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LM Fraile, CERN PH/ISLM Fraile, CERN PH/IS
Highlights from the ISOLDE facility25 January 2006
Highlights from the ISOLDE facilityHighlights from the ISOLDE facility25 January 2006
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
OutlineOutline
ISOLDE in perspectiveProduction of RIB - the ISOLDE facilityThe low energy Physics programme→ Nuclear Astrophysics→ Ground state properties→ Neutron shell closures→ Applications
REX-ISOLDE PhysicsTowards the future…
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Historical perspectiveHistorical perspective
1964 ISOLDE project approved
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ISOL type facilities in 1967ISOL type facilities in 1967
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Historical perspectiveHistorical perspective
1964 ISOLDE project approved 1967-90 ISOLDE operation on SC1992 ISOLDE relocated to PS Booster1995 REX post-accelerator approved2001 REX-ISOLDE experiments start
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Historical perspectiveHistorical perspective
1964 ISOLDE project approved 1967-90 ISOLDE operation on SC1992 ISOLDE relocated to PS Booster1995 REX post-accelerator approved2001 REX-ISOLDE experiments start2005 3080 hours of RIB2007 REX-ISOLDE upgrade to 4.2 MeV2010? HIE-ISOLDE
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ISOL vs. InISOL vs. In--flightflight
Experiments
ISOL
In-flight
DR
IVE
R:
Acc
eler
ator
Rea
ctor
Thintarget
Fragmentseparator
Storageringheavy ions
Thicktarget
Ionsource
Massseparator
Postaccelerator
p, d, n… meV to ~100 MeV/ums to long-lived
GeV/u regimeμs
Gascell
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
CERN Accelerator complexCERN Accelerator complex
1.0/1.4 GeV protonsPulse frequency: 1.2 s# pulses ~ 6/14Intensity: 3.2 x 1013
protons per pulse2 μA ≈ 3 kW→ up to 5 μA tested!
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Production / 1Production / 1stst selection stepselection step
pn
spallation
fragmentation
fissio
n
p
Many different materialsMany different structures
+
225Fr
+ +
NA11Li
+ +
141Cs NA
1.4 GeV p
238U
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Heat diffusion Heat diffusion -- EffusionEffusion
Material
Geometry
Density
Solid state structure
Dissociation temperature
Melting point
Vapour pressure
Effusion process
Adsorptionenthalpy
Temperature
Temperature Geometric path
Diffusion process
Half life
Ionsource
T ~ 2000 ºC
Thicktarget
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ISOLDE target handlingISOLDE target handling
Storing of targets in the tunnel
Target mounted on the Front-End
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Kr yieldsKr yields
[U. Köster et al., NIM B204 (2003) 347–352]
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Converter targetConverter target
Protons
nTransfer Line to Ion Source
Fission products
n
n
n
n
P
Spallationneutrons
Spallation targetISOLDE target (UCx)
1 GeV p
pn
238U
201Fr
+spallation
11Li X
+ +fragmentation
143Cs Y+ +
fission
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Converter targetConverter target
UCx # 208, W Surface with W Converter
Cs yields from UCx-target with and without converter
1.E+02
1.E+03
1.E+04
1.E+05
1.E+06
1.E+07
1.E+08
1.E+09
1.E+10
120 125 130 135 140 145 150
A number (Cs isotopes)
Ato
ms
per μ
C
Jaeri directJaeri converterExp. directExp w. converter
0
2000
4000
6000
8000
10000
-50 -40 -30 -20 -10 0 10 20 30 40 50Z [mm]
Cs c
ount
rate
[Hz]
142 Cs H-scan 1 GeV std beam 5E12142 Cs H-scan 1GeV focussed beam
10 mm
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Ionization / 2Ionization / 2ndnd selection stepselection step
Heated tube (up to 2400 ºC) made of a material (W, Ta…) with lower work function than the species to be ionized.
Extraction electrode (60 kV) The work function of the atomic state sets the
limit on the ionization potential:
• Alkalines
• Alkaline earths (heavier ones)
• Rare earths (lanthanides)
• Group IIIa (B) elements
Surface Ion Source
~5 eV
Continuum
Electronic ground state of a radioactive atom
Ionizer ground state
Continuum
Ionizer
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
IonizationIonization
Plasma created by electrons accelerated in a voltage (~130 V) between the extraction electrode and the line in a Ar/Xe environment. A magnetic field is used to guide the electrons.Extraction
electrode (60 kV)
The electron impact is highly non-selective, other parameters
• Noble gases, C,N,O [cold transfer line]
• Metals with low melting point, high vapor pressure (Cd, Hg) [temperature range]
• Molecule formation: Fluorines, oxides (Sr, Y, Ba, La)
Plasma Ion Source
Ei (impact) > Eionization
Continuum
Electronic ground state of a radioactive atom
Ei
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Ionization: RILISIonization: RILIS
Resonant ionization of atomic structure Repetition rate ~ 11 kHzRange: 210 nm – 1000 nm• Pumping with copper-vapour lasers (511 & 578 nm) • Adjustable dye lasers• Frequency doubling/tripling in non-linear crystals
Resonant Laser Ion Source
< 9 – 10 eV
Continuum
Electronic ground state of a radioactive atom
+
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Ionization: RILISIonization: RILIS
Highly selective
High efficiency (given by the thermal distribution over the atomic fine structure of the ground state):
• Not well surface ionized (or separated) elements
• Metals with 6-9 eV ionization gap and a 1st ionization step not too far into the UV
• Hyperfine splitting gives a possibility to separate nuclear isomeric states.
Schemes:4Be, 12Mg, 13Al, 20Ca, 21Sc, 25Mn, 27Co, 28Ni, 29Cu, 30Zn, 31Ga, 39Y, 47Ag, 48Cd, 49In, 50Sn, 51Sb, 65Tb, 66Dy, 70Yb, 81Tl, 82Pb, 83Bi …
Example: Mn, gap = 7.43 eV
λ1=279.8 nm λ2= 628.3 nm λ3= 510.5 (CVL)
Efficiency ~ 10%
Isotope shifts → retuningSuppression of (surface ionized) contaminants
Choice of ionizerBeam gate LIST Requested by ~50% of experiments
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Mass separation / 3Mass separation / 3rdrd selection stepselection step
“Isobaric”separationSeparation limited by the transverse size of the beamsCooling at low energy with RFQ cooler
BUFFER GASHIGH VOLTAGE
VDC(z)
z
r
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ISOLDE Table of elementsISOLDE Table of elementsH
Li
Na
Be
Mg
Cs
Rb
K
Fr
Ba
Sr
Ca
Ra
La
Y
Sc
Ac
Hf
Zr
Ti
Rf
Ta
Db
W
Sg
Re
Bh
Os
Hs
Ir
Mt
Pt
Ds
Au
Rg
Hg
112
Al
Tl
Si
Pb
P
Bi
S
Po
Cl
At
Nb
V
Mo
Cr
Tc
Mn
Ru
Fe
Rh
Co
Pd
Ni
Ag
Cu
Cd
Zn
In
Ga
Sn
Ge
Sb
As
Te
Se
I
Br
Xe
Kr
Ar
Rn
B C N O F Ne
He
Th
Ce
Pa
Pr
U
Nd
Np
Pm
Pu
Sm
Am
Eu
Cm
Gd
Bk
Tb
Cf
Dy
Es
Ho
Fm
Er
Md
Tm
No
Yb
Lr
Lu
+ SURFACE –hot PLASMA cooled
LASER
ION SOURCE:
113 114 115
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ISOLDE Nuclear chartISOLDE Nuclear chart
More than 850 isotopes of ~70 elements
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Nuclear PhysicsNuclear Decay
Spectroscopy and Reactions
Structure of NucleiExotic Decay Modes
Atomic PhysicsLaser Spectroscopy
and Direct Mass MeasurementsRadii, Moments, Nuclear Binding
Energies
NuclearAstrophysics
Dedicated Nuclear Decay/Reaction Studies
Element Synthesis, Solar Processes
f(N,Z)
Fundamental Physics
Direct Mass Measurements, Dedicated Decay Studies - WICKM unitarity tests, search for β-ν correlations, right-handed
currents
Applied PhysicsImplanted Radioactive
Probes, Tailored Isotopes for Diagnosis and Therapy Condensed matter physics
and Life sciences
What forWhat for……??
Strong + weak interactions
Hadronic few-body system
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ISOLDE in perspectiveProduction of RIB - the ISOLDE facilityThe low energy Physics programme→ Nuclear Astrophysics→ Ground state properties→ Neutron shell closures→ Applications
REX-ISOLDE PhysicsTowards the future…
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
The ISOLDE Physics programmeThe ISOLDE Physics programme
300 to 350 8-hour shifts per yearSome 35 experiments/yearISOLDE delivered 385 8-hour shifts in 2005!Program 2001-2004:
Life Sciences:4%
Nuclear Astrophysics: 10%
Fundamental properties: 19%
Solid StatePhysics: 20%
Nuclear Physics and Weak
Interaction: 47%
~20% of the time devoted to development~450 users from 25 countries/100 institutes
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ISOLDE beam time summary 2005ISOLDE beam time summary 200519
9819
9920
0020
0120
0220
0320
0420
050
204060
80
100
120
140
160
Biology and Medicine
Particle and Astrophysics
Atomic Physics
Solid state physics
Weak Interaction andNuclear Physics
Num
ber o
f shi
fts
Year
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
r3α ∝Γrad e-Q/kT
The tripleThe triple--alpha processalpha process
[H. Fynbo et al.]
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
0 0+
0,2+
0+
10.3
7.6542
12.71 1+
15.11 1+
7.285
4.4389 2+
3α threshold
0.9722
0.013
0.015
0.0008
12B 1+
The tripleThe triple--alpha process: alpha process: 1212B decayB decay
B 1220.2 ms
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
New detector design
Reduced deadlayer
The tripleThe triple--alpha process: setalpha process: set--upup
5 cm
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
0+
0+
0+7.6542
12.71 1+
15.11 1+
7.285
2+
4.4389
0
2+
E ≈ 13.9(3)MeVΓ ≈ 0.7(3) MeV
E=11.23(5)MeVΓ=2.5(2) MeV
The tripleThe triple--alpha process: alpha process: 1212B & B & 1212NN
Combined R-matrix fit of 12B and 12N
ISOLDE - JYFL
12B20 ms
12N11 ms
[H. Fynbo]
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
The tripleThe triple--alpha process: ratealpha process: rate
[Fynbo, Diget]
Primordial starsType II supernovae
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
New complete kinematics data obtained on
3α decays of 12C from β-decay of 12N and 12B
No low-lying 2+ state found→ Found one at higher energy
Properties of 10.3MeV state established → Interference
Rate of 3α process recalculated
The tripleThe triple--alpha processalpha process
[HOU Fynbo et al., data from ISOLDE and JYFL]
Nature 433 (2005) 136-139
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Nuclear structure studies of waiting point nuclei along the r-process path: neutron-rich Ag, Cd, Sn, and Sb isotopes [Kratz, Walters et al.]
Half livesPn valuesSpectroscopy→ Nuclear structure→ Astrophysics
Nuclear astrophysics: rNuclear astrophysics: r--processprocess
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
R- process abundances• Information from nuclear structure• Waiting point concept valid• No sizeable ν induced reactions
Nuclear masses from
AMDC, 2003
&
ETFSI-Q
Normalized to Nr, (130Te)
“short“ T1/2 “long“ T1/2
RR--processprocess
[K-L Kratz]
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ISOLDE in perspectiveProduction of RIB - the ISOLDE facilityThe low energy Physics programme→ Nuclear Astrophysics→ Ground state properties→ Neutron shell closures→ Applications
REX-ISOLDE PhysicsTowards the future…
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Nuclear ground state propertiesNuclear ground state properties
Atomic methods adopted to nuclear properties→ Spins → Moments→ Isotope shifts
Mass measurements: ISOLTRAP, MISTRAL→ CVC: Vud in CKM matrix→ IMME: M = a + bTz + cTz
2 + dTz3 ?
→ Astrophysics
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Nuclear ground state propertiesNuclear ground state properties
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
AstroAstro--physicsphysics
nuclear synthesis
δm/m ≈ 1·10-7
Weak Weak InteractionsInteractionssymmetry testsCVC hypothesis δm/m < 3·10-8
Nuclear Nuclear Physics Physics
mass formula models
δm/m ≈ 1·10-7
Atomic Atomic Physics Physics
binding energyQED in HCI
δm/m ≤ 1·10-9
General General PhysicsPhysics
fundam. constant test of CPT
δm/m ≤ 1·10-10
Physics &Physics &ChemistryChemistry
Basic information
δm/m ≈ 1·10-6
Mass measurementsMass measurements
[K. Blaum]
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Experimental Access to Ft valueExperimental Access to Ft value
Q – Decay energy ⇔ mass mT1/2 – Half-lifeb – Branching ratioPEC – Electron capture fractionδR – Radiative correctionδC – Isospin symmetry breaking correction
Unitarity of the CKM matrix→ Mean Ft value of all decay pairs contributes to Vud via GV→ Can check unitarity via sum of squares of the first row
)δ,δ,P,b,T,Q(FtFt C/ REC215=
δm/m < 3·10-8
Weak Weak InteractionsInteractionssymmetry tests,CVC hypothesis
d's'b'
dsb
Vud
Vcd
Vtd
Vus Vub
VcbVcs
VtbVts
= · 2A
2V2
ud = GGV
μ
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Superpositionstrong homogeneous
magnetic fieldweak electrostatic 3D
quadrupole field
PENNING trap
Cyclotron frequency: Bmq
c ⋅⋅=π
ν21
z0
r0
B
+ q/m
Typical frequenciesq = e, m = 100 u,B = 6 T⇒ f- ≈ 1 kHz
f+ ≈ 1 MHz
Penning trapPenning trap
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Nd:YAG
cluster ion source
cooling Penning trap
precision Penning trap
532 nm
ISOLDEbeam (DC)
HV platform
RFQ structure
MCP 5
precisionPenningtrap
coolingPenningtrap
carbon clusterion source
2.8-keV ionbunches
laser beam
MCP 3
MCP 1
60 keV
stable alkaliion referencesource
C60 pellet
80
100
120
140
160
180
200
220 32Ar
Mea
n TO
F (μ
s)
νRF − 2842679 (Hz)-40 -30 -20 -10 0 10 20 30
ion beam cooler and buncher
Removal of contaminant ions
determination of cyclotron frequency
B = 4.7 T
B = 6 T
1071195 1071200 1071205 1071210 1071215 1071220 1071225
200
220
240
260
280
300
320
340
Measurement Theoretical Fit
85Rb
Tim
e-of
-flig
ht [
μs]
Excitation frequency [Hz]
ωc = Bqm
The prototype: ISOLTRAPThe prototype: ISOLTRAP
[K. Blaum]
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
1 m
ISOLTRAP in the ISOLDE hallISOLTRAP in the ISOLDE hall
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Previous Status Ft ValuesPrevious Status Ft Values
Existing data for 9 light nuclides from 10C to 54Co
10C
14O
26mAl38mK
42Sc46V
50Mn 54Co
34Cl
3066
3068
3070
3072
3074
3076
3078
3080
Ft(s
)
mother nuclide
Ft = 3072.2(1.4) s
10C 14O 26mAl 34Cl 38mK 42Sc 46V 50Mn 54Co
10C 14O 26mAl 34Cl 38mK 42Sc 46V 50Mn 54Co
tQ
u(F
t) (
s)
0
1
2
3
4
Ft value:⇒ CVC hypothesis confirmed in this mass region |Vud| = 0.9740 ± 0.0005 ± 0.0005
Measurements in heavier nuclides needed
Proposed decay: 74Rb(β +)74Kr
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
TOF Cyclotron Resonance CurveTOF Cyclotron Resonance Curve
e
e
mmmm
ff
--
=refc
refc,
TOF as a function of the excitation frequency
Bmq
πf 21
=c
T1/2 = 65 ms
0 5 10 15 20 25 30220
240
260
280
300
320
340
[A. Kellerbauer et al]
Mea
n TO
F /
μs
νc - 1230051 / Hz
74Rb+Σ = 1100 ions
Determine atomic mass from frequency ratio with a well-known “reference mass”.
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Recent Results Recent Results –– Ft ValuesFt Values
ISOLTRAP:22Mg → 22Na :
δQ=0.28 keV34Ar → 34Cl :
δQ=0.41 keV74Rb → 74Kr :
δQ=4.5 keV
F. Herfurth et al., Eur. Phys. J. A 15, 17 (2002)A. Kellerbauer et al., Phys. Rev. Lett.93, 072502 (2004)M. Mukherjee et al., Phys. Rev. Lett. 93, 150801 (2004)
22Mg
74Rb
[I.S. Towner & J.C. Hardy, PRC 71, 055501 (2005)]
34ArLimit from QEC(38Ca)
62GaJYFLTRAP
LEBIT38Ca
CPT46V
66As
T. Eronen et al., to be published (2005)G. Savard et al., Phys. Rev. Lett. 95, 102501 (2005)
CVC hypothesis confirmed in this region
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
HalfHalf--Life and branchings at ISOLDELife and branchings at ISOLDE
Example: 62GaδT1/2 < 0.1 ms
Lucrecia Total Absorption Gamma-ray (TAgS) spectrometer• Large NaI scintillator• Beta, X-ray, and γ detectors• Neutron and gamma shielding
Ga 62116 ms
Zn 629.13 h
Cu 629.72 m
Ni 62stable
1376?
954 0+
2+
0+
1+?
62Zn
62Ga?
2330
1+2.2 - 4.5MeV
0+
0+
0.44% (2 states 0.3%)
1878 0.027%
99.49%99.88% T = 1, Tz = 1
ExperimentShell model
[Nowacki]
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ISOLDE in perspectiveProduction of RIB - the ISOLDE facilityThe low energy Physics programme→ Nuclear Astrophysics→ Ground state properties→ Neutron shell closures→ Applications
REX-ISOLDE PhysicsTowards the future…
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Physics at the neutron shell closuresPhysics at the neutron shell closures
Validity of magic numbers→ Out of stability, in particular neutron rich nuclei:
• N ~ 20, 50, 82 and 126
→ Physics at the N~20 island of inversion• CoulEx @ REX-ISOLDE• Moment measurements• Fast timing, β-decay
→ Nuclear structure for nuclear astrophysics• r-process (see above)
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
The N~20 island of inversionThe N~20 island of inversion
Cl31
Cl32
Cl33
Cl34
Cl35
Cl36
Cl37
Cl38
Cl39
Cl40
Cl41
Cl42
Cl43
Cl44
Cl45
Cl46
Cl47
Cl48
Cl49
Cl51
16 S27
S28
S29
S30
S31
S32
S33
S34
S35
S36
S37
S38
S39
S40
S41
S42
S43
S44
S45
S46
S47
S48 34
P26
P27
P28
P29
P30
P31
P32
P33
P34
P35
P36
P37
P38
P39
P40
P41
P42
P43
P44
P45
P46 32
14 Si22
Si23
Si24
Si25
Si26
Si27
Si28
Si29
Si30
Si31
Si32
Si33
Si34
Si35
Si36
Si37
Si38
Si39
Si40
Si41
Si42 30
Al22
Al23
Al24
Al25
Al26
Al27
Al28
Al29
Al30
Al31
Al32
Al33
Al34
Al35
Al36
Al37
Al38
Al39 28
12 Mg20
Mg21
Mg22
Mg23
Mg24
Mg25
Mg26
Mg27
Mg28
Mg29
Mg30
Mg31
Mg32
Mg33
Mg34
Mg35
Mg36 26
Na19
Na20
Na21
Na22
Na23
Na24
Na25
Na26
Na27
Na28
Na29
Na30
Na31
Na32
Na33
Na34
Na35
10 Ne16
Ne17
Ne18
Ne19
Ne20
Ne21
Ne22
Ne23
Ne24
Ne25
Ne26
Ne27
Ne28
Ne29
Ne30
Ne32 24
F15
F16
F17
F18
F19
F20
F21
F22
F23
F24
F25
F26
F27
F29 22
8 O12
O13
O14
O15
O16
O17
O18
O19
O20
O21
O22
O23
O24 18
20N11
N12
N13
N14
N15
N16
N17
N18
N19
N20
N21
N22
N23
6 C8
C9
C10
C11
C12
C13
C14
C15
C16
C17
C18
C19
C20
C22
6 84 10 12 14 16
Island of inversionWarburton et al., PRC41 (1990) 1147
New region of deformation…WHY?
WHERE?
Ground state propertiesThibault et al., PRC12 (1975) 644Huber et al., PRC18 (1978) 1978
DeformationDetraz et al., PRC19 (1979) 164Motobayashi et al., PLB346 (1995) 9Keim et al., EPJA8 (2000) 31Pritychenko et al., PRC63 (2000) 011305(R)
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
T. Otsuka et al., EPJA 15 (2002) 151Y. Utsuno et al., PRC 70 (2004) 044307
The N~20 island of inversionThe N~20 island of inversion
Neutron Effective Single Particle energies for 30Si and 24O, relative to 1s1/2. The change is due to the strongly attractive interaction between a proton in 0d5/2 and a neutron in 0d3/2.
Sketch of the sources of the correlation energy of the intruder and the normal states of semi-magic and open-shell nuclei.
N=20
fp-s
hell
sd-s
hell
d3/2s1/2d5/2
p1/2f5/2p3/2f7/2
1/25/23/27/2
3/21/25/2
N=8
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ATD ATD βγγβγγ(t) at N~20(t) at N~20
Ge-1Beta
BaF2 -1
BaF 2-
2
30Na ISOLDE beam
[H. Mach]
30Mg31Mg32Mg
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
IS414: Fast timing ~ N=20IS414: Fast timing ~ N=2030Mg, 32Mg: New scintillators bring new possibilities!30Mg, 32Mg: New scintillators bring new possibilities!
LaBr3:Ce
BaF2
HPGe
All major lines can be resolved in LaBr3 even in singles
The situation improves in coincidences!
The time resolution is similar for large BaF2 (120 ps) and for LaBr3(130 ps) at 60Co.
H. Mach et al.
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ATD ATD βγγβγγ(t) for (t) for 3232MgMg
Centroid Shift data for 32Mg
Cascade 2151-885 keV
Shift due to the lifetime of the 2+ state at 885 keV
Half-life of the 885 keV level in 32Mg
• T1/2(2+) = 16.0(4.2) ps
• B(E2; 01+ → 21+) = 327(87) e2fm4
• Expected final uncertainty of ~2.5 ps
[H. Mach et al.]
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
• Direct lifetime measurement of the 885 keV 2+ state in 32Mg
Currently T1/2 = 15.3(3.5) ps.
The analysis is in progress; further improvement is expected. The final aim is ~2 ps error.
• New fast timing measurements run on 33Mg and 32Mg in 2005
• Search for the E0 transitions in 30Mg also performed in 2005
• New states identified in 30MgEvidence for the 0+ intruder state in 30Mg
ATD ATD βγγβγγ(t) in the (t) in the MgMg regionregion
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
[from O. Niedermaier]
Low E CoulEx, Timing
Intermediate E CoulEx
B(E2)B(E2)’’s for Mg isotopess for Mg isotopes
ATD
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ISOLDE in perspectiveProduction of RIB - the ISOLDE facilityThe low energy Physics programme→ Nuclear Astrophysics→ Ground state properties→ Neutron shell closures→ Applications
REX-ISOLDE PhysicsTowards the future…
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
IS426: MIS426: Möössbauer ssbauer
Fe impurities tracked in Si1-xGex via 57Mn decay (Mössbauer)IIId elements are the most harmful metal impurities
Fe impurities tracked in Si1-xGex via 57Mn decay (Mössbauer)IIId elements are the most harmful metal impurities
[G. Weyer, H. Gunnlaugsson et al.]
FeiV
Interstitial – broadened by diffusion – substitutional
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
IS368: ZnO studiesIS368: ZnO studies
Arsenic is one of few p-type dopants in ZnOThe open question is its location
Arsenic is one of few p-type dopants in ZnOThe open question is its location
Recoil ~0.54eVRecoil ~0.54eV
0 100 200 300 400 500 600 700 800 9000.00.10.20.30.40.50.60.70.80.91.0
substitutional Zn sites SZn
interstitial T sites sum of SZn and T sites73
As f
ract
ion
annealing temperature [°C]Annealing temp (oC)
73As
frac
tion
total SZn+T
Substitutional SZn
Interstitial T
Channeling analysis:
[U. Wahl et al.]
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Medical physicsMedical physics
Example: samarium isotopes “in vivo” dosimetry by positron emission tomography (PET)142Sm (T1/2 = 72min) →142Pm (T1/2 = 40s)
Therapy: 153Sm (T1/2 = 47h)
PET scan of a rabbit 60 min p.i. of ISOLDE produced 142Sm in EDTMP solution
[G. Beyer et al.]
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ISOLDE in perspectiveProduction of RIB - the ISOLDE facilityThe low energy Physics programme→ Nuclear Astrophysics→ Ground state properties→ Neutron shell closures→ Applications
REX-ISOLDE PhysicsTowards the future…
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
The REXThe REX--ISOLDE postISOLDE post--acceleratoraccelerator
REXEBIS
ExperimentsREXTRAP
MASS SEPARATOR
7-GAP RESONATORS
@ 101.28 MHzIHS
RFQ
9-GAP RESONATOR@ 202.56 MHz
3.0 MeV/u 2.2 MeV/u 1.2 MeV/u0.3 MeV/u
ISOLDE beam
REX-ISOLDE
60 keV
Rebuncher
∆E
Accumulation Cooling Ejection
singlychargedions fromREXTRAP
electron gun(0.5 A/ 5kV)
solenoid(2T)
collector
drift tubes
separationfrom residualgas ions
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
The REXThe REX--ISOLDE postISOLDE post--acceleratoraccelerator
Beam preparation needed:Semi-continuous beam (release time in ms range)Emittance ~35 π mm mrad @ 60 keVOccasionally not isobarically nor molecularly clean beams.
Low intensities, short half lives…Breeding time (A/q < 4.5) < 20 msRepetition rate = 50 Hz Beam intensity < 109 /sAround ~ 35% of beamtime
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
REXREX--ISOLDE beamsISOLDE beams
By changing charge breeding time at EBIS it is possible to accelerate all the species produced at ISOLDE!
Radioactive elements accelerated in REX up to 2004
ISOTOPES Charge A/qBreeding time (ms) Comments
9,11Li 2,3+ 4.50,3.00 5–8 Without/with stripper foil, Ne & Ar buffer gases24,25,26,27,28,29Na 6,7,8+ 3.11–4.17 1528,30,31,32Mg 7,8,9+ 3.11–4.29 14–1888Kr 21+ 4.19 3874,76,78Zn 18,20,21+ 3.70–4.11 38,78122,124,126Cd 30,31+ 4.06–4.13 148156Eu 30+ 5.20 38 Only RFQ 300 keV/u153Sm 27,28,30+ 5.10–5.67 30 Only RFQ 300 keV/u70Se 17+ 4.12 33 Molecular sideband17F 5+ 3.40 8 Molecular sideband, with stripper foil110Sn 27+ 4.07 98148Pm 30+ 4.93 38 Only RFQ 300 keV/u
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Main detector setup at REXMain detector setup at REX
MINIBALL24, 6-fold segmented detectors = 144 channels
Resolution: 2.1-2.3 keV (core), 2.3-2.6 (segments)
Photo Peak efficiency: 9.5%, (11.3% w. add-back)
Completely digital electronics after Pre-amp.
Concentric-radial DSSSD
4 sectors, 16 concentric,
24 radial strips. 0.5mm thickness
Pitch: 2mm*3.5 deg
Area: 50 000 mm2 (93% active)
Charged particle detection
CD detector (Si)
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Experimental information:• B(E2), • Spectroscopic factors, • New levels…
Experiments at REXExperiments at REX--ISOLDEISOLDE
Coulomb Excitation: on Ni, PdTransfer Reactions: PE(D), 9Be, 10Be (radioactive)Coulomb Excitation: on Ni, PdTransfer Reactions: PE(D), 9Be, 10Be (radioactive)
REX-ISOLDE RIBγ
Target
RIB + 1n, 2nPPAC
Excited RIB, p, 2α
CD detector
MINIBALL array
Start detector Stop detector
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
REXREX--ISOLDE 2005ISOLDE 2005
IS430: neutron-rich Be isotopes, reactions with 11Be
IS412: Towards the doubly magic 78Ni (Leuven)
IS411: B(E2) measurements around 132Sn (Munich)
IS418: Towards the doubly magic 100Sn(CERN/Lund)
IS423: Mixed symmetry states in 88Kr(Warsaw)
IS405: Shape coexistence in 70Se (CERN/Liverpool)
IS435: Coulex of Cu isotopes, N=40 (CERN/Leuven)
IS415: g-factors in Xe/Te (Bonn)
IS367: study of unbound 10Li via 9Li(d,p) reaction
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
6-
1+
CoulEx 68m,gCu (2.86 MeV/u) @ 120Sn (2.3 mg/cm2)CoulEx 68m,gCu (2.86 MeV/u) @ 120Sn (2.3 mg/cm2)
68Cu 6- (+1+)
120Sn2+-0+
Energy (keV)
68Cu 1+
PRELIMINARY 2005[G. Georgiev, I. Stefanescu, et al.]
IS435: PostIS435: Post--accelerated isomeric beams!accelerated isomeric beams!
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
PRELIMINARYG. Georgiev, I. Stefanescu, et al.
178 keV(prompt)
Doppler corr.
Doppler corr. Sn68Cu 6- (+1+)
693 keV(delayed)
85 keV (delayed)no Doppler corr.
IS435: PostIS435: Post--accelerated isomeric beams!accelerated isomeric beams!
1+(2+)
(3+)(6-)
(4-)
(3-)
84.6
610.5721.6
(?)
0.068Cu
778
956178
693
85
πp3/2 - νg9/2
πp3/2 - νp1/2
T1/2=7.84 ns
68Zn(t,3He)68Cu
68Cu CoulEx @ 120Sn
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Coulomb excitation of Coulomb excitation of 7070SeSe
P. Butler, D. Jenkins et al.
CoulEx 70Se (2.86 MeV/u) @ 104Pd CoulEx 70Se (2.86 MeV/u) @ 104Pd
→ Molecular SeCO beamShape coexistence
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
IS430: d(IS430: d(1111Be,x) Be,x) @ 2.2 MeV/u@ 2.2 MeV/u
9Li + α10Be + t11Be + d12Be + p
9Li + α10Be + t11Be + d12Be + p
[H. Jeppesen, K. Riisager et al.]105 11Be ions @ REX
PRELIMINARY Sep 2005
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
ISOLDE in perspectiveProduction of RIB - the ISOLDE facilityThe low energy Physics programme→ Nuclear Astrophysics→ Ground state properties→ Neutron shell closures→ Applications
REX-ISOLDE PhysicsTowards the future…
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
HIEHIE--ISOLDEISOLDE
The ISOLDE upgradeINTENSITY→ Proton beam increased from 2 to 6 μA (LINAC 4):→ New targets
BEAM QUALITY→ Improve isobaric mass separation: RFQ cooler & new HRS→ ECR + highly-charged ion beamline
ENERGY→ REXtrap and REX-EBIS upgrades→ Staged upgrade of the REX facility to 10 MeV/u
[Butler, Lindroos]
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
CRC, Louvain-la-Neuve, Belgiumdelivering ISOL beams since 1989
REX-ISOLDE, CERNdelivering ISOL beams since 2001
GSI, Darmstadt, Germanydelivering IF beams since 1990
MAFF, Munich, GermanyISOL beams
SPES, Legnaro, ItalyISOL beams
EXCYT, Catania, ItalyISOL beams
GANIL, Caen, Francedelivering IF beams since 1984(SPIRAL) ISOL beams since 2001 Dubna ISOL beamsSPIRAL IIISOL beams
HIE-ISOLDEISOL beams
FAIRIF beams
Accelerated beam facilities in EuropeAccelerated beam facilities in Europe
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
The 2The 2ndnd generation ISOL facilitiesgeneration ISOL facilities
Facility Driver Power Energy Beams
HIE-ISOLDECERN
PS Boosterp @ 1.4 GeV
10 µA10 kW
0.8 – 10.0 MeV/u LINAC
Any from ~850
ISAC-IITRIUMFCanada
p @ 500 MeV 50 kW0.15 – 6.5
MeV/uLINAC
To be developed
SPIRAL2GANILFrance
d @ 40 MeVHI @ 15 MeV/u
200 kW(2ary target)
2 – 25 MeV/uCYCLOTRON
Fission products (mostly)
SPESLegnaro
Italyp @ 100 MeV 200 kW
(2ary target)10 MeV/u
LINACFission
products
MAFFMunich
Germanyn reactor 1014 n/cm2·s 7 MeV/u
LINACFission
products
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
For 90Kr :5 orders of magnitude increase in yield for ISOL
products from existing REX-ISOLDEAt least 2 orders of magnitude increase from a 2nd
generation ISOL facility
100 kW direct production
5 MW spallation n target→ 100 MeV/u RIB
The EURISOL projectThe EURISOL project
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
EURISOLEURISOL--DS 2005DS 2005--20092009
CERN: 3 task leaders+ management
Approved Design Study 2005-2009Project started 1 February 2005
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
Location Driver Post-accelerator
Fragmentseparator
Type of facility
GSI –FAIR synchrotron,heavy ions: 1.5 A GeV
- ‘Super-FRS’ In-Flight
EURISOL protons, 1 GeV,1-5 MW
CW Linac, up to 100 A
MeV- ISOL
USA: RIARare IsotopeAccelerator
900 MeV protonsheavy ions:
400 A MeV, 100 kW
Linac up to 8–15 A
MeV
4-dipoleSeparator
ISOLIn-Flight
JAPAN: RIKEN RIB Factory
Ring-cyclotronsup to 400 A MeV (lightions); up to 150 A MeV
(heavy ions)
-
3 Fragmentseparators
Storage & cooler rings
In-Flight
Next generation RIB facilitiesNext generation RIB facilities
L.M. Fraile Séminaire DPNC, UGe 25 Jan 2006
SPL
HIE-ISOLDEPS booster
A possible EURISOL layoutA possible EURISOL layout
[P Butler]