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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 1 Summary of RED-IMPACT results on the Impact of P&T on the High Level Waste Management E.M. Gonzalez (CIEMAT), on behalf of the RED-IMPACT collaboration 10 th International Exchange Meeting on Partitioning and Transmutation, IEMPT10 Mito (Japan) 6-10 October 2008

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Page 1: Summary of RED-IMPACT results on the Impact of P&T on · PDF fileRomania: CITON Slovakia: DECOM, ... Summary of RED-IMPACT results on the Impact of P&T IEMPT10 / Mito ... For granite

Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 1

Summary of RED-IMPACT results on the Impact of P&T on the High Level Waste

Management

E.M. Gonzalez (CIEMAT), on behalf of the RED-IMPACT collaboration

10th International Exchange Meeting on Partitioning and Transmutation, IEMPT10

Mito (Japan) 6-10 October 2008

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 2

RED-IMPACTImpact of Partitioning, Transmutation and Waste Reduction

Technologies on the Final Nuclear Waste Disposal

Research50%

Waste Agencies

18%

Nuclear Industry &

Utilities32%

23 partners + 2 subcontractors KTH-Sweden: CoordinatorFZJ-Germany: Co-CoordinatorBelgium: BN; SCK-CENCzech Republic: NRI; RAWRAEC: ITU-KarlsruheFrance: Areva ANP, CEA; COGEMAGermany:FANP; GRS; IER; KKPNetherlands: NRGRomania: CITONSlovakia: DECOM, VUJESpain: CIEMAT; EA; ENRESAUK: NexiaSolutions; NIREX; UCEC CONTRACT NO. FI6W-CT-2004-002408

Duration: March 2004 – September 2007

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 3

RED-IMPACT

• WP1: Review of waste management and transmutation strategies, selection of fuel cycles scenarios

• WP2: Feasibility of the industrial deployment of selected scenarios and their impact on waste management

• WP3: Assessment of waste streams, waste features, leach resistance, heat generation, reprocessing capability etc. for selected fuel cycles.

• WP4: Assessment of the benefits of P&T/C in advanced fuel cycles for waste management and geological disposal.

• WP5: Economic, environmental and societal assessment of fuel cycle strategies

• WP6: Synthesis and dissemination of results

After a comprehensive inventory of existing and foreseen nuclear fuelcycle facilities in Europe, including a review of worldwide ongoing R&D programson P&T, and assuming the potential evolution of P&T technologies and advancedfuel cycles (including Gen III & Gen IV reactors and ADS), the project hasestimated the effect of P&T on waste management when using existing deepgeological repository designs.

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 4

Scenarios for Fuel Cycles• Industrial scenarios @ equilibrium

– Scenario A1: (reference) : once through open cycle with Gen-II / III reactors

– Scenario A2 : mono-recycling of plutonium in Gen-III reactors (+ variants)

– Scenario A3 : Multirecycling of Pu (only) in Sodium Fast Reactors (EFR)

• Innovative scenarios @ equilibrium– Scenario B1 : Multi-recycling of Pu & MA in Sodium Fast

Reactors (EFR) plus advanced PUREX

– Scenario B2 : mono-recycling of plutonium in Gen-III reactors and burning of Minor Actinides in ADS plus advanced PUREX & PYRO

– Scenario B3 : mono-recycling of plutonium in Gen-III reactors + burning of plutonium in Gen-IV fast reactors + burning of Minor Actinides in ADS including advanced PUREX and PYRO (reduced efforts)

• Transition Scenarios

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 5

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Scenarios for Fuel Cycles

A1

B1

B2

B3 A3

A2

(NEA /Red-Impact)

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 6

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Scenarios for Fuel CyclesOnly presently deployed actinide (Pu) recycleHLW Waste Streams:

Irradiated U (enriched)MOX Spent fuelPurex HLW:

FF, 100% MAU & Pu losses

Pu reprocessing in LWR (single)The reference cooling time is 50 yearsUO2 Initial enrichment in 235U = 4.20% /

MOX 8.5% PuVariants:

Multiple recycling of Pu in LWR Different reactors and fuels for Pu recyclingDifferent fuel burnup for Pu recycling

Enrichment

U natural U Depleted

UOX Fabr.

MOX Fabr.

UOX irradiation

in LWR

MOX irradiation

in LWR

PUREXReproc.

Cooling:

2 years

Irradiated enriched U

Final HL WasteDisposal

Pu

MA, FP, Pu lossesIrr. MOX

Storage Storage

Enrichment

U natural U Depleted

UOX Fabr.

MOX Fabr.

UOX irradiation

in LWR

MOX irradiation

in LWR

PUREXReproc.

Cooling:

2 years

Irradiated enriched U

Final HL WasteDisposal

Pu

MA, FP, Pu lossesIrr. MOX

Storage Storage

4.20%235U

50 years

50GWd/THM

8.5%Pu

PUREXReproc .

Irradiated

depleted U

Cooling:

2 years

Pu

Storage

PUREXReproc .

Irradiated

depleted U

Cooling:

2 years

Pu

Storage

50 years

50GWd/THM

@ Surface

@ Deep underground

Scenario A2

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 7

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Scenarios for Fuel Cycles

Final WasteDisposal

FP+ReprocessingLosses U + Pu +MA

U Depleted

MOX Fabr.

MOX irradiationin LMFR

Storage PUREXReproc.

Storage

Pu + MA

45 years

5 yearsFissil part : 136 GWd/tHMAxial blankets : 15 GWd/tHMRadial blankets : 24 GWd/tHM

23.2% Pu, 2.7% MA

2 years

Irradiated U Depleted

Scenario B1

Generation IV fast reactorEFR CD9/91, Core, Axial and Radial Blankets23.2% Pu and 2.7% MA in “MOX”

Variants: Separate handling of FP heat sources (Cs+Sr)- 99% Cs & Sr separated from HLW - 99% Sr separated from HLW- Increased FF loading of Univ. Canister (40 → 60 kg)- Increased FF loading + 99% Cs & Sr separated from HLW- Increased FF loading + 99% Sr separated from HLW

HLW Waste Streams:Irradiated U (depleted)Purex HLW:

FF, MA, U, Pu losses

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 8

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Scenarios for Fuel Cycles

Scenario B2

Simplified double strata: with LWR UOX, Mono-recycling of PU in LWR and multi-recycling of Pu+MA in fast spectrun ADS (no Fast reactor)Variants: ADS with TRU Oxide fuel in ZrO2 inert matrix

(+ 8.5% Pu content in MOX and 5 years LWR UOX spent fuel cooling time)Separate handling of FP heat sources (Cs+Sr) (studied in B1)

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 9

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Packages

4.30 m

0.12 m

4.54 m0.9 m

0.7 m4.30 m4.30 m

0.12 m0.12 m

4.54 m0.9 m

0.7 m

0.9 m

0.7 m

ILW: UC-C

Spent Fuel: SPA

HLW:UC-V

Number of packages, volume and gallery length, heat and radiation levels (n, γ)

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 10

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Deep Geological Repositories

Granite SpainGranite Czech

Republic

Salt Germany Boom Clay Belgium

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 11

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

HLW: Waste Streams and Isotopic v.

Fractions of main chemical elements incorporated into the vitrified HLW (%)

101010101010Carbon

000000Fuel Assembly Structurals(particles)

B2B1A3

100100100100100100Others

1-----Zr of the ADS fuel matrix

(also for the Zr-fission product)

111111Chlorine

Blankets + Core (FR)

0

100

100

1

0

0.1

0.1

MOX (PWR)

Extended PUREX

0

100

0

1

0

0.1

0.1

ZrN +TRUN(ADS)

PYRO

0

100

100

1

0

0.1

0.1

UOX (PWR)

Extended PUREX

Blankets + Core (FR)UOX (PWR)REPROCESSED FUEL

000HLIGHT

ELEMENTS(Fuel Impurities)

100100100Others

111Iodine

Noble Metals

Noble Gases

MA

U and Pu

FISSION PRODUCTS

(FP)

ACTINIDES(An)

REPROCESSING TYPE

SCENARIO

Extended PUREX

Standard PUREX

Standard PUREX

100100100

000

0.1100100

0.10.10.1

A2

101010101010Carbon

000000Fuel Assembly Structurals(particles)

B2B1A3

100100100100100100Others

1-----Zr of the ADS fuel matrix

(also for the Zr-fission product)

111111Chlorine

Blankets + Core (FR)

0

100

100

1

0

0.1

0.1

MOX (PWR)

Extended PUREX

0

100

0

1

0

0.1

0.1

ZrN +TRUN(ADS)

PYRO

0

100

100

1

0

0.1

0.1

UOX (PWR)

Extended PUREX

Blankets + Core (FR)UOX (PWR)REPROCESSED FUEL

000HLIGHT

ELEMENTS(Fuel Impurities)

100100100Others

111Iodine

Noble Metals

Noble Gases

MA

U and Pu

FISSION PRODUCTS

(FP)

ACTINIDES(An)

REPROCESSING TYPE

SCENARIO

Extended PUREX

Standard PUREX

Standard PUREX

100100100

000

0.1100100

0.10.10.1

A2

Red-Impact- HLW hypothesis

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 12

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Derived magnitudes: Heat Load

1,E-02

1,E-01

1,E+00

1,E+01

1,E+02

1,E+03

1,E+04

1 10 100 1000 10000Cooling time (a)

Hea

t afte

r unl

oadi

ng (W

/TW

he) B2 B1 A3

A2 A1

Red-Impact HLWs (total) thermal powerevolution with time

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 13

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Derived magnitudes: Heat Load

1,E-02

1,E-01

1,E+00

1,E+01

1,E+02

1,E+03

1,E+04

1 10 100 1000 10000Cooling time (a)

Hea

t afte

r unl

oadi

ng (W

/TW

he)

B2 - ActinB1 - ActinA3 - ActinA2 - ActinA1 - ActinB2 - FPB1 - FPA3 - FPA2 - FPA1 - FP

Red-Impact HLWs (total) thermal powerevolution with time(Actinides and Fission Fragments contributions)

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 14

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Derived magnitudes: Heat Load

HLW total thermal power per TWeh in the scenarios

Scenario A1 A2 A3 B1 B2

Fuel Type LWR-UOx

LWR-MOx

LWR-UOx

(reproc.)

Total A2

FR-MOx (reproc.)

FR-MOx (reproc.)

LWR-UOx

(reproc.)

LWR-MOx

(reproc.)

ADS-TRU-Nitride

Total B2

Thermal Power (W) after 50 years

(emplacement time) 2096 836 1205 2042 1270 713 869 86 145 1100

Thermal Power (W) after 150 years 766 457 275 732 384 73 83 9 17 108

Thermal Power (W) after 1000 years 185 117 27 144 82 2 0 0 1 1

Thermal Power (W) after 10000 years 43 24 2 26 7 2 0 0 0 1

Red-Impact HLWs thermal power (total per waste stream)

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 15

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

HLW Heat Load -> Capacity

Red-Impact temperature at the interface between the gallery lining and the Boom Clay (Belgian repository concept for disposal in clay)

The main thermal limitation for the repository concept is that the maximum temperature at the gallery lining / Boom Clay interface has to remain below 100 °C. For granite repositories the temperature in the bentonite buffer has to remain lower than 100 °C

time (years)

Length of the needed HLW disposal galleries B1/A1 reduced by 3

RED-Impact cases for different Granite/Clay repositories 1.6 < B1/A1 < 6

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 16

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

HLW Heat Load -> CapacityCs & Sr separation from HLW

• Two variant scenarios of B1 in which it is assumed that only Sr orboth Cs and Sr are separated from the HLW prior to vitrificationstudied.

• Separating Sr only, results in a further reduction of the neededgallery length with a factor 1.5, or about a factor 5 in comparisonwith the "once through" reference fuel cycle A1.

• Separating Cs and Sr makes that the thermal output of the vitrifiedHLW is so low that cooling times are not longer needed, or thatother repository concepts can be used.

• However, for the estimation of the needed gallery length oneshould not forget that the separated Cs has to be disposed of in ageological repository also, because it contains the long-lived 135Csisotope (half-life 2.3 million years).

• Separating Cs and Sr, if it is assumed that the conditioned Cs-waste is disposed after a cooling time of 100 years (50 more thannormal), the needed gallery length can be reduced with a factor 4in comparison with scenario B1 and with a factor 13 in comparisonwith scenario A1.

• Longer cooling times would increase the reduction factors.

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 17

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

ILW: Waste Streams and Isotopic v.

Fractions of main chemical elements incorporated into the compacted ILW (%)

000000Carbon

100100100100100100Fuel Assembly Structurals

B2B1A3

0.20.20.20.20.20.2Others

100-----Zr of the ADS fuel matrix

(also for the Zr-fission product)

0.20.20.20.20.20.2Chlorine

Blankets + Core (FR)

40

0.2

0.2

1

0

0.02

0.02

MOX (PWR)

Extended PUREX

40

0.2

100

1

0

0.02

0.02

ZrN +TRUN(ADS)

PYRO

40

0.2

0.2

1

0

0.02

0.02

UOX (PWR)

Extended PUREX

Blankets + Core (FR)UOX (PWR)REPROCESSED FUEL

404040HLIGHT

ELEMENTS(Fuel Impurities)

0.20.20.2Others

111Iodine

Noble Metals

Noble Gases

MA

U and Pu

FISSION PRODUCTS

(FP)

ACTINIDES(An)

REPROCESSING TYPE

SCENARIO

Extended PUREX

Standard PUREX

Standard PUREX

0.20.20.2

000

0.020.020.02

0.020.020.02

A2

000000Carbon

100100100100100100Fuel Assembly Structurals

B2B1A3

0.20.20.20.20.20.2Others

100-----Zr of the ADS fuel matrix

(also for the Zr-fission product)

0.20.20.20.20.20.2Chlorine

Blankets + Core (FR)

40

0.2

0.2

1

0

0.02

0.02

MOX (PWR)

Extended PUREX

40

0.2

100

1

0

0.02

0.02

ZrN +TRUN(ADS)

PYRO

40

0.2

0.2

1

0

0.02

0.02

UOX (PWR)

Extended PUREX

Blankets + Core (FR)UOX (PWR)REPROCESSED FUEL

404040HLIGHT

ELEMENTS(Fuel Impurities)

0.20.20.2Others

111Iodine

Noble Metals

Noble Gases

MA

U and Pu

FISSION PRODUCTS

(FP)

ACTINIDES(An)

REPROCESSING TYPE

SCENARIO

Extended PUREX

Standard PUREX

Standard PUREX

0.20.20.2

000

0.020.020.02

0.020.020.02

A2

Red-Impact – ILW hypothesis

Large amounts of ILW can compromise the capacity improvements from the HLW heat reductions

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 18

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Number of Waste PackagesRed-Impact- HLW waste packages

HLW forms and packages production per scenario

Scenario A1 A2 A3 B1 B2

Fuel Type LWR-UOx LWR-MOx LWR-UOx (reproc.)

FR-MOx (reproc.)

FR-MOx (reproc.)

LWR-UOx (reproc.)

LWR-MOx (reproc.)

ADS TRU-Nitride

(reproc.) Waste Forms per

tHM 2.18 2.21 1.12 2.09 1.98 1.08 1.07 2.61

tHM / TWeh 2.46 0.25 2.21 1.15 1.15 1.91 0.24 0.12

Waste Forms per TWe/h 5.35 SFA 0.54 SFA 2.48 UC-V 2.40 UC-V 2.27 UC-V 2.07 UC-V 0.26 UC-V 0.33 UC-V

Waste Forms per HLW Package 4 1 1 1 1 1 1 1

Waste Packages per TWeh 1.34 0.54 2.48 2.40 2.27 2.07 0.26 0.33

Package Volume (m3)

2.89 1.51 0.53 0.53 0.53 0.53 0.53 0.53

HLWs Volume (m3/TWeh)

3.87 0.82 1.32 1.27 1.21 1.10 0.14 0.17

HLWs TOTAL Volume (m3/TWeh)

3.87 2.14 1.27 1.21 1.41

Red-Impact- ILW waste packagesILW forms and packages production per scenario

Scenario A1 A2 A3 B1 B2

Fuel Type LWR-UOx

LWR-MOx

LWR-UOx

(reproc.)

FR-MOx (reproc.)

FR-MOx (reproc.)

LWR-UOx (reproc.)

LWR-MOx (reproc.)

ADS-TRU Nitride

(reproc.)

ADS (operation)

Waste Forms per tHM - - 1.00 4.10 4.10 1.00 1.01 6.22 0.27

tHM / TWeh 2.46 0.25 2.21 1.15 1.15 1.91 0.24 0.12 0.12

Waste Forms per TWe/h - - 2.21 4.71 4.71 1.91 0.24 0.78 0.03

Waste Forms per ILW Package - - 4 4 4 4 4 4 4

Waste Packages per TWeh - - 0.55 1.18 1.18 0.48 0.06 0.19 0.01

Package Volume (m3)

- - 4.5 4.5 4.5 4.5 4.5 4.5 4.5

ILWs Volume (m3/TWeh)

- - 2.49 5.31 5.31 2.15 0.27 0.87 0.04

ILWs TOTAL Volume

(m3/TWeh) - 2.49 5.31 5.31 3.33

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 19

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

ILW: Waste Streams and Isotopic v.

Red-Impact relevant fission and activation products in the solid wastes (HLWs + ILWs)

AIAI

AI = Activation of impurities in fuel or structural materials

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 20

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

HLW + ILW: RadiotoxicityRed-Impact HLWs and ILWs radiotoxicity

evolution with time

1E+02

1E+03

1E+04

1E+05

1E+06

1E+07

1E+08

1E+09

1 10 100 1,000 10,000 100,000 1,000,000

TIME AFTER FUEL UNLOADING (YEARS)

RA

DIO

TOXI

C IN

VEN

TOR

Y (S

v/TW

eh)

A2 HLW A2 ILW A2 RepU

A3 HLW A3 ILW A3 RepU

B1 HLW B1 ILW B1 RepU

B2 HLW B2 ILW B2 RepU

A1

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 21

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Individual Dose from repository: HLW A1 in Granite-H

glass is assumed to dissolve completely in 72000 years

Vitrified HLW A2 in Granite-H72000 y

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 22

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Individual Dose from repository: HLW

Granite-H

Note that the matrix lifetime has a strong effect on doses due to the mobile fission and activation products such as 129I, 14C and 36Cl

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 23

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Individual Dose from repository: HLW

B-Clay

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 24

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

B-Clay

Individual Dose from repository: HLW

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 25

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Salt (altered evolution)

Individual Dose from repository: HLW

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 26

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

• For all considered host formations, the impact of P&T on the maximum doseis limited, because the maximum dose is essentially due to long-lived fissionproducts.

• One of the most important contributors to the total dose is 129I. The amountof 129I going into the repository as HLW very strongly depends on thefraction of spent fuel that is reprocessed.

• For those long-lived fission products that pass to the HLW duringreprocessing (79Se, 126Sn and 135Cs) doses arising from the differentscenarios are quite similar.

• For 129I and 14C and 36Cl (activation products) the inventories in the HLWare much smaller than in the original fuel, because large fractions of thoseelements have been released as effluents.

• The decrease in doses due to 129I, 14C and 36Cl in the scenarios withreprocessing is a consequence of the reduced inventory in the HLW.

• The transmutation of most actinides in fast reactors or accelerator-drivensystems in case of advanced fuel cycle scenarios has little impact on theresulting doses, because the low solubility of the actinides in reducingconditions and the strong sorption on minerals present in the buffer and hostformation .

• When the waste disposal configuration is adapted to the thermal output ofthe disposed waste, the higher disposal density in case of advanced fuelcycles can result in a decrease of the release rate of solubility limitedradionuclides (79Se, 99Tc and 126Sn,) in case of disposal.

Individual Dose from repository: HLW

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 27

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Individual Dose from repository: ILW

A2 B2

A3/B1

Dose from ILW dominated by I129, Cl36, C14, Cs135.It was assumed that the waste matrix does not provide any isolation

ILW in Granite-H

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 28

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Individual Dose from repository: ILW

ILW in B-Clay

The the main contributors to the total dose are 129I, 36Cl and 79Se. The matrix lifetime was taken equal to 1000 years.

In B-Clay, the about 50-m thick clay barrier spreads the release of mobile fission and activation products from the host clay formation into the surrounding aquifer layers over several tens of thousands of years, minimizing their radiotoxicity at release time.

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 29

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Dose Human intrusion

Annual dose in the geotechnical worker scenario, for 8 HLW and SF types vs Cigar Lake Uranium ore body and ICRP intervention levels

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 30

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

Time dependent Scenarios

Transition Scenarios: A1 to A3 or B1

Transition Scenarios: A1 to B2

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 31

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

1000

2000

3000

4000

5000

6000

7000

2000 2010 2020 2030 2040 2050 2060 2070 2080 2090 2100 2110 2120 2130 2140 2150 2160 2170 2180 2190 2200

YEAR

WP

per y

ear

TSA3 (total WPs: 411 641)

TSB1 (total WPs: 393 953)

TSB2 (total WPs: 441 243)

Annual production of HLW packages in Transition Scenarios

Detailed and well anticipated planning is needed to achieve equilibrated and optimized facilities and resources utilization.

Time dependent Scenarios

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 32

Scenario

Mass flow

Isotopic V.

Waste Strs:HLW, ILW,…

Heat, RdTx, RdAc,

Repository C

Volume

P.A.: Doses

Varia

nts

& T

ime

Dep

ende

nt S

cena

rios

Packages

1E+8

1E+9

1E+10

1E+11

1E+12

1E+13

1E+14

1 10 100 1,000 10,000 100,000 1,000,000

Time after Fuel Unloading (years) - Reprocessing at time = 5 years (2y for pyro-reprocessing)

Rad

ioto

xic

Inve

ntor

y (S

v)

A3 Transition HLW A3 Equilibrium HLW

B1 Transition HLW B1 Equilibrium HLW

B2 Transition HLW B2 Equilibrium HLW

A3 Transition Rep-U B1 Transition Rep-U

B2 Transition Rep-U A1

Radiotoxicity inventories for transition scenarios

Optimized program of reprocessing as a function of technology maturity to achieve maximum improvements on radiotoxicity inventory and capacity of the repository.

Time dependent Scenarios

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 33

Red-Impact main conclusions

FP6 RED-IMPACT project has extended the 2002 & 2006 NEA/OCDE studies on P&T adding improvements on:

• A more complete evaluation of wastes:─ intermediate level wastes, ILW, ─ more detailed structural materials and fuel impurities activation─ the activation of all the specific components of the ADS (spallation

target structural materials and coolant activation, spallation products activation,…).

• More details in the Cs & Sr separate handling scenarios,• The performance assessment, including in this case the handling of the

ILW, has been improved,• A large effort to evaluate the transition process from the present European

situation to hypothetical future scenarios.• A first methodology to include indicators for all aspects related to waste

management (technical, economical, social, environmental,…) in a single evaluation mechanism

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Summary of RED-IMPACT results on the Impact of P&T… IEMPT10 / Mito (Japan) E.M. Gonzalez 34

Red-Impact main conclusions • P&T reduces the final waste Radiotoxicity and its Thermal Load from the wastes to

the repository, and strongly accelerates the Thermal load decay after 100 years.• This will allow to reduce the gallery length required for HLW in granite and clay

repositories, increasing their capacity (factor 1.6-6). The effect is enhanced bydelaying disposal to >100y from discharge, separating Sr &Cs handling or both.

• There is small or no advantage from P&T on the dose to the average member ofthe critical group from the normal evolution scenarios. But significant advantage forimprovable human intrusion scenarios.

• ILW could compromise the advantages if prevention is not taken:─ Large volume of ILW (where to store then, compacted packages?, …)─ Dose to average individual larger than from HLW (how to isolate then?)

• Transition scenarios show the importance of long term planning of resources andinfrastructure availability for the feasibility and performance of P&T.

• Transition scenarios indicates that using early P&T technology before is fullyfunctional (MA handling) might limit the final performance for scenarios mainlyoriented to reduction of wastes (like reduction of nuclear park).

• Independently of the minimization technologies used, there will be always need ofhighly isolated final repository for the residual (losses,…) HLW.