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Predictive relationships for the permeability of unconsolidated sands based on SIP and pore surface fractal dimensions Malcolm Ingham and Sheen Joseph, Victoria University of Wellington, PO Box 600, Wellington, New Zealand Permeability prediction based on S por and D For sandstone samples Zhang &Weller (2014) have demonstrated a relationship between S por and the fractal dimension (D) of the pore surface and incorporated D into a more general form of the PaRiS model (originally proposed by Pape et al. (1987)) to predict permeability = 1 8 ( 2 ) 2−4 −3 2 2 −3 (1) We (Joseph et al., 2016) have made SIP and permeability measurements on unconsolidated sand samples both of individual size fractions and mixtures of sizes. For these samples S por has been calculated from measurements of porosity and the masses and mean grain diameters of the samples. From the calculated values of S por the fractal dimension of the pore surface has been estimated using a relationship, based on that of Zhang & Weller (2014) =2+ log −log( 2 ) log 2 (2) in which the effective hydraulic radius = 8 . Compared to sandstone samples reported by Zhang & Weller, for which D increases with S por , we find D for our unconsolidated samples to be very close to 2 for 10 m (Figure 1). A plot of permeability predicted by (1) against measured permeability is in excellent agreement (Figure 2). Use of average values of D (2.0 for unconsolidated samples and 2.307 for sandstone samples) still gives good predictions of permeability (Figure 2). Permeability prediction based on " and Assuming D = 2 for the unconsolidated sands, the predictive relationship for permeability based on the value of " at 1 Hz is: = 1.357 10 −28 8 " −4.739 (3) with k in m 2 and " in S/m. The comparable relationship for predicting permeability from the Cole-Cole time constant is = 5.247 10 −10 8 1.113 (4) with k in m 2 and in seconds. Plots of the permeability predicted by these equations against the measured permeability are shown in Figures 5 and 6. For these samples, predictions based on " show a considerable degree of scatter (Figure 5). Predictions based on (Figure 6(a)) are much less scattered but tend to overestimate the permeability. If an average value of D (1.932) is used, and equations (3) and (4) adjusted appropriately, much better predictions of k are obtained (e.g. Figure 6(b)). Relationships between S por and SIP parameters Although the use of the PaRiS model gives excellent predictions of permeability, the requirement to have a knowledge of S por makes it difficult to apply in a field setting. It is therefore appropriate to seek relationships between S por and parameters that are readily obtainable from field measurements. Two such parameters are the imaginary part of the complex conductivity (" ) measured at a frequency of 1 Hz, and the Cole- Cole time constant (). Derived fits between these parameters and S por for the unconsolidated sands are shown in Figures 3 and 4 and, with the assumption of D = 2, lead to predictive relationships for permeability based on and . 1E-17 1E-16 1E-15 1E-14 1E-13 1E-12 1E-11 1E-10 1E-09 1E-08 1.E-17 1.E-16 1.E-15 1.E-14 1.E-13 1.E-12 1.E-11 1.E-10 1.E-09 k pred (m 2 ) k (m 2 ) Figure 1: Calculated value of pore fractal dimension D as a function of specific internal surface S por . Diamonds– unconsolidated sand samples; triangles– sandstone samples (Zhang & Weller, 2014). Figure 2: Permeability predicted by equation (1) plotted against measured permeability. Diamonds unconsolidated sand samples using calculated values of D; squares - unconsolidated sand samples using D = 2.0; triangles – sandstone samples (Zhang & Weller, 2014) using measured values of D; circles - . sandstone samples using D = 2.307. y = 5.068E-07x 4.949E-01 R² = 4.254E-01 1.E-05 1.E-04 1.E-03 1.E+03 1.E+04 1.E+05 1.E+06 s // at 1 Hz (Sm -1 ) S por (m -1 ) y = 6.657E+09x -2.019E+00 R² = 8.498E-01 1.E-01 1.E+00 1.E+01 1.E+02 1.E+03 1.E+04 1.E+05 1.E+06 (s) S por (m -1 ) 1.0 1.5 2.0 2.5 3.0 1.E+03 1.E+04 1.E+05 1.E+06 1.E+07 1.E+08 1.E+09 D S por (m -1 ) 1E-17 1E-15 1E-13 1E-11 1E-09 1.E-17 1.E-15 1.E-13 1.E-11 1.E-09 k pred (m 2 ) k (m 2 ) Figure 3: Relationship between " 1 , the imaginary part of the conductivity at a frequency of 1 Hz, and S por . Figure 4: Relationship between , the Cole- Cole time constant, and S por . 1E-12 1E-11 1E-10 1E-09 1E-08 1E-12 1E-11 1E-10 1E-09 k pred (m 2 ) k (m 2 ) 1E-12 1E-11 1E-10 1E-09 1E-08 1E-12 1E-11 1E-10 1E-09 k pred (m 2 ) k (m 2 ) Figure 5: Plot of permeability predicted by equation (3) against measured permeability for unconsolidated sand samples. Figure 6: (a) Plot of permeability predicted by equation (4) against measured permeability for unconsolidated sand samples; (b) improved prediction of permeability based on the Cole-Cole time constant obtained by using an average value of pore fractal dimension (D) of 1.932. 1E-12 1E-11 1E-10 1E-09 1E-12 1E-11 1E-10 1E-09 k pred (m 2 ) k (m 2 ) (a) (b) Conclusions For unconsolidated sand samples for which the effective hydraulic radius is greater than 10 m the calculated pore surface fractal dimension is close to, but just less than, 2. Using the calculated values of D in the generalized PaRiS model (equation (1)) gives excellent predictions of permeability. Using a constant value of 2 leads to a slight overestimate of permeability. Power law relationships between both " and and S por allow predictive relationships based on these parameters to be developed. Assumption of D = 2 in these relationships, as representative of unconsolidated samples, leads to an overestimation of k. However, use of an average value of D, slightly lower than 2, gives improved predictions using both " and . References Joseph, S., Ingham, M. & Gouws, G., 2016. Water Resources Research, In Press. Pape, H., Reipe, L. & Schopper, J.R., 1987. Journal of Microscopy, 148, 121-147. Zhang, Z. & Weller, A., 2014. Geophysics,79, D377-D387. Contact details malcolm [email protected] sheen [email protected] s s

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Page 1: Predictive relationships for the permeability of ... › fileadmin › user_upload › AP04.pdf · 1.E+03 1.E+04 1.E+05 1.E+06 1.E+07 1.E+08 1.E+09 D S por (m-1) 1E-17 1E-15 1E-13

Predictive relationships for the permeability of unconsolidated sands based on SIP and pore surface fractal dimensions

Malcolm Ingham and Sheen Joseph, Victoria University of Wellington, PO Box 600, Wellington, New Zealand

Permeability prediction based on Spor and D

For sandstone samples Zhang &Weller (2014) have demonstrated arelationship between Spor and the fractal dimension (D) of the poresurface and incorporated D into a more general form of the PaRiSmodel (originally proposed by Pape et al. (1987)) to predictpermeability

𝑘 =1

8𝐹(𝜆𝑁2)

2𝐷−4

𝐷−3𝑆𝑝𝑜𝑟

2

2

𝐷−3(1)

We (Joseph et al., 2016) have made SIP and permeabilitymeasurements on unconsolidated sand samples both of individualsize fractions and mixtures of sizes.

For these samples Spor has been calculated from measurements ofporosity and the masses and mean grain diameters of the samples.

From the calculated values of Spor the fractal dimension of the poresurface has been estimated using a relationship, based on that ofZhang & Weller (2014)

𝐷 = 2 +log 𝑆𝑝𝑜𝑟 −log( 2 𝑟𝑒𝑓𝑓)

log 𝑟𝑒𝑓𝑓 𝜆𝐻2𝑂(2)

in which the effective hydraulic radius 𝑟𝑒𝑓𝑓 = 8𝑘𝐹.

Compared to sandstone samples reported by Zhang & Weller, forwhich D increases with Spor, we find D for our unconsolidatedsamples to be very close to 2 for 𝑟𝑒𝑓𝑓 10 m (Figure 1).

A plot of permeability predicted by (1) against measuredpermeability is in excellent agreement (Figure 2).

Use of average values of D (2.0 for unconsolidated samples and2.307 for sandstone samples) still gives good predictions ofpermeability (Figure 2).

Permeability prediction based on 𝝈" and Assuming D = 2 for the unconsolidated sands, the predictive

relationship for permeability based on the value of 𝜎" at 1 Hz is:

𝑘 =1.357 𝑥 10−28

8𝐹𝜎"−4.739 (3)

with k in m2 and 𝜎" in S/m. The comparable relationship for predicting permeability from the

Cole-Cole time constant is

𝑘 =5.247 𝑥 10−10

8𝐹𝜏1.113 (4)

with k in m2and in seconds. Plots of the permeability predicted by these equations against the

measured permeability are shown in Figures 5 and 6. For these samples, predictions based on 𝜎" show a considerable

degree of scatter (Figure 5). Predictions based on (Figure 6(a)) are much less scattered but

tend to overestimate the permeability. If an average value of D (1.932) is used, and equations (3) and (4)

adjusted appropriately, much better predictions of k are obtained(e.g. Figure 6(b)).

Relationships between Spor and SIP parameters Although the use of the PaRiS model gives excellent predictions of

permeability, the requirement to have a knowledge of Spor makes itdifficult to apply in a field setting. It is therefore appropriate to seekrelationships between Spor and parameters that are readilyobtainable from field measurements.

Two such parameters are the imaginary part of the complexconductivity (𝜎" ) measured at a frequency of 1 Hz, and the Cole-Cole time constant ().

Derived fits between these parameters and Spor for theunconsolidated sands are shown in Figures 3 and 4 and, with theassumption of D = 2, lead to predictive relationships forpermeability based on 𝜎“ and .

1E-17

1E-16

1E-15

1E-14

1E-13

1E-12

1E-11

1E-10

1E-09

1E-08

1.E-17 1.E-16 1.E-15 1.E-14 1.E-13 1.E-12 1.E-11 1.E-10 1.E-09

k pre

d (m

2 )

k (m2)

Figure 1: Calculated value of pore fractaldimension D as a function of specific internalsurface Spor. Diamonds– unconsolidated sandsamples; triangles– sandstone samples (Zhang& Weller, 2014).

Figure 2: Permeability predicted by equation(1) plotted against measured permeability.Diamonds – unconsolidated sand samplesusing calculated values of D; squares -unconsolidated sand samples using D = 2.0;triangles – sandstone samples (Zhang & Weller,2014) using measured values of D; circles - .sandstone samples using D = 2.307.

y = 5.068E-07x4.949E-01

R² = 4.254E-01

1.E-05

1.E-04

1.E-03

1.E+03 1.E+04 1.E+05 1.E+06

s//

at

1 H

z (S

m-1

)

Spor (m-1)

y = 6.657E+09x-2.019E+00

R² = 8.498E-01

1.E-01

1.E+00

1.E+01

1.E+02

1.E+03 1.E+04 1.E+05 1.E+06

(s

)

Spor (m-1)

1.0

1.5

2.0

2.5

3.0

1.E+03 1.E+04 1.E+05 1.E+06 1.E+07 1.E+08 1.E+09

D

Spor (m-1)

1E-17

1E-15

1E-13

1E-11

1E-09

1.E-17 1.E-15 1.E-13 1.E-11 1.E-09

k pre

d (m

2)

k (m2)

Figure 3: Relationship between 𝜎"1𝐻𝑧 , theimaginary part of the conductivity at afrequency of 1 Hz, and Spor.

Figure 4: Relationship between , the Cole-Cole time constant, and Spor.

1E-12

1E-11

1E-10

1E-09

1E-08

1E-12 1E-11 1E-10 1E-09

k pre

d(m

2)

k (m2)

1E-12

1E-11

1E-10

1E-09

1E-08

1E-12 1E-11 1E-10 1E-09

k pre

d(m

2)

k (m2)

Figure 5: Plot of permeability predicted byequation (3) against measured permeabilityfor unconsolidated sand samples.

Figure 6: (a) Plot of permeability predicted by equation (4) against measured permeability forunconsolidated sand samples; (b) improved prediction of permeability based on the Cole-Coletime constant obtained by using an average value of pore fractal dimension (D) of 1.932.

1E-12

1E-11

1E-10

1E-09

1E-12 1E-11 1E-10 1E-09

k pre

d(m

2)

k (m2)

(a) (b)

Conclusions For unconsolidated sand samples for which the effective hydraulic

radius is greater than 10 m the calculated pore surface fractaldimension is close to, but just less than, 2.

Using the calculated values of D in the generalized PaRiS model(equation (1)) gives excellent predictions of permeability. Using aconstant value of 2 leads to a slight overestimate of permeability.

Power law relationships between both 𝜎" and and Spor allowpredictive relationships based on these parameters to bedeveloped.

Assumption of D = 2 in these relationships, as representative ofunconsolidated samples, leads to an overestimation of k. However,use of an average value of D, slightly lower than 2, gives improvedpredictions using both 𝜎" and .

ReferencesJoseph, S., Ingham, M. & Gouws, G., 2016. Water Resources Research,In Press.Pape, H., Reipe, L. & Schopper, J.R., 1987. Journal of Microscopy, 148,121-147.Zhang, Z. & Weller, A., 2014. Geophysics,79, D377-D387.

Contact [email protected]@gmail.com

s s