‘‡๐œ•๐ถWV๐œ•๐ถWV๐œ•๐‘‡๐ธ ๐‘‘๐‘‡๐ธ +

    ๐œ•aLW,๐‘‡๐œ•๐œŽLW

    ๐œ•๐œŽLW๐œ•๐‘‡๐ธ ๐‘‘๐‘‡๐ธ, (15)

    with ๐œ•aLW,๐‘‡/๐œ•๐ถWV as the partial derivative describing thelw (total) absorptivity changes as a function of the watervapor concentration ๐ถWV, ๐œ•๐ถWV/๐œ•๐‘‡๐ธ as the changes of๐ถWV with the surface temperature, ๐œ•aLW,๐‘‡/๐œ•๐œŽLW as theabsorptivity changes with the lw absorption cross-section๐œŽLW, and ๐œ•๐œŽLW/๐œ•๐‘‡๐ธ as the changes of the cross-sectionwith temperature. So, the first term in (15) describes thegrowth of aLW or a๐‘‡ with the vapor concentration, whichon its own is strongly temperature dependent due to theClausius-Clapeyron equation; the second term represents thevariations of aLW,๐‘‡ with the absorption cross-section, whichchanges due to temperature dependent population densitiesof the involvedmolecular states and the linewidths (for detailssee, e.g., Harde-2013 [18]).

    The partial derivative ๐œ•aLW,๐‘‡/๐œ•๐ถWV can be found bycalculating the absorptivity as a function of the WV con-centration and then taking the slope to this curve at a givenconcentration. Figure 9 displays the lw absorptivity aWV =aLW only of water vapor at clear sky via the concentration(lower graph, black diamonds) and on the other hand thetotal absorptivity a๐‘‡ (blue squares) resulting from all GHgases and the clouds. Both graphs were calculated applyingan MRT lineshape and in the latter case assuming the globalmean cloud cover of 66%, an altitude of 6 km, and anemissivity of 0.48. The pink lines are fits to the absorptivitieswith logarithmic progression.

    In this context it has to be mentioned that the absorp-tivities, reflecting integrals of the absorption coefficients and,thus, integrals of the cross-sections over the altitude andover the spectral distribution (see Harde-2014 [16], (2โ€“4)),inherently include the general temperature dependence ofthe absorption coefficients with altitude, but this has to bedistinguished from the surface temperature variations, whichinfluence the whole vertical temperature distribution overthe atmosphere and which are represented by the secondterm in (15). The decrease in the WV absorptivity aWV at anincreasing ground temperature from 16 to 21โˆ˜C at otherwisesame conditions is represented by green triangles in Figure 9for three WV concentrations.

    In AR5-WG1-Chap.8.3.1 we can read that most inter-comparison studies of the RF of GH gases are for clearsky and aerosol-free conditions, while the introduction ofclouds would greatly complicate the targets of research andare usually omitted in the intercomparison exercises of GCMradiation codes and LBL codes. Therefore, obviously alsofor an assessment of the WV feedback cloud effects wereneglected. In addition, most of the GCMs emanate from amean WV concentration of 7,750 ppm, in agreement withthe US Standard Atmosphere 1976, representing mid-latitudebut not global mean conditions. The slope to the clear skyWV absorptivity at 7,750 ppm then gives ๐œ•aWV/๐œ•๐ถWV =0.0018%/ppm, and a WV increase of 7%/โˆ˜C, as assumed inAR5-WG1-FAQ-8.1, contributes to ๐œ•๐ถWV/๐œ•๐‘‡๐ธ = 542 ppm/โˆ˜C.Substituting aLW by aWV this gives for the first term on theright side of (15) the following:

    ๐‘‘aWV๐‘‘๐‘‡๐ธ (1. term) =

    ๐œ•aWV๐œ•๐ถWV

    ๐œ•๐ถWV๐œ•๐‘‡๐ธ = 0.98%/

    โˆ˜C (16)

  • 16 International Journal of Atmospheric Sciences

    100

    80

    60

    40

    20

    0

    a T,a

    WV

    (%)

    water vapor concentration (ppm)24000200001600012000800040000

    log ๏ฟฝt aTaWV: clear sky, 16โˆ˜C

    log ๏ฟฝt aWVaWV: clear sky, 21โˆ˜C

    aT: Cc-66%, 16โˆ˜C

    Figure 9: Lw water vapor absorptivity aWV (black diamonds)and total absorptivity a๐‘‡ (blue squares) as a function of the WVconcentration at a surface temperature of 16โˆ˜C.Themagenta graphsrepresent logarithmic fits to the absorptivities. Green trianglesindicate calculation of aWV at 21โˆ˜C.

    and is almost exactly the absorptivity change per โˆ˜C, neces-sary to deduce a WV feedback of fWV = 1.6W/m

    2/โˆ˜C and anamplification factor of two, as published in AR5.

    So, under these assumptions the IPCC data can wellbe reproduced. But as outlined above, this approach omitsclouds, emanates from a lower WV concentration, andneglects any surface temperature dependence of the absorp-tion cross-section of the GH gases.

    Our own considerations include a spectral overlap andinterference of WV with other GH gases as well as withclouds, and we assume a global mean WV concentration (atstandard conditions) of 14,615 ppm. Both aspects contributeto a larger total absorptivity a๐‘‡, but to a reduced pitch aroundthe mean WV concentration and result in a slope ๐œ•a๐‘‡/๐œ•๐ถWV= 0.00042%/ppm. Together with a WV increase of 5.9%/โˆ˜C(see above), which due to the higher WV concentration nowcontributes to a gain per โˆ˜C of ๐œ•๐ถWV/๐œ•๐‘‡๐ธ = 862 ppm/โˆ˜C,this gives for the first term in (15) an increase of the totalabsorptivity of (๐‘‘a๐‘‡/๐‘‘๐‘‡๐ธ)1. term = 0.36%/โˆ˜C.

    The temperature variation of a๐‘‡ via the absorption cross-section can be found by calculating the absorptivities fordifferent surface temperatures at otherwise identical vaporand gas concentrations. Since for these calculations weassume a fixed temperature at the tropopause of 216.6 K,independent of the surface temperature, any ๐‘‡๐ธ-variationsfade with altitude and, thus, also the respective absorptivitychanges fade.Therefore, such calculations rather give a lowerlimit for these changes, yielding a temperature dependence of(๐‘‘a๐‘‡/๐‘‘๐‘‡๐ธ)2. term = โˆ’0.08%/โˆ˜C. Inserting this value for the 2ndterm in (15), this contributes to a total lw absorptivity changewith temperature of

    ๐‘‘a๐‘‡๐‘‘๐‘‡๐ธ = 0.36 โˆ’ 0.08 = 0.28%/

    โˆ˜C, (17)

    which exactly reproduces the result of (13) and was alreadyderived from the slope of Figure 7.

    The direct comparison of the different approaches clearlyshows the different assumptions and their influence on theWV feedback. Whereas our result only contributes to anincrease of the direct CO2 influence (basic climate sensitivity)of 14%, the IPCC follows from a gain of 100%, which is morethan 7 times larger than our result.

    4.3.2. Lapse Rate Feedback. The average temperaturedecrease with altitude over the troposphere is specified as6.5โˆ˜C/km and assumed to be constant up to the tropopauseat about 11 km altitude [35]. This lapse rate has a directinfluence on the power, which is asymmetrically reradiatedby the atmosphere in downward and upward direction.In our radiation transfer calculations (see Section 3) thisasymmetry is expressed by the parameter ๐‘“๐ด, for which atthe standard lapse rate we find a back-radiated fraction ofabout ๐‘“๐ด = 62% and a rejected portion to space of (1 โˆ’ ๐‘“๐ด)= 38%, slightly varying with the individual assumptions likecloud cover, lineshape, or humidity in an RT calculation.When the vertical temperature profile changes and/or theback-radiation varies due to concentration changes of theGH gases with the temperature, as a direct consequencealso the radiation balance will be modified. This induces aclimatic effect, known as lapse rate feedback.

    It is well known that the tropopause height is significantlyvaryingwith the climate zone (also over the seasons) and in sofar directly related to the local ground temperature. Adetaileddescription of the tropopause altitude and its variation withlatitude has been given by Hoinka [56]. While the meanabsorption and reradiation over some longer or shorter dis-tance in the troposphere will not noticeably be influenced, aslong as the optical depth is the same, changes of the lapse ratewith the ground temperature directly affect the back-radiatedfraction๐‘“๐ด and, thus, the total balance of EASy. However, dueto dominating wet-adiabatic convection in the atmospherethe lapse rate can be expected to a large extent to be the sameeven at strongly varying surface temperatures. Nevertheless, aremaining variation of ๐‘“๐ด with temperature can be observedwhich is induced by the stronger WV changes with theclimate zone and thus with the surface temperature. Thegreen line in Figure 7 displays this variation of ๐‘“๐ด with theground temperature for the case of a constant lapse rateover the three climate zones as well as over the troposphereand supposing a vertical WV distribution in agreement withthe Clausius-Clapeyron-equation. Under these conditions wefind a temperature dependence of ๐‘‘๐‘“๐ด/๐‘‘๐‘‡๐ธ = 0.11%/โˆ˜C asalready specified in (14), which on its own would contributeto a positive lapse rate feedback of f+LR = +0.85W/m2/โˆ˜C.

    On the other side in AR5 we can read โ€œboth theory andclimate models indicate that global warming will reduce therate of temperature decrease with altitude, producing a negativelapse rate feedback that attenuates the greenhouse effect.โ€

    So, global circulation models predict an enhanced warm-ing in the upper troposphere of tropical regions, particularlyin response to an increasing water vapor concentration,which should result in a negative feedback. On the otherhand, at mid- to high-latitudes, a larger low level warming is

  • International Journal of Atmospheric Sciences 17

    expected as response to the positive radiative warming, thus,providing a positive feedback, as this is expected from theprevious considerations. Since the influence of the tropics isassumed to dominate, in AR4 a resulting negative feedbackof โˆ’0.85W/m2/โˆ˜C was predicted [26, 57], which now hasbeen reduced to fLR = โˆ’0.6W/m2/โˆ˜C (AR5-WG1-Tab.9.5).In our accounting scheme this corresponds to temperaturedependence of the back-radiated fraction of ๐‘‘๐‘“๐ด/๐‘‘๐‘‡๐ธ = ๐‘๐‘Ž =โˆ’0.078%/โˆ˜C and is represented in Figure 7 as magenta line.

    Since the water vapor has a more or less strongerinfluence on the lapse rate, both effects are often consideredtogether. For the combined feedback we then find fWV+LR =โˆ’0.18W/m2/โˆ˜C with an attenuation of 0.95, while the IPCCspecifies a value of fWV+LR = 1.1W/m2/โˆ˜Cwith an amplifica-tion of the climate sensitivity of 1.47 (AR5-WG1-Chap.9, notdifferentiated between clear sky or cloudiness).

    4.3.3. Surface Albedo Feedback. It is well known that changesto the physical properties of the land surface and sea ice willperturb the climate, both by exerting an RF and bymodifyingother processes such as the fluxes of latent and sensibleheat or the transfer of momentum from the atmosphere.Also the other way round is climate influencing the surfaceproperties, which again act back on the climate. So, anincreasing ground temperature reduces the Earthโ€™s reflectivityvia melting ice shields in the polar regions and it changesthe vegetation. With varying reflectivity particularly the swradiation balance will be modified in such a manner thatwith reducing sw reflectivity ๐‘ŸSE more power is absorbed bythe Earthโ€™s surface which then contributes to an additionalheating of the ground.

    This surface albedo influence is estimated as a positivefeedback of fSA = 0.3 ยฑ 0.1W/m2/โˆ˜C (AR5-WG1-Tab.9.5).In our simulations we introduce this albedo feedback as atemperature dependent change of the Earthโ€™s reflectivity with

    ๐‘‘๐‘Ÿ๐‘†๐ธ๐‘‘๐‘‡๐ธ = โˆ’0.143%/

    โˆ˜C, (18)

    which under clear sky contributes to an increase of the climatesensitivity of 12% and at mean overcast of 10%.

    4.3.4. Convection Feedback. Sensible heat represents theenergy transfer through thermal conduction and convectionfrom the warmer surface to the colder atmosphere. At thereference CO2 concentration of 380 ppm and temperature๐‘‡๐‘… = 16โˆ˜C this heat flux was chosen to be 17W/m2 inagreement with the TFK-scheme, and this flux was assumedto be constant in the previous simulations. However, thedriving force for this flux is the temperature difference at theboundary layer between surface and atmosphere. In addition,advection in form of a horizontal energy transfer along theboundary through wind and water currents takes place. Thistransfer is only indirectly dependent on the temperaturedifference; therefore, it is close-by to assume a power transferper surface area, which is represented by a temperature

    independent portion ๐ผ๐ถ0 and a temperature dependent partin the form

    ๐ผ๐ถ (๐‘‡๐ธ, ๐‘‡๐ด) = ๐ผ๐ถ0 + โ„Ž๐‘ (๐‘‡๐ธ โˆ’ ๐‘‡๐ด๐ถ) , (19)with โ„Ž๐ถ as the heat transfer coefficient and ๐‘‡๐ด๐ถ as the airtemperature at the convection zone.

    Since in first approximation ๐‘‡๐ด๐ถ can be assumed toscale synchronously with the lower atmospheric temperature๐‘‡๐ด, typically reflecting a temperature equivalent to an airlayer temperature in about 800m altitude, but convectionis only dominant over about 200m height, the temperaturedifference (๐‘‡๐ธ โˆ’ ๐‘‡๐ด๐ถ) in (19) is considered to be just one-quarter of the difference (๐‘‡๐ธ โˆ’ ๐‘‡๐ด) (see Harde-2014 [16],Subsections 4.4 and 5.4.4).

    Due to the second term in this equation any changesin the surface and atmospheric temperature, which may beinduced by CO2, initiate a feedback on EASy. We call thisconvection feedback.

    From Figure 6(a) we see that under clear sky the airtemperature reacts less sensitively to CO2 variations than theEarth temperature, and the difference (๐‘‡๐ธ โˆ’ ๐‘‡๐ด) increaseswith rising CO2 concentration. Therefore, also the sensibleheat flux grows with the concentration and contributes to anadditional cooling with a negative feedback.

    This feedback gets maximum, when the first term on theright side of (19) vanishes and the total heat flux of 17W/m2at 380 ppm CO2 is determined by the second term. Underregular cloud cover with a temperature difference (๐‘‡๐ธโˆ’๐‘‡๐ด) =5.2โˆ˜C the heat convection coefficient can assume a maximumvalue of โ„Ž๐ถ,max = 17/0.25/5.2 = 13W/m2/โˆ˜C. When choosinga smaller convection parameter, this automatically reducesthe feedback but increases the first term in (19), so that atthe reference CO2 concentration always a sensible heat fluxof 17W/m2 is guaranteed (for clear sky it gets slightly larger).

    FromFigures 6(b) and 6(c) we further recognize that withincreasing cloud cover the difference in (๐‘‡๐ธ โˆ’ ๐‘‡๐ด) more andmore disappears and, thus, any feedback gets smaller.

    With โ„Ž๐ถ,max = 13W/m2/โˆ˜C we calculate at clear sky aclimate sensitivity of ๐ถ๐‘† = 1.68โˆ˜C with a feedback of fCO =โˆ’0.19W/m2/โˆ˜C and an attenuation factor of 0.94, whereasat regular cloud cover the sensitivity turns into ๐ถ๐‘† = 1.07โˆ˜Cwith a feedback of only fCO = โˆ’0.06W/m2/โˆ˜C and a dampingfactor of 0.98. With a more moderate convection coefficientof 4โ€“6W/m2/โˆ˜C, as this has to be expected, when somelarger fraction of the sensible heat transfer has to be assignedto advective processes, convection feedback still furtherdecreases, and with a damping of less than 1% then thisfeedback process can well be neglected.

    4.3.5. Evaporation Feedback. Latent heat describes the energytransf