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NCSP IE and T&E Activities at Sandia Nuclear Criticality Safety Program Technical Program Review Washington, D.C. March 15, 2017 Presented by Gary A. Harms Sandia National Laboratories SAND2017-2772 PE Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy’s National Nuclear Security Administration under contract DE-AC04-94AL85000.

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Page 1: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

NCSP IE and T&E Activities at Sandia

Nuclear Criticality Safety ProgramTechnical Program Review

Washington, D.C.March 15, 2017

Presented byGary A. Harms

Sandia National LaboratoriesSAND2017-2772 PE

Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of

Energy’s National Nuclear Security Administration under contract DE-AC04-94AL85000.

Page 2: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 2

SAND2017-2772 PE

Hands-On Criticality Safety Trainingat Sandia

• Two hands-on critical experiment classes are currently offered.

• The first is part of a two-week class for Nuclear Criticality Safety Professionals, 1 week at LANL and one week at Sandia or at NCERC.

• The other is a one-week class at Sandia for Nuclear Material Managers.

• Information about the classes and how to register is at http://ncsp.llnl.gov/classMain.html

Page 3: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 3

SAND2017-2772 PE

The Classes Continue to Servea Diverse Audience

Page 4: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 4

SAND2017-2772 PE

The Sandia Classes

• The Sandia classes are a series of four experiments– Approach on fuel– Approach on moderator height– “Split table” approach– Fuel removal approach

• Lectures on various subjects are integrated with the experiments

• Remember: http://ncsp.llnl.gov/classMain.html

Page 5: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 5

SAND2017-2772 PE

Sandia Integral Experiment Requests

IER Title Sponsor CED

206 Re-establish the 4.3% Enriched Critical Experiment Capability at Sandia SNL 3B

209 7uPCX 0.855 cm Pitch, Variable Depth Pure Water Moderator SNL 3A

230 Characterize the Thermal Capabilities of the 7uPCX SNL 2

285 Titanium Cross Sections in a Thermal Application (7uPCX) SRNL

304 Temperature Dependent Critical Benchmarks ORNL 1

305 Critical Experiments with UO2 Rods and Molybdenum foils IRSN 1

306 Critical Experiments with UO2 Rods and Rhodium Foils IRSN 1

441 Epithermal HEX Lattices with SNL 7uPCX Fuel for Testing Nuclear Data ORNL 1

451 Titanium Cross Sections in a Thermal Application (BUCCX) SRNL 3B

452 Inversion Point of the Isothermal Reactivity Coefficient SNL Pre-1

Page 6: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 6

SAND2017-2772 PE

Sandia Integral Experiment Requests

IER Title Sponsor CED

206 Re-establish the 4.3% Enriched Critical Experiment Capability at Sandia SNL 3B

209 7uPCX 0.855 cm Pitch, Variable Depth Pure Water Moderator SNL 3A

230 Characterize the Thermal Capabilities of the 7uPCX SNL 2

285 Titanium Cross Sections in a Thermal Application (7uPCX) SRNL

304 Temperature Dependent Critical Benchmarks ORNL 1

305 Critical Experiments with UO2 Rods and Molybdenum foils IRSN 1

306 Critical Experiments with UO2 Rods and Rhodium Foils IRSN 1

441 Epithermal HEX Lattices with SNL 7uPCX Fuel for Testing Nuclear Data ORNL 1

451 Titanium Cross Sections in a Thermal Application (BUCCX) SRNL 3B

452 Inversion Point of the Isothermal Reactivity Coefficient SNL Pre-1

Page 7: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 7

SAND2017-2772 PE

IER-285

• This experiment was done to answer a request from SRNL for integral critical experiments with titanium in a thermal system

• This experiment series was done as a set of progressive fuel-rod-replacement experiments in the 7uPCX critical assembly

• We used titanium and aluminum replacement rods• A benchmark evaluation (LEU-COMP-THERM-097) has

been published in the International Handbook of Evaluated Criticality Safety Benchmark Experiments

• We are working on a set of experiments (IER-451) with titanium sleeves on another set of fuel rods (BUCCX)

Page 8: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 8

SAND2017-2772 PE

Case 1

Fuel RodEmpty Grid Location

Fuel 1457Expt. 0Empty 0Total 1457

Page 9: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 9

SAND2017-2772 PE

Case 16

Fuel RodEmpty Grid LocationAluminum Experiment Rod

Fuel 1429Expt. 36 AlEmpty 0Total 1465

Page 10: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 10

SAND2017-2772 PE

Case 8

Fuel RodEmpty Grid LocationTitanium Experiment Rod

Fuel 1573Expt. 36 TiEmpty 0Total 1609

Page 11: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 11

SAND2017-2772 PE

Case 18

Fuel RodEmpty Grid Location

Fuel 1037Expt. 0Empty 172Total 1209

Page 12: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 12

SAND2017-2772 PE

Case 19

Fuel RodEmpty Grid LocationAluminum Experiment Rod

Fuel 1097Expt. 36 AlEmpty 136Total 1269

Page 13: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 13

SAND2017-2772 PE

Case 24

Fuel RodEmpty Grid LocationTitanium Experiment Rod

Fuel 1485Expt. 36 TiEmpty 136Total 1657

Page 14: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 14

SAND2017-2772 PE

A comparison of the neutron spectrain the titanium rods

1 10 9 1 10 8

1 10 7 1 10 6

1 10 5 1 10 4

1 10 3 1 10 2

1 10 1 1 100

1 101 1 102

0 100

1 10 3

2 10 3

3 10 3

4 10 3

5 10 3

0.80 cm Pitch1.60 cm Pitch

Energy (MeV)

Nor

mal

ized

Let

harg

y Fl

ux

Page 15: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 15

SAND2017-2772 PE

A comparison of the capture ratein the titanium rods

1 10 9 1 10 8

1 10 7 1 10 6

1 10 5 1 10 4

1 10 3 1 10 2

1 10 1 1 100

1 101 1 102

0 100

5 10 3

1 10 2

1.5 10 2

0.80 cm Pitch1.60 cm Pitch

Energy (MeV)

Nor

mal

ized

Ti C

aptu

re R

ate

Page 16: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 16

SAND2017-2772 PE

The bottom line in the LCT097 evaluation

• 24 benchmark configurations– 17 at 0.8 cm pitch

• 1 with no experiment rods• 8 with aluminum experiment rods• 8 with titanium experiment rods

– 7 at 1.6 cm pitch• 1 with no experiment rods• The remainder with 36 Ti + Al experiment rods• 0, 4, 9, 16, 25, 36 titanium experiment rods

• Benchmark model keffs from 0.9991 to 0.9998• Overall uncertainties in keff of 0.0007 to 0.0011

Page 17: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 17

SAND2017-2772 PE

MCNP6.1.1 + ENDF/B-VII.0 Calculation of Benchmark Models

Expt. Ti 0 4 9 16 25 36 36 36 36 0 0 0 0 0 0 0 0 0 0 4 9 16 25 36 Ti Expt.Rods Al 0 0 0 0 0 0 0 0 0 4 9 16 25 36 36 36 36 0 36 32 27 20 11 0 Al Rods

Case 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 Case

Increasing TiIncreasing Al

Pitch Ti

Pitch Al

Ti Al

1.60.8

1.13 1.6 2.4

1.13

1.6

2.40.8

Experiment Rod Pitch (cm)

0 5 10 15 20 250.002

0.0015

0.001

0.0005

0

0.0005

0.001ENDF/B-VII.0

Case Number

Rea

ctiv

ity O

ffset

Page 18: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 18

SAND2017-2772 PE

Add ENDF/B-VII.1 cross sections

Expt. Ti 0 4 9 16 25 36 36 36 36 0 0 0 0 0 0 0 0 0 0 4 9 16 25 36 Ti Expt.Rods Al 0 0 0 0 0 0 0 0 0 4 9 16 25 36 36 36 36 0 36 32 27 20 11 0 Al Rods

Case 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 Case

0 5 10 15 20 250.002

0.0015

0.001

0.0005

0

0.0005

0.001ENDF/B-VII.0ENDF/B-VII.1

Case Number

Rea

ctiv

ity O

ffset Increasing Ti

Increasing Al

Pitch Ti

Pitch Al

Ti Al

1.60.8

1.13 1.6 2.4

1.13

1.6

2.40.8

Experiment Rod Pitch (cm)

Page 19: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 19

SAND2017-2772 PE

The experiments test changes to the Ti cross sections

0.05 0.04 0.03 0.02 0.01 00.0005

0

0.0005

0.001

0.0015ENDF/B-VII.0ENDF/B-VII.1

Titanium Reactivity

Tita

nium

to A

lum

inum

Rea

ctiv

ity D

iffer

ence

The 48Ti capture cross section was increased about 6% between ENDF/B-VII.0 and ENDF/B-VII.1

Page 20: NCSP IE and T&E Activities at Sandia€¦ · SAND2017-2772 PE Sandia Integral Experiment Requests IER Title Sponsor CED 206 Re-establish the 4.3% Enriched Critical Experiment Capability

Sandia NCSP IE and T&E – p. 20

SAND2017-2772 PE

Sandia Integral Experiment Requests

IER Title Sponsor CED

206 Re-establish the 4.3% Enriched Critical Experiment Capability at Sandia SNL 3B

209 7uPCX 0.855 cm Pitch, Variable Depth Pure Water Moderator SNL 3A

230 Characterize the Thermal Capabilities of the 7uPCX SNL 2

285 Titanium Cross Sections in a Thermal Application (7uPCX) SRNL

304 Temperature Dependent Critical Benchmarks ORNL 1

305 Critical Experiments with UO2 Rods and Molybdenum foils IRSN 1

306 Critical Experiments with UO2 Rods and Rhodium Foils IRSN 1

441 Epithermal HEX Lattices with SNL 7uPCX Fuel for Testing Nuclear Data ORNL 1

451 Titanium Cross Sections in a Thermal Application (BUCCX) SRNL 3B

452 Inversion Point of the Isothermal Reactivity Coefficient SNL Pre-1